Towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production
Abstract Lignocellulosic biomass is considered as a recalcitrant substrate for anaerobic digestion due to its complex nature that limits its biological degradation. Therefore, suitable preprocessing for the improvement of the performance of conventional anaerobic digestion remains a challenge in the...
Ausführliche Beschreibung
Autor*in: |
Novakovic, Jelica [verfasserIn] Kontogianni, Nikoleta [verfasserIn] Barampouti, Elli Maria [verfasserIn] Mai, Sofia [verfasserIn] Moustakas, Konstantinos [verfasserIn] Malamis, Dimitris [verfasserIn] Loizidou, Maria [verfasserIn] |
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Format: |
E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2020 |
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Schlagwörter: |
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Anmerkung: |
© Springer-Verlag GmbH Germany, part of Springer Nature 2020 |
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Übergeordnetes Werk: |
Enthalten in: Environmental science and pollution research - Berlin : Springer, 1994, 28(2020), 19 vom: 28. Apr., Seite 24486-24498 |
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Übergeordnetes Werk: |
volume:28 ; year:2020 ; number:19 ; day:28 ; month:04 ; pages:24486-24498 |
Links: |
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DOI / URN: |
10.1007/s11356-020-08905-y |
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Katalog-ID: |
SPR044127014 |
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520 | |a Abstract Lignocellulosic biomass is considered as a recalcitrant substrate for anaerobic digestion due to its complex nature that limits its biological degradation. Therefore, suitable preprocessing for the improvement of the performance of conventional anaerobic digestion remains a challenge in the development of anaerobic digestion technology. The physical and chemical characteristics of wheat straw (WS), as a representative lignocellulosic biomass, have a significant impact on the anaerobic digestion process in terms of quantity and quality of the produced biogas. This study aimed at investigating the enzymatic saccharification and detoxification of straw prior to anaerobic digestion with the final objective of enhancing the performance of conventional anaerobic systems of recalcitrant fractions of agricultural waste. The experimental activity was performed in lab and pilot scale treating WS. Alkaline delignification of straw using sodium hydroxide (NaOH) was studied prior to enzymatic hydrolysis for the production of easily biodegradable sugars. After defining the optimum conditions for the pretreatment scheme, the anaerobic digestability of the effluents produced was measured. Finally, the final liquid effluents were fed to a pilot scale anaerobic digester of 0.5 $ m^{3} $ volume, applying an increasing organic loading rate (OLR) regime (in terms of chemical oxygen demand (COD) from 0.2 to 15 kg COD/$ m^{3} $/day). The optimum conditions for the delignification and enzymatic hydrolysis of WS were defined as 0.5 M NaOH at 50 °C for 3–5 h and 15 μL Cellic CTec2/g pretreated straw at 50 °C. It was proven that the resulting liquid effluents could be fed to an anaerobic digester in the ratio that they are produced with satisfactory COD removal efficiencies (over 70%) for OLRs up to 10 kg COD/$ m^{3} $/day. This value is correspondent to a hydraulic retention time of around 7.5 days, much lower than the respective one for untreated straw (over 12 days). | ||
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700 | 1 | |a Malamis, Dimitris |e verfasserin |4 aut | |
700 | 1 | |a Loizidou, Maria |e verfasserin |4 aut | |
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10.1007/s11356-020-08905-y doi (DE-627)SPR044127014 (DE-599)SPRs11356-020-08905-y-e (SPR)s11356-020-08905-y-e DE-627 ger DE-627 rakwb eng 333.7 690 ASE 43.00 bkl 43.50 bkl 58.50 bkl Novakovic, Jelica verfasserin aut Towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2020 Abstract Lignocellulosic biomass is considered as a recalcitrant substrate for anaerobic digestion due to its complex nature that limits its biological degradation. Therefore, suitable preprocessing for the improvement of the performance of conventional anaerobic digestion remains a challenge in the development of anaerobic digestion