Quantum-efficiency enhancement and mechanical responsiveness of solid-state photoluminescent flexible materials containing uniaxial cellulose nanocrystal arrays
Abstract Assembling cellulose nanocrystals (CNCs) can induce solid-state photoluminescence based on Stokes scattering. Such photoluminescent materials are free of photo-quenching and show great potential in optical applications, whereas poor flexibility of assembled CNC arrays limits their applicati...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Liu, Siyuan [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2022 |
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| Schlagwörter: |
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| Anmerkung: |
© The Author(s), under exclusive licence to Springer Nature B.V. 2022 |
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| Übergeordnetes Werk: |
Enthalten in: Cellulose - Dordrecht [u.a.] : Springer Science + Business Media B.V, 1994, 29(2022), 3 vom: 17. Jan., Seite 1393-1403 |
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| Übergeordnetes Werk: |
volume:29 ; year:2022 ; number:3 ; day:17 ; month:01 ; pages:1393-1403 |
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| DOI / URN: |
10.1007/s10570-022-04424-w |
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| Katalog-ID: |
SPR046275398 |
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| 245 | 1 | 0 | |a Quantum-efficiency enhancement and mechanical responsiveness of solid-state photoluminescent flexible materials containing uniaxial cellulose nanocrystal arrays |
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| 520 | |a Abstract Assembling cellulose nanocrystals (CNCs) can induce solid-state photoluminescence based on Stokes scattering. Such photoluminescent materials are free of photo-quenching and show great potential in optical applications, whereas poor flexibility of assembled CNC arrays limits their applications. Here, a binary co-assembly of 1D nanoparticles and long-chain polymers was explored to produce the uniaxial CNC arrays into transparent poly(vinyl alcohol) (PVA) membranes, which enhanced the mechanical properties, especially ductility. Besides, the CNC assembly was controlled by adjusting the mass ratio between CNCs and PVA. The result indicated that co-assembling with PVA could improve the uniaxial orientation of CNC arrays, which played a crucial role in enhancing the emission quantum efficiency (EQE). Stretching the PVA/CNC membrane could further induce an enhancement in EQE together with a blue shift in excitation wavelength. The mechanism study on stimulation-response suggested that the EQE enhancement and blue shift came from the change in uniaxial orientation degree and periodicity of the CNC assembly, respectively. Since the stimulation-responsive enhancement in EQE (from ca. 40 to 60%) can even be observed by naked eyes, we believe such cellulose-based materials can be widely used in optical sensors. | ||
| 650 | 4 | |a Cellulose nanocrystals |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Poly(vinyl alcohol) |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Uniaxial assembly |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Mechanical responsiveness |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Luminescence enhancement |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Shi, Zhenxu |4 aut | |
| 700 | 1 | |a Wang, Xuhong |4 aut | |
| 700 | 1 | |a Gong, Yanbin |4 aut | |
| 700 | 1 | |a Li, Xijun |4 aut | |
| 700 | 1 | |a Jia, Xin |4 aut | |
| 700 | 1 | |a Gan, Lin |4 aut | |
| 700 | 1 | |a Huang, Jin |0 (orcid)0000-0003-0648-2525 |4 aut | |
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10.1007/s10570-022-04424-w doi (DE-627)SPR046275398 (SPR)s10570-022-04424-w-e DE-627 ger DE-627 rakwb eng Liu, Siyuan verfasserin aut Quantum-efficiency enhancement and mechanical responsiveness of solid-state photoluminescent flexible materials containing uniaxial cellulose nanocrystal arrays 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature B.V. 2022 Abstract Assembling cellulose nanocrystals (CNCs) can induce solid-state photoluminescence based on Stokes scattering. Such photoluminescent materials are free of photo-quenching and show great potential in optical applications, whereas poor flexibility of assembled CNC arrays limits their applications. Here, a binary co-assembly of 1D nanoparticles and long-chain polymers was explored to produce the uniaxial CNC arrays into transparent