$ Mn_{3} %$ O_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media
The development of cost-effective, abundant, and durable catalyst accelerating oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) is of important significance for commercialization of fuel cells and metal–oxygen batteries. In this work, the nanostructure of $ Mn_{3} %$ O_{4} $/Graph...
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Gespeichert in:
| Autor*in: |
Akbarian, Parisa [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2022 |
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| Anmerkung: |
© The Author(s), under exclusive licence to The Materials Research Society 2022 |
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| Übergeordnetes Werk: |
Enthalten in: Journal of materials research - Berlin : Springer, 1986, 37(2022), 4 vom: 14. Feb., Seite 887-896 |
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| Übergeordnetes Werk: |
volume:37 ; year:2022 ; number:4 ; day:14 ; month:02 ; pages:887-896 |
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| DOI / URN: |
10.1557/s43578-021-00436-7 |
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SPR046376534 |
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| 520 | |a The development of cost-effective, abundant, and durable catalyst accelerating oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) is of important significance for commercialization of fuel cells and metal–oxygen batteries. In this work, the nanostructure of $ Mn_{3} %$ O_{4} $/Graphene Quantum Dots (GQDs) was reported as a novel and high-performance ORR catalyst. The $ Mn_{3} %$ O_{4} $ nanoparticles were casted on GQDs via facile electrodeposition method. The performance of fabricated catalyst towards ORR is similar to Pt/C catalyst. The ORR onset potential for $ Mn_{3} %$ O_{4} $/GQDs-CP is − 0.1 V vs. (Hg/HgO), which is similar to that of the Pt/C-CP. The diffusion-limiting current density of the $ Mn_{3} %$ O_{4} $/GQDs-CP is approximately − 3.1 mA $ cm^{−2} $, which is higher than the $ Mn_{3} %$ O_{4} $/C-CP (− 2.5 mA $ cm^{−2} $) and GQDs/CP (− 2.01 mA $ cm^{−2} $). Moreover, the higher stability was obtained for $ Mn_{3} %$ O_{4} $/GQDs-CP in comparison to Pt/C-CP. The excellent catalytic activity of the $ Mn_{3} %$ O_{4} $/GQDs-CP electrode stemmed from the synergistic effect between $ Mn_{3} %$ O_{4} $ and the GQDs nanoparticles. Graphical abstract | ||
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10.1557/s43578-021-00436-7 doi (DE-627)SPR046376534 (SPR)s43578-021-00436-7-e DE-627 ger DE-627 rakwb eng Akbarian, Parisa verfasserin aut $ Mn_{3} %$ O_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to The Materials Research Society 2022 The development of cost-effective, abundant, and durable catalyst accelerating oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) is of important significance for commercialization of fuel cells and metal–oxygen batteries. In this work, the nanostructure of $ Mn_{3} %$ O_{4} $/Graphene Quantum Dots (GQDs) was reported as a novel and high-performance ORR catalyst. The $ Mn_{3} %$ O_{4} $ nanoparticles were casted on GQDs via facile electrodeposition method. The performance of fabricated catalyst towards ORR is similar to Pt/C catalyst. The ORR onset potential for $ Mn_{3} %$ O_{4} $/GQDs-CP is − 0.1 V vs. (Hg/HgO), which is similar to that of the Pt/C-CP. The diffusion-limiting current density of the $ Mn_{3} %$ O_{4} $/GQDs-CP is approximately − 3.1 mA $ cm^{−2} $, which is higher than the $ Mn_{3} %$ O_{4} $/C-CP (− 2.5 mA $ cm^{−2} $) and GQDs/CP (− 2.01 mA $ cm^{−2} $). Moreover, the higher stability was obtained for $ Mn_{3} %$ O_{4} $/GQDs-CP in comparison to Pt/C-CP. The excellent catalytic activity of the $ Mn_{3} %$ O_{4} $/GQDs-CP electrode stemmed from the synergistic effect between $ Mn_{3} %$ O_{4} $ and the GQDs nanoparticles. Graphical abstract Kheirmand, Mehdi aut Enthalten in Journal of materials research Berlin : Springer, 1986 37(2022), 4 vom: 14. Feb., Seite 887-896 (DE-627)320527026 (DE-600)2015297-8 2044-5326 nnns volume:37 year:2022 number:4 day:14 month:02 pages:887-896 https://dx.doi.org/10.1557/s43578-021-00436-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 37 2022 4 14 02 887-896 |