technology. The physical and chemical characteristics of wheat straw (WS), as a representative lignocellulosic biomass, have a significant impact on the anaerobic digestion process in terms of quantity and quality of the produced biogas. This study aimed at investigating the enzymatic saccharification and detoxification of straw prior to anaerobic digestion with the final objective of enhancing the performance of conventional anaerobic systems of recalcitrant fractions of agricultural waste. The experimental activity was performed in lab and pilot scale treating WS. Alkaline delignification of straw using sodium hydroxide (NaOH) was studied prior to enzymatic hydrolysis for the production of easily biodegradable sugars. After defining the optimum conditions for the pretreatment scheme, the anaerobic digestability of the effluents produced was measured. Finally, the final liquid effluents were fed to a pilot scale anaerobic digester of 0.5 $ m^{3} $ volume, applying an increasing organic loading rate (OLR) regime (in terms of chemical oxygen demand (COD) from 0.2 to 15 kg COD/$ m^{3} $/day). The optimum conditions for the delignification and enzymatic hydrolysis of WS were defined as 0.5 M NaOH at 50 °C for 3–5 h and 15 μL Cellic CTec2/g pretreated straw at 50 °C. It was proven that the resulting liquid effluents could be fed to an anaerobic digester in the ratio that they are produced with satisfactory COD removal efficiencies (over 70%) for OLRs up to 10 kg COD/$ m^{3} $/day. This value is correspondent to a hydraulic retention time of around 7.5 days, much lower than the respective one for untreated straw (over 12 days). Anaerobic digestion (dpeaa)DE-He213 Delignification (dpeaa)DE-He213 Enzyme loading (dpeaa)DE-He213 Particle size (dpeaa)DE-He213 Scale-up (dpeaa)DE-He213 Sugars yield (dpeaa)DE-He213 Kontogianni, Nikoleta verfasserin aut Barampouti, Elli Maria verfasserin aut Mai, Sofia verfasserin aut Moustakas, Konstantinos verfasserin aut Malamis, Dimitris verfasserin aut Loizidou, Maria verfasserin aut Enthalten in Environmental science and pollution research Berlin : Springer, 1994 28(2020), 19 vom: 28. Apr., Seite 24486-24498 (DE-627)320517926 (DE-600)2014192-0 1614-7499 nnns volume:28 year:2020 number:19 day:28 month:04 pages:24486-24498 https://dx.doi.org/10.1007/s11356-020-08905-y lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OPC-GGO SSG-OPC-ASE GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 43.00 ASE 43.50 ASE 58.50 ASE AR 28 2020 19 28 04 24486-24498 |
spelling |
10.1007/s11356-020-08905-y doi (DE-627)SPR044127014 (DE-599)SPRs11356-020-08905-y-e (SPR)s11356-020-08905-y-e DE-627 ger DE-627 rakwb eng 333.7 690 ASE 43.00 bkl 43.50 bkl 58.50 bkl Novakovic, Jelica verfasserin aut Towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2020 Abstract Lignocellulosic biomass is considered as a recalcitrant substrate for anaerobic digestion due to its complex nature that limits its biological degradation. Therefore, suitable preprocessing for the improvement of the performance of conventional anaerobic digestion remains a challenge in the development of anaerobic digestion technology. The physical and chemical characteristics of wheat straw (WS), as a representative lignocellulosic biomass, have a significant impact on the anaerobic digestion process in terms of quantity and quality of the produced biogas. This study aimed at investigating the enzymatic saccharification and detoxification of straw prior to anaerobic digestion with the final objective of enhancing the performance of conventional anaerobic systems of recalcitrant fractions of agricultural waste. The experimental activity was performed in lab and pilot scale treating WS. Alkaline delignification of straw using sodium hydroxide (NaOH) was studied prior to enzymatic hydrolysis for the production of easily biodegradable sugars. After defining the optimum conditions for the pretreatment scheme, the anaerobic digestability of the effluents produced was measured. Finally, the final liquid effluents were fed to a pilot scale anaerobic digester of 0.5 $ m^{3} $ volume, applying an increasing organic loading rate (OLR) regime (in terms of chemical oxygen demand (COD) from 0.2 to 15 kg COD/$ m^{3} $/day). The optimum conditions for the delignification and enzymatic hydrolysis of WS were defined as 0.5 M NaOH at 50 °C for 3–5 h and 15 μL Cellic CTec2/g