Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes

Highlights The fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically.The advantages and challenges of 2D perovskite light-emitting diodes (PeLED) have been also discussed, which may benefit the audient to get insight into the 2D perovsk...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Ren, Miao [verfasserIn] Cao, Sheng Zhao, Jialong Zou, Bingsuo Zeng, Ruosheng

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2021

Schlagwörter:	Two-dimension Perovskite Light-emitting diodes Optical properties

Anmerkung:	© The Author(s) 2021

Übergeordnetes Werk:	Enthalten in: Nano-Micro letters - Berlin : Springer, 2009, 13(2021), 1 vom: 02. Aug.
Übergeordnetes Werk:	volume:13 ; year:2021 ; number:1 ; day:02 ; month:08

Links:	Volltext

DOI / URN:	10.1007/s40820-021-00685-5

Katalog-ID:	SPR044729057

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520			\|a Highlights The fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically.The advantages and challenges of 2D perovskite light-emitting diodes (PeLED) have been also discussed, which may benefit the audient to get insight into the 2D perovskite materials as well as the resultant LED devices.An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided.
520			\|a Abstract Two-dimensional (2D) perovskites are known as one of the most promising luminescent materials due to their structural diversity and outstanding optoelectronic properties. Compared with 3D perovskites, 2D perovskites have natural quantum well structures, large exciton binding energy (Eb) and outstanding thermal stability, which shows great potential in the next-generation displays and solid-state lighting. In this review, the fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically. Based on the advantages of 2D perovskites, such as special energy funnel process, ultra-fast energy transfer, dense film and low efficiency roll-off, the remarkable achievements of 2D perovskite light-emitting diodes (PeLEDs) are summarized, and exciting challenges of 2D perovskite are also discussed. An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. This review provides an overview of the recent developments of 2D perovskite materials and LED applications, and outlining challenges for achieving the high-performance devices.
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allfields	10.1007/s40820-021-00685-5 doi (DE-627)SPR044729057 (SPR)s40820-021-00685-5-e DE-627 ger DE-627 rakwb eng Ren, Miao verfasserin aut Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2021 Highlights The fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically.The advantages and challenges of 2D perovskite light-emitting diodes (PeLED) have been also discussed, which may benefit the audient to get insight into the 2D perovskite materials as well as the resultant LED devices.An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. Abstract Two-dimensional (2D) perovskites are known as one of the most promising luminescent materials due to their structural diversity and outstanding optoelectronic properties. Compared with 3D perovskites, 2D perovskites have natural quantum well structures, large exciton binding energy (Eb) and outstanding thermal stability, which shows great potential in the next-generation displays and solid-state lighting. In this review, the fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically. Based on the advantages of 2D perovskites, such as special energy funnel process, ultra-fast energy transfer, dense film and low efficiency roll-off, the remarkable achievements of 2D perovskite light-emitting diodes (PeLEDs) are summarized, and exciting challenges of 2D perovskite are also discussed. An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. This review provides an overview of the recent developments of 2D perovskite materials and LED applications, and outlining challenges for achieving the high-performance devices. Two-dimension (dpeaa)DE-He213 Perovskite (dpeaa)DE-He213 Light-emitting diodes (dpeaa)DE-He213 Optical properties (dpeaa)DE-He213 Cao, Sheng aut Zhao, Jialong aut Zou, Bingsuo aut Zeng, Ruosheng aut Enthalten in Nano-Micro letters Berlin : Springer, 2009 13(2021), 1 vom: 02. Aug. (DE-627)680319581 (DE-600)2642093-4 2150-5551 nnns volume:13 year:2021 number:1 day:02 month:08 https://dx.doi.org/10.1007/s40820-021-00685-5 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_206 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2027 GBV_ILN_2055 GBV_ILN_2111 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 13 2021 1 02 08