poly(vinyl alcohol) (PVA) membranes, which enhanced the mechanical properties, especially ductility. Besides, the CNC assembly was controlled by adjusting the mass ratio between CNCs and PVA. The result indicated that co-assembling with PVA could improve the uniaxial orientation of CNC arrays, which played a crucial role in enhancing the emission quantum efficiency (EQE). Stretching the PVA/CNC membrane could further induce an enhancement in EQE together with a blue shift in excitation wavelength. The mechanism study on stimulation-response suggested that the EQE enhancement and blue shift came from the change in uniaxial orientation degree and periodicity of the CNC assembly, respectively. Since the stimulation-responsive enhancement in EQE (from ca. 40 to 60%) can even be observed by naked eyes, we believe such cellulose-based materials can be widely used in optical sensors. Cellulose nanocrystals (dpeaa)DE-He213 Poly(vinyl alcohol) (dpeaa)DE-He213 Uniaxial assembly (dpeaa)DE-He213 Mechanical responsiveness (dpeaa)DE-He213 Luminescence enhancement (dpeaa)DE-He213 Shi, Zhenxu aut Wang, Xuhong aut Gong, Yanbin aut Li, Xijun aut Jia, Xin aut Gan, Lin aut Huang, Jin (orcid)0000-0003-0648-2525 aut Enthalten in Cellulose Dordrecht [u.a.] : Springer Science + Business Media B.V, 1994 29(2022), 3 vom: 17. Jan., Seite 1393-1403 (DE-627)306353857 (DE-600)1496831-9 1572-882X nnns volume:29 year:2022 number:3 day:17 month:01 pages:1393-1403 https://dx.doi.org/10.1007/s10570-022-04424-w lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 29 2022 3 17 01 1393-1403 |
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10.1007/s10570-022-04424-w doi (DE-627)SPR046275398 (SPR)s10570-022-04424-w-e DE-627 ger DE-627 rakwb eng Liu, Siyuan verfasserin aut Quantum-efficiency enhancement and mechanical responsiveness of solid-state photoluminescent flexible materials containing uniaxial cellulose nanocrystal arrays 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature B.V. 2022 Abstract Assembling cellulose nanocrystals (CNCs) can induce solid-state photoluminescence based on Stokes scattering. Such photoluminescent materials are free of photo-quenching and show great potential in optical applications, whereas poor flexibility of assembled CNC arrays limits their applications. Here, a binary co-assembly of 1D nanoparticles and long-chain polymers was explored to produce the uniaxial CNC arrays into transparent poly(vinyl alcohol) (PVA) membranes, which enhanced the mechanical properties, especially ductility. Besides, the CNC assembly was controlled by adjusting the mass ratio between CNCs and PVA. The result indicated that co-assembling with PVA could improve the uniaxial orientation of CNC arrays, which played a crucial role in enhancing the emission quantum efficiency (EQE). Stretching the PVA/CNC membrane could further induce an enhancement in EQE together with a blue shift in excitation wavelength. The mechanism study on stimulation-response suggested that the EQE enhancement and blue shift came from the change in uniaxial orientation degree and periodicity of the CNC assembly, respectively. Since the stimulation-responsive enhancement in EQE (from ca. 40 to 60%) can even be observed by naked eyes, we believe such cellulose-based materials can be widely used in optical sensors. Cellulose nanocrystals (dpeaa)DE-He213 Poly(vinyl alcohol) (dpeaa)DE-He213 Uniaxial assembly (dpeaa)DE-He213 Mechanical responsiveness (dpeaa)DE-He213 Luminescence enhancement (dpeaa)DE-He213 Shi, Zhenxu aut Wang, Xuhong aut Gong, Yanbin aut Li, Xijun aut Jia, Xin aut Gan, Lin aut Huang, Jin (orcid)0000-0003-0648-2525 aut Enthalten in Cellulose Dordrecht [u.a.] : Springer Science + Business Media B.V, 1994 29(2022), 3 vom: 17. Jan., Seite 1393-1403 (DE-627)306353857 (DE-600)1496831-9 1572-882X nnns volume:29 year:2022 number:3 day:17 month:01 pages:1393-1403 https://dx.doi.org/10.1007/s10570-022-04424-w lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 29 2022 3 17 01 1393-1403 |