pretreated straw at 50 °C. It was proven that the resulting liquid effluents could be fed to an anaerobic digester in the ratio that they are produced with satisfactory COD removal efficiencies (over 70%) for OLRs up to 10 kg COD/$ m^{3} $/day. This value is correspondent to a hydraulic retention time of around 7.5 days, much lower than the respective one for untreated straw (over 12 days). Anaerobic digestion (dpeaa)DE-He213 Delignification (dpeaa)DE-He213 Enzyme loading (dpeaa)DE-He213 Particle size (dpeaa)DE-He213 Scale-up (dpeaa)DE-He213 Sugars yield (dpeaa)DE-He213 Kontogianni, Nikoleta verfasserin aut Barampouti, Elli Maria verfasserin aut Mai, Sofia verfasserin aut Moustakas, Konstantinos verfasserin aut Malamis, Dimitris verfasserin aut Loizidou, Maria verfasserin aut Enthalten in Environmental science and pollution research Berlin : Springer, 1994 28(2020), 19 vom: 28. Apr., Seite 24486-24498 (DE-627)320517926 (DE-600)2014192-0 1614-7499 nnns volume:28 year:2020 number:19 day:28 month:04 pages:24486-24498 https://dx.doi.org/10.1007/s11356-020-08905-y lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OPC-GGO SSG-OPC-ASE GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 43.00 ASE 43.50 ASE 58.50 ASE AR 28 2020 19 28 04 24486-24498 |
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10.1007/s11356-020-08905-y doi (DE-627)SPR044127014 (DE-599)SPRs11356-020-08905-y-e (SPR)s11356-020-08905-y-e DE-627 ger DE-627 rakwb eng 333.7 690 ASE 43.00 bkl 43.50 bkl 58.50 bkl Novakovic, Jelica verfasserin aut Towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2020 Abstract Lignocellulosic biomass is considered as a recalcitrant substrate for anaerobic digestion due to its complex nature that limits its biological degradation. Therefore, suitable preprocessing for the improvement of the performance of conventional anaerobic digestion remains a challenge in the development of anaerobic digestion technology. The physical and chemical characteristics of wheat straw (WS), as a representative lignocellulosic biomass, have a significant impact on the anaerobic digestion process in terms of quantity and quality of the produced biogas. This study aimed at investigating the enzymatic saccharification and detoxification of straw prior to anaerobic digestion with the final objective of enhancing the performance of conventional anaerobic systems of recalcitrant fractions of agricultural waste. The experimental activity was performed in lab and pilot scale treating WS. Alkaline delignification of straw using sodium hydroxide (NaOH) was studied prior to enzymatic hydrolysis for the production of easily biodegradable sugars. After defining the optimum conditions for the pretreatment scheme, the anaerobic digestability of the effluents produced was measured. Finally, the final liquid effluents were fed to a pilot scale anaerobic digester of 0.5 $ m^{3} $ volume, applying an increasing organic loading rate (OLR) regime (in terms of chemical oxygen demand (COD) from 0.2 to 15 kg COD/$ m^{3} $/day). The optimum conditions for the delignification and enzymatic hydrolysis of WS were defined as 0.5 M NaOH at 50 °C for 3–5 h and 15 μL Cellic CTec2/g pretreated straw at 50 °C. It was proven that the resulting liquid effluents could be fed to an anaerobic digester in the ratio that they are produced with satisfactory COD removal efficiencies (over 70%) for OLRs up to 10 kg COD/$ m^{3} $/day. This value is correspondent to a hydraulic retention time of around 7.5 days, much lower than the respective one for untreated straw (over 12 days). Anaerobic digestion (dpeaa)DE-He213 Delignification (dpeaa)DE-He213 Enzyme loading (dpeaa)DE-He213 Particle size (dpeaa)DE-He213 Scale-up (dpeaa)DE-He213 Sugars yield (dpeaa)DE-He213 Kontogianni, Nikoleta verfasserin aut Barampouti, Elli Maria verfasserin aut Mai, Sofia verfasserin aut Moustakas, Konstantinos verfasserin aut Malamis, Dimitris verfasserin aut Loizidou, Maria verfasserin aut Enthalten in Environmental science and pollution research Berlin : Springer, 1994 28(2020), 19 vom: 28. Apr., Seite 24486-24498 (DE-627)320517926 (DE-600)2014192-0 1614-7499 nnns volume:28 year:2020 number:19 day:28 month:04 pages:24486-24498 https://dx.doi.org/10.1007/s11356-020-08905-y lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OPC-GGO SSG-OPC-ASE GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 43.00 ASE 43.50 ASE 58.50 ASE AR 28 2020 19 28 04 24486-24498 |