spelling	10.1007/s40820-021-00685-5 doi (DE-627)SPR044729057 (SPR)s40820-021-00685-5-e DE-627 ger DE-627 rakwb eng Ren, Miao verfasserin aut Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2021 Highlights The fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically.The advantages and challenges of 2D perovskite light-emitting diodes (PeLED) have been also discussed, which may benefit the audient to get insight into the 2D perovskite materials as well as the resultant LED devices.An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. Abstract Two-dimensional (2D) perovskites are known as one of the most promising luminescent materials due to their structural diversity and outstanding optoelectronic properties. Compared with 3D perovskites, 2D perovskites have natural quantum well structures, large exciton binding energy (Eb) and outstanding thermal stability, which shows great potential in the next-generation displays and solid-state lighting. In this review, the fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically. Based on the advantages of 2D perovskites, such as special energy funnel process, ultra-fast energy transfer, dense film and low efficiency roll-off, the remarkable achievements of 2D perovskite light-emitting diodes (PeLEDs) are summarized, and exciting challenges of 2D perovskite are also discussed. An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. This review provides an overview of the recent developments of 2D perovskite materials and LED applications, and outlining challenges for achieving the high-performance devices. Two-dimension (dpeaa)DE-He213 Perovskite (dpeaa)DE-He213 Light-emitting diodes (dpeaa)DE-He213 Optical properties (dpeaa)DE-He213 Cao, Sheng aut Zhao, Jialong aut Zou, Bingsuo aut Zeng, Ruosheng aut Enthalten in Nano-Micro letters Berlin : Springer, 2009 13(2021), 1 vom: 02. Aug. (DE-627)680319581 (DE-600)2642093-4 2150-5551 nnns volume:13 year:2021 number:1 day:02 month:08 https://dx.doi.org/10.1007/s40820-021-00685-5 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_206 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2027 GBV_ILN_2055 GBV_ILN_2111 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 13 2021 1 02 08
allfields_unstemmed	10.1007/s40820-021-00685-5 doi (DE-627)SPR044729057 (SPR)s40820-021-00685-5-e DE-627 ger DE-627 rakwb eng Ren, Miao verfasserin aut Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2021 Highlights The fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically.The advantages and challenges of 2D perovskite light-emitting diodes (PeLED) have been also discussed, which may benefit the audient to get insight into the 2D perovskite materials as well as the resultant LED devices.An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. Abstract Two-dimensional (2D) perovskites are known as one of the most promising luminescent materials due to their structural diversity and outstanding optoelectronic properties. Compared with 3D perovskites, 2D perovskites have natural quantum well structures, large exciton binding energy (Eb) and outstanding thermal stability, which shows great potential in the next-generation displays and solid-state lighting. In this review, the fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically. Based on the advantages of 2D perovskites, such as special energy funnel process, ultra-fast energy transfer, dense film and low efficiency roll-off, the remarkable achievements of 2D perovskite light-emitting diodes (PeLEDs) are summarized, and exciting challenges of 2D perovskite are also discussed. An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. This review provides an overview of the recent developments of 2D perovskite materials and LED applications, and outlining challenges for achieving the high-performance devices. Two-dimension (dpeaa)DE-He213 Perovskite (dpeaa)DE-He213 Light-emitting diodes (dpeaa)DE-He213 Optical properties (dpeaa)DE-He213 Cao, Sheng aut Zhao, Jialong aut Zou, Bingsuo aut Zeng, Ruosheng aut Enthalten in Nano-Micro letters Berlin : Springer, 2009 13(2021), 1 vom: 02. Aug. (DE-627)680319581 (DE-600)2642093-4 2150-5551 nnns volume:13 year:2021 number:1 day:02 month:08 https://dx.doi.org/10.1007/s40820-021-00685-5 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_206 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2027 GBV_ILN_2055 GBV_ILN_2111 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 13 2021 1 02 08
allfieldsGer	10.1007/s40820-021-00685-5 doi (DE-627)SPR044729057 (SPR)s40820-021-00685-5-e DE-627 ger DE-627 rakwb eng Ren, Miao verfasserin aut Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2021 Highlights The fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically.The advantages and challenges of 2D perovskite light-emitting diodes (PeLED) have been also discussed, which may benefit the audient to get insight into the 2D perovskite materials as well as the resultant LED devices.An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. Abstract Two-dimensional (2D) perovskites are known as one of the most promising luminescent materials due to their structural diversity and outstanding optoelectronic properties. Compared with 3D perovskites, 2D perovskites have natural quantum well structures, large exciton binding energy (Eb) and outstanding thermal stability, which shows great potential in the next-generation displays and solid-state lighting. In this review, the fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically. Based on the advantages of 2D