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10.1007/s10570-022-04424-w doi (DE-627)SPR046275398 (SPR)s10570-022-04424-w-e DE-627 ger DE-627 rakwb eng Liu, Siyuan verfasserin aut Quantum-efficiency enhancement and mechanical responsiveness of solid-state photoluminescent flexible materials containing uniaxial cellulose nanocrystal arrays 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature B.V. 2022 Abstract Assembling cellulose nanocrystals (CNCs) can induce solid-state photoluminescence based on Stokes scattering. Such photoluminescent materials are free of photo-quenching and show great potential in optical applications, whereas poor flexibility of assembled CNC arrays limits their applications. Here, a binary co-assembly of 1D nanoparticles and long-chain polymers was explored to produce the uniaxial CNC arrays into transparent poly(vinyl alcohol) (PVA) membranes, which enhanced the mechanical properties, especially ductility. Besides, the CNC assembly was controlled by adjusting the mass ratio between CNCs and PVA. The result indicated that co-assembling with PVA could improve the uniaxial orientation of CNC arrays, which played a crucial role in enhancing the emission quantum efficiency (EQE). Stretching the PVA/CNC membrane could further induce an enhancement in EQE together with a blue shift in excitation wavelength. The mechanism study on stimulation-response suggested that the EQE enhancement and blue shift came from the change in uniaxial orientation degree and periodicity of the CNC assembly, respectively. Since the stimulation-responsive enhancement in EQE (from ca. 40 to 60%) can even be observed by naked eyes, we believe such cellulose-based materials can be widely used in optical sensors. Cellulose nanocrystals (dpeaa)DE-He213 Poly(vinyl alcohol) (dpeaa)DE-He213 Uniaxial assembly (dpeaa)DE-He213 Mechanical responsiveness (dpeaa)DE-He213 Luminescence enhancement (dpeaa)DE-He213 Shi, Zhenxu aut Wang, Xuhong aut Gong, Yanbin aut Li, Xijun aut Jia, Xin aut Gan, Lin aut Huang, Jin (orcid)0000-0003-0648-2525 aut Enthalten in Cellulose Dordrecht [u.a.] : Springer Science + Business Media B.V, 1994 29(2022), 3 vom: 17. Jan., Seite 1393-1403 (DE-627)306353857 (DE-600)1496831-9 1572-882X nnns volume:29 year:2022 number:3 day:17 month:01 pages:1393-1403 https://dx.doi.org/10.1007/s10570-022-04424-w lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 29 2022 3 17 01 1393-1403 |
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10.1007/s10570-022-04424-w doi (DE-627)SPR046275398 (SPR)s10570-022-04424-w-e DE-627 ger DE-627 rakwb eng Liu, Siyuan verfasserin aut Quantum-efficiency enhancement and mechanical responsiveness of solid-state photoluminescent flexible materials containing uniaxial cellulose nanocrystal arrays 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature B.V. 2022 Abstract Assembling cellulose nanocrystals (CNCs) can induce solid-state photoluminescence based on Stokes scattering. Such photoluminescent materials are free of photo-quenching and show great potential in optical applications, whereas poor flexibility of assembled CNC arrays limits their applications. Here, a binary co-assembly of 1D nanoparticles and long-chain polymers was explored to produce the uniaxial CNC arrays into transparent poly(vinyl alcohol) (PVA) membranes, which enhanced the mechanical properties, especially ductility. Besides, the CNC assembly was controlled by adjusting the mass ratio between CNCs and PVA. The result indicated that co-assembling with PVA could improve the uniaxial orientation of CNC arrays, which played a crucial role in enhancing the emission quantum efficiency (EQE). Stretching the PVA/CNC membrane could further induce an enhancement in EQE together with a blue shift in excitation wavelength. The mechanism study on stimulation-response suggested that the EQE enhancement and blue shift came from the change in uniaxial orientation degree and periodicity of the CNC assembly, respectively. Since the stimulation-responsive enhancement in EQE (from ca. 40 to 60%) can even be observed by naked eyes, we believe such cellulose-based materials can be widely used in optical sensors. Cellulose nanocrystals (dpeaa)DE-He213 Poly(vinyl alcohol) (dpeaa)DE-He213 Uniaxial assembly (dpeaa)DE-He213 Mechanical responsiveness (dpeaa)DE-He213 Luminescence enhancement (dpeaa)DE-He213 Shi, Zhenxu aut Wang, Xuhong aut Gong, Yanbin aut Li, Xijun aut Jia, Xin aut Gan, Lin aut Huang, Jin (orcid)0000-0003-0648-2525 aut Enthalten in Cellulose Dordrecht [u.a.] : Springer Science + Business Media B.V, 1994 29(2022), 3 vom: 17. Jan., Seite 1393-1403 (DE-627)306353857 (DE-600)1496831-9 1572-882X nnns volume:29 year:2022 number:3 day:17 month:01 pages:1393-1403 https://dx.doi.org/10.1007/s10570-022-04424-w lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 29 2022 3 17 01 1393-1403 |