allfieldsGer |
10.1007/s11356-020-08905-y doi (DE-627)SPR044127014 (DE-599)SPRs11356-020-08905-y-e (SPR)s11356-020-08905-y-e DE-627 ger DE-627 rakwb eng 333.7 690 ASE 43.00 bkl 43.50 bkl 58.50 bkl Novakovic, Jelica verfasserin aut Towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2020 Abstract Lignocellulosic biomass is considered as a recalcitrant substrate for anaerobic digestion due to its complex nature that limits its biological degradation. Therefore, suitable preprocessing for the improvement of the performance of conventional anaerobic digestion remains a challenge in the development of anaerobic digestion technology. The physical and chemical characteristics of wheat straw (WS), as a representative lignocellulosic biomass, have a significant impact on the anaerobic digestion process in terms of quantity and quality of the produced biogas. This study aimed at investigating the enzymatic saccharification and detoxification of straw prior to anaerobic digestion with the final objective of enhancing the performance of conventional anaerobic systems of recalcitrant fractions of agricultural waste. The experimental activity was performed in lab and pilot scale treating WS. Alkaline delignification of straw using sodium hydroxide (NaOH) was studied prior to enzymatic hydrolysis for the production of easily biodegradable sugars. After defining the optimum conditions for the pretreatment scheme, the anaerobic digestability of the effluents produced was measured. Finally, the final liquid effluents were fed to a pilot scale anaerobic digester of 0.5 $ m^{3} $ volume, applying an increasing organic loading rate (OLR) regime (in terms of chemical oxygen demand (COD) from 0.2 to 15 kg COD/$ m^{3} $/day). The optimum conditions for the delignification and enzymatic hydrolysis of WS were defined as 0.5 M NaOH at 50 °C for 3–5 h and 15 μL Cellic CTec2/g pretreated straw at 50 °C. It was proven that the resulting liquid effluents could be fed to an anaerobic digester in the ratio that they are produced with satisfactory COD removal efficiencies (over 70%) for OLRs up to 10 kg COD/$ m^{3} $/day. This value is correspondent to a hydraulic retention time of around 7.5 days, much lower than the respective one for untreated straw (over 12 days). Anaerobic digestion (dpeaa)DE-He213 Delignification (dpeaa)DE-He213 Enzyme loading (dpeaa)DE-He213 Particle size (dpeaa)DE-He213 Scale-up (dpeaa)DE-He213 Sugars yield (dpeaa)DE-He213 Kontogianni, Nikoleta verfasserin aut Barampouti, Elli Maria verfasserin aut Mai, Sofia verfasserin aut Moustakas, Konstantinos verfasserin aut Malamis, Dimitris verfasserin aut Loizidou, Maria verfasserin aut Enthalten in Environmental science and pollution research Berlin : Springer, 1994 28(2020), 19 vom: 28. Apr., Seite 24486-24498 (DE-627)320517926 (DE-600)2014192-0 1614-7499 nnns volume:28 year:2020 number:19 day:28 month:04 pages:24486-24498 https://dx.doi.org/10.1007/s11356-020-08905-y lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OPC-GGO SSG-OPC-ASE GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 43.00 ASE 43.50 ASE 58.50 ASE AR 28 2020 19 28 04 24486-24498 |
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10.1007/s11356-020-08905-y doi (DE-627)SPR044127014 (DE-599)SPRs11356-020-08905-y-e (SPR)s11356-020-08905-y-e DE-627 ger DE-627 rakwb eng 333.7 690 ASE 43.00 bkl 43.50 bkl 58.50 bkl Novakovic, Jelica verfasserin aut Towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production 2020 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Springer-Verlag GmbH Germany, part of Springer Nature 2020 Abstract Lignocellulosic biomass is considered as a recalcitrant substrate for anaerobic digestion due to its complex nature that limits its biological degradation. Therefore, suitable preprocessing for the improvement of the performance of conventional anaerobic digestion remains a challenge in the development of anaerobic digestion technology. The physical and chemical characteristics of wheat straw (WS), as a representative lignocellulosic biomass, have a significant impact on the anaerobic digestion process in terms of quantity and quality of the produced biogas. This study aimed at investigating the enzymatic saccharification and detoxification of straw prior to anaerobic digestion with the final objective of enhancing the