perovskites, such as special energy funnel process, ultra-fast energy transfer, dense film and low efficiency roll-off, the remarkable achievements of 2D perovskite light-emitting diodes (PeLEDs) are summarized, and exciting challenges of 2D perovskite are also discussed. An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. This review provides an overview of the recent developments of 2D perovskite materials and LED applications, and outlining challenges for achieving the high-performance devices. Two-dimension (dpeaa)DE-He213 Perovskite (dpeaa)DE-He213 Light-emitting diodes (dpeaa)DE-He213 Optical properties (dpeaa)DE-He213 Cao, Sheng aut Zhao, Jialong aut Zou, Bingsuo aut Zeng, Ruosheng aut Enthalten in Nano-Micro letters Berlin : Springer, 2009 13(2021), 1 vom: 02. Aug. (DE-627)680319581 (DE-600)2642093-4 2150-5551 nnns volume:13 year:2021 number:1 day:02 month:08 https://dx.doi.org/10.1007/s40820-021-00685-5 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_206 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2027 GBV_ILN_2055 GBV_ILN_2111 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 13 2021 1 02 08
allfieldsSound	10.1007/s40820-021-00685-5 doi (DE-627)SPR044729057 (SPR)s40820-021-00685-5-e DE-627 ger DE-627 rakwb eng Ren, Miao verfasserin aut Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2021 Highlights The fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically.The advantages and challenges of 2D perovskite light-emitting diodes (PeLED) have been also discussed, which may benefit the audient to get insight into the 2D perovskite materials as well as the resultant LED devices.An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. Abstract Two-dimensional (2D) perovskites are known as one of the most promising luminescent materials due to their structural diversity and outstanding optoelectronic properties. Compared with 3D perovskites, 2D perovskites have natural quantum well structures, large exciton binding energy (Eb) and outstanding thermal stability, which shows great potential in the next-generation displays and solid-state lighting. In this review, the fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically. Based on the advantages of 2D perovskites, such as special energy funnel process, ultra-fast energy transfer, dense film and low efficiency roll-off, the remarkable achievements of 2D perovskite light-emitting diodes (PeLEDs) are summarized, and exciting challenges of 2D perovskite are also discussed. An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. This review provides an overview of the recent developments of 2D perovskite materials and LED applications, and outlining challenges for achieving the high-performance devices. Two-dimension (dpeaa)DE-He213 Perovskite (dpeaa)DE-He213 Light-emitting diodes (dpeaa)DE-He213 Optical properties (dpeaa)DE-He213 Cao, Sheng aut Zhao, Jialong aut Zou, Bingsuo aut Zeng, Ruosheng aut Enthalten in Nano-Micro letters Berlin : Springer, 2009 13(2021), 1 vom: 02. Aug. (DE-627)680319581 (DE-600)2642093-4 2150-5551 nnns volume:13 year:2021 number:1 day:02 month:08 https://dx.doi.org/10.1007/s40820-021-00685-5 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_39 GBV_ILN_40 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_95 GBV_ILN_105 GBV_ILN_110 GBV_ILN_151 GBV_ILN_161 GBV_ILN_206 GBV_ILN_213 GBV_ILN_230 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_2005 GBV_ILN_2009 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2027 GBV_ILN_2055 GBV_ILN_2111 GBV_ILN_4012 GBV_ILN_4037 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4249 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4335 GBV_ILN_4338 GBV_ILN_4367 GBV_ILN_4700 AR 13 2021 1 02 08
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source	Enthalten in Nano-Micro letters 13(2021), 1 vom: 02. Aug. volume:13 year:2021 number:1 day:02 month:08
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author	Ren, Miao
spellingShingle	Ren, Miao misc Two-dimension misc Perovskite misc Light-emitting diodes misc Optical properties Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes
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title	Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes
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title_full	Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes
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title_sort	advances and challenges in two-dimensional organic–inorganic hybrid perovskites toward high-performance light-emitting diodes
title_auth	Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes