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10.1007/s10570-022-04424-w doi (DE-627)SPR046275398 (SPR)s10570-022-04424-w-e DE-627 ger DE-627 rakwb eng Liu, Siyuan verfasserin aut Quantum-efficiency enhancement and mechanical responsiveness of solid-state photoluminescent flexible materials containing uniaxial cellulose nanocrystal arrays 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature B.V. 2022 Abstract Assembling cellulose nanocrystals (CNCs) can induce solid-state photoluminescence based on Stokes scattering. Such photoluminescent materials are free of photo-quenching and show great potential in optical applications, whereas poor flexibility of assembled CNC arrays limits their applications. Here, a binary co-assembly of 1D nanoparticles and long-chain polymers was explored to produce the uniaxial CNC arrays into transparent poly(vinyl alcohol) (PVA) membranes, which enhanced the mechanical properties, especially ductility. Besides, the CNC assembly was controlled by adjusting the mass ratio between CNCs and PVA. The result indicated that co-assembling with PVA could improve the uniaxial orientation of CNC arrays, which played a crucial role in enhancing the emission quantum efficiency (EQE). Stretching the PVA/CNC membrane could further induce an enhancement in EQE together with a blue shift in excitation wavelength. The mechanism study on stimulation-response suggested that the EQE enhancement and blue shift came from the change in uniaxial orientation degree and periodicity of the CNC assembly, respectively. Since the stimulation-responsive enhancement in EQE (from ca. 40 to 60%) can even be observed by naked eyes, we believe such cellulose-based materials can be widely used in optical sensors. Cellulose nanocrystals (dpeaa)DE-He213 Poly(vinyl alcohol) (dpeaa)DE-He213 Uniaxial assembly (dpeaa)DE-He213 Mechanical responsiveness (dpeaa)DE-He213 Luminescence enhancement (dpeaa)DE-He213 Shi, Zhenxu aut Wang, Xuhong aut Gong, Yanbin aut Li, Xijun aut Jia, Xin aut Gan, Lin aut Huang, Jin (orcid)0000-0003-0648-2525 aut Enthalten in Cellulose Dordrecht [u.a.] : Springer Science + Business Media B.V, 1994 29(2022), 3 vom: 17. Jan., Seite 1393-1403 (DE-627)306353857 (DE-600)1496831-9 1572-882X nnns volume:29 year:2022 number:3 day:17 month:01 pages:1393-1403 https://dx.doi.org/10.1007/s10570-022-04424-w lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 29 2022 3 17 01 1393-1403 |
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Enthalten in Cellulose 29(2022), 3 vom: 17. Jan., Seite 1393-1403 volume:29 year:2022 number:3 day:17 month:01 pages:1393-1403 |
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Cellulose nanocrystals Poly(vinyl alcohol) Uniaxial assembly Mechanical responsiveness Luminescence enhancement |
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Liu, Siyuan @@aut@@ Shi, Zhenxu @@aut@@ Wang, Xuhong @@aut@@ Gong, Yanbin @@aut@@ Li, Xijun @@aut@@ Jia, Xin @@aut@@ Gan, Lin @@aut@@ Huang, Jin @@aut@@ |
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Liu, Siyuan |
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Liu, Siyuan misc Cellulose nanocrystals misc Poly(vinyl alcohol) misc Uniaxial assembly misc Mechanical responsiveness misc Luminescence enhancement Quantum-efficiency enhancement and mechanical responsiveness of solid-state photoluminescent flexible materials containing uniaxial cellulose nanocrystal arrays |
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Quantum-efficiency enhancement and mechanical responsiveness of solid-state photoluminescent flexible materials containing uniaxial cellulose nanocrystal arrays Cellulose nanocrystals (dpeaa)DE-He213 Poly(vinyl alcohol) (dpeaa)DE-He213 Uniaxial assembly (dpeaa)DE-He213 Mechanical responsiveness (dpeaa)DE-He213 Luminescence enhancement (dpeaa)DE-He213 |
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quantum-efficiency enhancement and mechanical responsiveness of solid-state photoluminescent flexible materials containing uniaxial cellulose nanocrystal arrays |
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Quantum-efficiency enhancement and mechanical responsiveness of solid-state photoluminescent flexible materials containing uniaxial cellulose nanocrystal arrays |
| abstract |