performance of conventional anaerobic systems of recalcitrant fractions of agricultural waste. The experimental activity was performed in lab and pilot scale treating WS. Alkaline delignification of straw using sodium hydroxide (NaOH) was studied prior to enzymatic hydrolysis for the production of easily biodegradable sugars. After defining the optimum conditions for the pretreatment scheme, the anaerobic digestability of the effluents produced was measured. Finally, the final liquid effluents were fed to a pilot scale anaerobic digester of 0.5 $ m^{3} $ volume, applying an increasing organic loading rate (OLR) regime (in terms of chemical oxygen demand (COD) from 0.2 to 15 kg COD/$ m^{3} $/day). The optimum conditions for the delignification and enzymatic hydrolysis of WS were defined as 0.5 M NaOH at 50 °C for 3–5 h and 15 μL Cellic CTec2/g pretreated straw at 50 °C. It was proven that the resulting liquid effluents could be fed to an anaerobic digester in the ratio that they are produced with satisfactory COD removal efficiencies (over 70%) for OLRs up to 10 kg COD/$ m^{3} $/day. This value is correspondent to a hydraulic retention time of around 7.5 days, much lower than the respective one for untreated straw (over 12 days). Anaerobic digestion (dpeaa)DE-He213 Delignification (dpeaa)DE-He213 Enzyme loading (dpeaa)DE-He213 Particle size (dpeaa)DE-He213 Scale-up (dpeaa)DE-He213 Sugars yield (dpeaa)DE-He213 Kontogianni, Nikoleta verfasserin aut Barampouti, Elli Maria verfasserin aut Mai, Sofia verfasserin aut Moustakas, Konstantinos verfasserin aut Malamis, Dimitris verfasserin aut Loizidou, Maria verfasserin aut Enthalten in Environmental science and pollution research Berlin : Springer, 1994 28(2020), 19 vom: 28. Apr., Seite 24486-24498 (DE-627)320517926 (DE-600)2014192-0 1614-7499 nnns volume:28 year:2020 number:19 day:28 month:04 pages:24486-24498 https://dx.doi.org/10.1007/s11356-020-08905-y lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OPC-GGO SSG-OPC-ASE GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 43.00 ASE 43.50 ASE 58.50 ASE AR 28 2020 19 28 04 24486-24498 |
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Enthalten in Environmental science and pollution research 28(2020), 19 vom: 28. Apr., Seite 24486-24498 volume:28 year:2020 number:19 day:28 month:04 pages:24486-24498 |
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Novakovic, Jelica @@aut@@ Kontogianni, Nikoleta @@aut@@ Barampouti, Elli Maria @@aut@@ Mai, Sofia @@aut@@ Moustakas, Konstantinos @@aut@@ Malamis, Dimitris @@aut@@ Loizidou, Maria @@aut@@ |
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Therefore, suitable preprocessing for the improvement of the performance of conventional anaerobic digestion remains a challenge in the development of anaerobic digestion technology. The physical and chemical characteristics of wheat straw (WS), as a representative lignocellulosic biomass, have a significant impact on the anaerobic digestion process in terms of quantity and quality of the produced biogas. This study aimed at investigating the enzymatic saccharification and detoxification of straw prior to anaerobic digestion with the final objective of enhancing the performance of conventional anaerobic systems of recalcitrant fractions of agricultural waste. The experimental activity was performed in lab and pilot scale treating WS. Alkaline delignification of straw using sodium hydroxide (NaOH) was studied prior to enzymatic hydrolysis for the production of easily biodegradable sugars. After defining the optimum conditions for the pretreatment scheme, the anaerobic digestability of the effluents produced was measured. Finally, the final liquid effluents were fed to a pilot scale anaerobic digester of 0.5 $ m^{3} $ volume, applying an increasing organic loading rate (OLR) regime (in terms of chemical oxygen demand (COD) from 0.2 to 15 kg COD/$ m^{3} $/day). The optimum conditions for the delignification and enzymatic hydrolysis of WS were defined as 0.5 M NaOH at 50 °C for 3–5 h and 15 μL Cellic CTec2/g pretreated straw at 50 °C. It was proven that the resulting liquid effluents could be fed to an anaerobic digester in the ratio that they are produced with satisfactory COD removal efficiencies (over 70%) for OLRs up to 10 kg COD/$ m^{3} $/day. 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|
author |
Novakovic, Jelica |