abstract	Highlights The fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically.The advantages and challenges of 2D perovskite light-emitting diodes (PeLED) have been also discussed, which may benefit the audient to get insight into the 2D perovskite materials as well as the resultant LED devices.An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. Abstract Two-dimensional (2D) perovskites are known as one of the most promising luminescent materials due to their structural diversity and outstanding optoelectronic properties. Compared with 3D perovskites, 2D perovskites have natural quantum well structures, large exciton binding energy (Eb) and outstanding thermal stability, which shows great potential in the next-generation displays and solid-state lighting. In this review, the fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically. Based on the advantages of 2D perovskites, such as special energy funnel process, ultra-fast energy transfer, dense film and low efficiency roll-off, the remarkable achievements of 2D perovskite light-emitting diodes (PeLEDs) are summarized, and exciting challenges of 2D perovskite are also discussed. An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. This review provides an overview of the recent developments of 2D perovskite materials and LED applications, and outlining challenges for achieving the high-performance devices. © The Author(s) 2021
abstractGer	Highlights The fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically.The advantages and challenges of 2D perovskite light-emitting diodes (PeLED) have been also discussed, which may benefit the audient to get insight into the 2D perovskite materials as well as the resultant LED devices.An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. Abstract Two-dimensional (2D) perovskites are known as one of the most promising luminescent materials due to their structural diversity and outstanding optoelectronic properties. Compared with 3D perovskites, 2D perovskites have natural quantum well structures, large exciton binding energy (Eb) and outstanding thermal stability, which shows great potential in the next-generation displays and solid-state lighting. In this review, the fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically. Based on the advantages of 2D perovskites, such as special energy funnel process, ultra-fast energy transfer, dense film and low efficiency roll-off, the remarkable achievements of 2D perovskite light-emitting diodes (PeLEDs) are summarized, and exciting challenges of 2D perovskite are also discussed. An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. This review provides an overview of the recent developments of 2D perovskite materials and LED applications, and outlining challenges for achieving the high-performance devices. © The Author(s) 2021
abstract_unstemmed	Highlights The fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically.The advantages and challenges of 2D perovskite light-emitting diodes (PeLED) have been also discussed, which may benefit the audient to get insight into the 2D perovskite materials as well as the resultant LED devices.An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. Abstract Two-dimensional (2D) perovskites are known as one of the most promising luminescent materials due to their structural diversity and outstanding optoelectronic properties. Compared with 3D perovskites, 2D perovskites have natural quantum well structures, large exciton binding energy (Eb) and outstanding thermal stability, which shows great potential in the next-generation displays and solid-state lighting. In this review, the fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically. Based on the advantages of 2D perovskites, such as special energy funnel process, ultra-fast energy transfer, dense film and low efficiency roll-off, the remarkable achievements of 2D perovskite light-emitting diodes (PeLEDs) are summarized, and exciting challenges of 2D perovskite are also discussed. An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. This review provides an overview of the recent developments of 2D perovskite materials and LED applications, and outlining challenges for achieving the high-performance devices. © The Author(s) 2021
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title_short	Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes
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Compared with 3D perovskites, 2D perovskites have natural quantum well structures, large exciton binding energy (Eb) and outstanding thermal stability, which shows great potential in the next-generation displays and solid-state lighting. In this review, the fundamental structure, photophysical and electrical properties of 2D perovskite films were illustrated systematically. Based on the advantages of 2D perovskites, such as special energy funnel process, ultra-fast energy transfer, dense film and low efficiency roll-off, the remarkable achievements of 2D perovskite light-emitting diodes (PeLEDs) are summarized, and exciting challenges of 2D perovskite are also discussed. An outlook on further improving the efficiency of pure-blue PeLEDs, enhancing the operational stability of PeLEDs and reducing the toxicity to push this field forward was also provided. 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Advances and Challenges in Two-Dimensional Organic–Inorganic Hybrid Perovskites Toward High-Performance Light-Emitting Diodes

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