Abstract Assembling cellulose nanocrystals (CNCs) can induce solid-state photoluminescence based on Stokes scattering. Such photoluminescent materials are free of photo-quenching and show great potential in optical applications, whereas poor flexibility of assembled CNC arrays limits their applications. Here, a binary co-assembly of 1D nanoparticles and long-chain polymers was explored to produce the uniaxial CNC arrays into transparent poly(vinyl alcohol) (PVA) membranes, which enhanced the mechanical properties, especially ductility. Besides, the CNC assembly was controlled by adjusting the mass ratio between CNCs and PVA. The result indicated that co-assembling with PVA could improve the uniaxial orientation of CNC arrays, which played a crucial role in enhancing the emission quantum efficiency (EQE). Stretching the PVA/CNC membrane could further induce an enhancement in EQE together with a blue shift in excitation wavelength. The mechanism study on stimulation-response suggested that the EQE enhancement and blue shift came from the change in uniaxial orientation degree and periodicity of the CNC assembly, respectively. Since the stimulation-responsive enhancement in EQE (from ca. 40 to 60%) can even be observed by naked eyes, we believe such cellulose-based materials can be widely used in optical sensors. © The Author(s), under exclusive licence to Springer Nature B.V. 2022 |
| abstractGer |
Abstract Assembling cellulose nanocrystals (CNCs) can induce solid-state photoluminescence based on Stokes scattering. Such photoluminescent materials are free of photo-quenching and show great potential in optical applications, whereas poor flexibility of assembled CNC arrays limits their applications. Here, a binary co-assembly of 1D nanoparticles and long-chain polymers was explored to produce the uniaxial CNC arrays into transparent poly(vinyl alcohol) (PVA) membranes, which enhanced the mechanical properties, especially ductility. Besides, the CNC assembly was controlled by adjusting the mass ratio between CNCs and PVA. The result indicated that co-assembling with PVA could improve the uniaxial orientation of CNC arrays, which played a crucial role in enhancing the emission quantum efficiency (EQE). Stretching the PVA/CNC membrane could further induce an enhancement in EQE together with a blue shift in excitation wavelength. The mechanism study on stimulation-response suggested that the EQE enhancement and blue shift came from the change in uniaxial orientation degree and periodicity of the CNC assembly, respectively. Since the stimulation-responsive enhancement in EQE (from ca. 40 to 60%) can even be observed by naked eyes, we believe such cellulose-based materials can be widely used in optical sensors. © The Author(s), under exclusive licence to Springer Nature B.V. 2022 |
| abstract_unstemmed |
Abstract Assembling cellulose nanocrystals (CNCs) can induce solid-state photoluminescence based on Stokes scattering. Such photoluminescent materials are free of photo-quenching and show great potential in optical applications, whereas poor flexibility of assembled CNC arrays limits their applications. Here, a binary co-assembly of 1D nanoparticles and long-chain polymers was explored to produce the uniaxial CNC arrays into transparent poly(vinyl alcohol) (PVA) membranes, which enhanced the mechanical properties, especially ductility. Besides, the CNC assembly was controlled by adjusting the mass ratio between CNCs and PVA. The result indicated that co-assembling with PVA could improve the uniaxial orientation of CNC arrays, which played a crucial role in enhancing the emission quantum efficiency (EQE). Stretching the PVA/CNC membrane could further induce an enhancement in EQE together with a blue shift in excitation wavelength. The mechanism study on stimulation-response suggested that the EQE enhancement and blue shift came from the change in uniaxial orientation degree and periodicity of the CNC assembly, respectively. Since the stimulation-responsive enhancement in EQE (from ca. 40 to 60%) can even be observed by naked eyes, we believe such cellulose-based materials can be widely used in optical sensors. © The Author(s), under exclusive licence to Springer Nature B.V. 2022 |
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Quantum-efficiency enhancement and mechanical responsiveness of solid-state photoluminescent flexible materials containing uniaxial cellulose nanocrystal arrays |
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https://dx.doi.org/10.1007/s10570-022-04424-w |
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Shi, Zhenxu Wang, Xuhong Gong, Yanbin Li, Xijun Jia, Xin Gan, Lin Huang, Jin |
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10.1007/s10570-022-04424-w |
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| score |
7.399809 |