spellingShingle |
Novakovic, Jelica ddc 333.7 bkl 43.00 bkl 43.50 bkl 58.50 misc Anaerobic digestion misc Delignification misc Enzyme loading misc Particle size misc Scale-up misc Sugars yield Towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production |
authorStr |
Novakovic, Jelica |
ppnlink_with_tag_str_mv |
@@773@@(DE-627)320517926 |
format |
electronic Article |
dewey-ones |
333 - Economics of land & energy 690 - Buildings |
delete_txt_mv |
keep |
author_role |
aut aut aut aut aut aut aut |
collection |
springer |
remote_str |
true |
illustrated |
Not Illustrated |
issn |
1614-7499 |
topic_title |
333.7 690 ASE 43.00 bkl 43.50 bkl 58.50 bkl Towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production Anaerobic digestion (dpeaa)DE-He213 Delignification (dpeaa)DE-He213 Enzyme loading (dpeaa)DE-He213 Particle size (dpeaa)DE-He213 Scale-up (dpeaa)DE-He213 Sugars yield (dpeaa)DE-He213 |
topic |
ddc 333.7 bkl 43.00 bkl 43.50 bkl 58.50 misc Anaerobic digestion misc Delignification misc Enzyme loading misc Particle size misc Scale-up misc Sugars yield |
topic_unstemmed |
ddc 333.7 bkl 43.00 bkl 43.50 bkl 58.50 misc Anaerobic digestion misc Delignification misc Enzyme loading misc Particle size misc Scale-up misc Sugars yield |
topic_browse |
ddc 333.7 bkl 43.00 bkl 43.50 bkl 58.50 misc Anaerobic digestion misc Delignification misc Enzyme loading misc Particle size misc Scale-up misc Sugars yield |
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Elektronische Aufsätze Aufsätze Elektronische Ressource |
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Towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production |
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Towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production |
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Novakovic, Jelica |
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Novakovic, Jelica Kontogianni, Nikoleta Barampouti, Elli Maria Mai, Sofia Moustakas, Konstantinos Malamis, Dimitris Loizidou, Maria |
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towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production |
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Towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production |
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Abstract Lignocellulosic biomass is considered as a recalcitrant substrate for anaerobic digestion due to its complex nature that limits its biological degradation. Therefore, suitable preprocessing for the improvement of the performance of conventional anaerobic digestion remains a challenge in the development of anaerobic digestion technology. The physical and chemical characteristics of wheat straw (WS), as a representative lignocellulosic biomass, have a significant impact on the anaerobic digestion process in terms of quantity and quality of the produced biogas. This study aimed at investigating the enzymatic saccharification and detoxification of straw prior to anaerobic digestion with the final objective of enhancing the performance of conventional anaerobic systems of recalcitrant fractions of agricultural waste. The experimental activity was performed in lab and pilot scale treating WS. Alkaline delignification of straw using sodium hydroxide (NaOH) was studied prior to enzymatic hydrolysis for the production of easily biodegradable sugars. After defining the optimum conditions for the pretreatment scheme, the anaerobic digestability of the effluents produced was measured. Finally, the final liquid effluents were fed to a pilot scale anaerobic digester of 0.5 $ m^{3} $ volume, applying an increasing organic loading rate (OLR) regime (in terms of chemical oxygen demand (COD) from 0.2 to 15 kg COD/$ m^{3} $/day). The optimum conditions for the delignification and enzymatic hydrolysis of WS were defined as 0.5 M NaOH at 50 °C for 3–5 h and 15 μL Cellic CTec2/g pretreated straw at 50 °C. It was proven that the resulting liquid effluents could be fed to an anaerobic digester in the ratio that they are produced with satisfactory COD removal efficiencies (over 70%) for OLRs up to 10 kg COD/$ m^{3} $/day. This value is correspondent to a hydraulic retention time of around 7.5 days, much lower than the respective one for untreated straw (over 12 days). © Springer-Verlag GmbH Germany, part of Springer Nature 2020 |
abstractGer |
Abstract Lignocellulosic biomass is considered as a recalcitrant substrate for anaerobic digestion due to its complex nature that limits its biological degradation. Therefore, suitable preprocessing for the improvement of the performance of conventional anaerobic digestion remains a challenge in the development of anaerobic digestion technology. The physical and chemical characteristics of wheat straw (WS), as a representative lignocellulosic biomass, have a significant impact on the anaerobic digestion process in terms of quantity and quality of the produced biogas. This study aimed at investigating the enzymatic saccharification and detoxification of straw prior to anaerobic digestion with the final objective of enhancing the performance of conventional anaerobic systems of recalcitrant fractions of agricultural waste. The experimental activity was performed in lab and pilot scale treating WS. Alkaline delignification of straw using sodium hydroxide (NaOH) was studied prior to enzymatic hydrolysis for the production of easily biodegradable sugars. After defining the optimum conditions for the pretreatment scheme, the anaerobic digestability of the effluents produced was measured. Finally, the final liquid effluents were fed to a pilot scale anaerobic digester of 0.5 $ m^{3} $ volume, applying an increasing organic loading rate (OLR) regime (in terms of chemical oxygen demand (COD) from 0.2 to 15 kg COD/$ m^{3} $/day). The optimum conditions for the delignification and enzymatic hydrolysis of WS were defined as 0.5 M NaOH at 50 °C for 3–5 h and 15 μL Cellic CTec2/g pretreated straw at 50 °C. It was proven that the resulting liquid effluents could be fed to an anaerobic digester in the ratio that they are produced with satisfactory COD removal efficiencies (over 70%) for OLRs up to 10 kg COD/$ m^{3} $/day. This value is correspondent to a hydraulic retention time of around 7.5 days, much lower than the respective one for untreated straw (over 12 days). © Springer-Verlag GmbH Germany, part of Springer Nature 2020 |
abstract_unstemmed |
Abstract Lignocellulosic biomass is considered as a recalcitrant substrate for anaerobic digestion due to its complex nature that limits its biological degradation. Therefore, suitable preprocessing for the improvement of the performance of conventional anaerobic digestion remains a challenge in the development of anaerobic digestion technology. The physical and chemical characteristics of wheat straw (WS), as a representative lignocellulosic biomass, have a significant impact on the anaerobic digestion process in terms of quantity and quality of the produced biogas. This study aimed at investigating the enzymatic saccharification and detoxification of straw prior to anaerobic digestion with the final objective of enhancing the performance of conventional anaerobic systems of recalcitrant fractions of agricultural waste. The experimental activity was performed in lab and pilot scale treating WS. Alkaline delignification of straw using sodium hydroxide (NaOH) was studied prior to enzymatic hydrolysis for the production of easily biodegradable sugars. After defining the optimum conditions for the pretreatment scheme, the anaerobic digestability of the effluents produced was measured. Finally, the final liquid effluents were fed to a pilot scale anaerobic digester of 0.5 $ m^{3} $ volume, applying an increasing organic loading rate (OLR) regime (in terms of chemical oxygen demand (COD) from 0.2 to 15 kg COD/$ m^{3} $/day). The optimum conditions for the delignification and enzymatic hydrolysis of WS were defined as 0.5 M NaOH at 50 °C for 3–5 h and 15 μL Cellic CTec2/g pretreated straw at 50 °C. It was proven that the resulting liquid effluents could be fed to an anaerobic digester in the ratio that they are produced with satisfactory COD removal efficiencies (over 70%) for OLRs up to 10 kg COD/$ m^{3} $/day. This value is correspondent to a hydraulic retention time of around 7.5 days, much lower than the respective one for untreated straw (over 12 days). © Springer-Verlag GmbH Germany, part of Springer Nature 2020 |
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Towards upscaling the valorization of wheat straw residues: alkaline pretreatment using sodium hydroxide, enzymatic hydrolysis and biogas production |
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|
score |
7.39909 |