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10.1557/s43578-021-00436-7 doi (DE-627)SPR046376534 (SPR)s43578-021-00436-7-e DE-627 ger DE-627 rakwb eng Akbarian, Parisa verfasserin aut $ Mn_{3} %$ O_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to The Materials Research Society 2022 The development of cost-effective, abundant, and durable catalyst accelerating oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) is of important significance for commercialization of fuel cells and metal–oxygen batteries. In this work, the nanostructure of $ Mn_{3} %$ O_{4} $/Graphene Quantum Dots (GQDs) was reported as a novel and high-performance ORR catalyst. The $ Mn_{3} %$ O_{4} $ nanoparticles were casted on GQDs via facile electrodeposition method. The performance of fabricated catalyst towards ORR is similar to Pt/C catalyst. The ORR onset potential for $ Mn_{3} %$ O_{4} $/GQDs-CP is − 0.1 V vs. (Hg/HgO), which is similar to that of the Pt/C-CP. The diffusion-limiting current density of the $ Mn_{3} %$ O_{4} $/GQDs-CP is approximately − 3.1 mA $ cm^{−2} $, which is higher than the $ Mn_{3} %$ O_{4} $/C-CP (− 2.5 mA $ cm^{−2} $) and GQDs/CP (− 2.01 mA $ cm^{−2} $). Moreover, the higher stability was obtained for $ Mn_{3} %$ O_{4} $/GQDs-CP in comparison to Pt/C-CP. The excellent catalytic activity of the $ Mn_{3} %$ O_{4} $/GQDs-CP electrode stemmed from the synergistic effect between $ Mn_{3} %$ O_{4} $ and the GQDs nanoparticles. Graphical abstract Kheirmand, Mehdi aut Enthalten in Journal of materials research Berlin : Springer, 1986 37(2022), 4 vom: 14. Feb., Seite 887-896 (DE-627)320527026 (DE-600)2015297-8 2044-5326 nnns volume:37 year:2022 number:4 day:14 month:02 pages:887-896 https://dx.doi.org/10.1557/s43578-021-00436-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 37 2022 4 14 02 887-896 |
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10.1557/s43578-021-00436-7 doi (DE-627)SPR046376534 (SPR)s43578-021-00436-7-e DE-627 ger DE-627 rakwb eng Akbarian, Parisa verfasserin aut $ Mn_{3} %$ O_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to The Materials Research Society 2022 The development of cost-effective, abundant, and durable catalyst accelerating oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) is of important significance for commercialization of fuel cells and metal–oxygen batteries. In this work, the nanostructure of $ Mn_{3} %$ O_{4} $/Graphene Quantum Dots (GQDs) was reported as a novel and high-performance ORR catalyst. The $ Mn_{3} %$ O_{4} $ nanoparticles were casted on GQDs via facile electrodeposition method. The performance of fabricated catalyst towards ORR is similar to Pt/C catalyst. The ORR onset potential for $ Mn_{3} %$ O_{4} $/GQDs-CP is − 0.1 V vs. (Hg/HgO), which is similar to that of the Pt/C-CP. The diffusion-limiting current density of the $ Mn_{3} %$ O_{4} $/GQDs-CP is approximately − 3.1 mA $ cm^{−2} $, which is higher than the $ Mn_{3} %$ O_{4} $/C-CP (− 2.5 mA $ cm^{−2} $) and GQDs/CP (− 2.01 mA $ cm^{−2} $). Moreover, the higher stability was obtained for $ Mn_{3} %$ O_{4} $/GQDs-CP in comparison to Pt/C-CP. The excellent catalytic activity of the $ Mn_{3} %$ O_{4} $/GQDs-CP electrode stemmed from the synergistic effect between $ Mn_{3} %$ O_{4} $ and the GQDs nanoparticles. Graphical abstract Kheirmand, Mehdi aut Enthalten in Journal of materials research Berlin : Springer, 1986 37(2022), 4 vom: 14. Feb., Seite 887-896 (DE-627)320527026 (DE-600)2015297-8 2044-5326 nnns volume:37 year:2022 number:4 day:14 month:02 pages:887-896 https://dx.doi.org/10.1557/s43578-021-00436-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 37 2022 4 14 02 887-896 |
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10.1557/s43578-021-00436-7 doi (DE-627)SPR046376534 (SPR)s43578-021-00436-7-e DE-627 ger DE-627 rakwb eng Akbarian, Parisa verfasserin aut $ Mn_{3} %$ O_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to The Materials Research Society 2022 The development of cost-effective, abundant, and durable catalyst accelerating oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) is of important significance for commercialization of fuel cells and metal–oxygen batteries. In this work, the nanostructure of $ Mn_{3} %$ O_{4} $/Graphene Quantum Dots (GQDs) was reported as a novel and high-performance ORR catalyst. The $ Mn_{3} %$ O_{4} $ nanoparticles were casted on GQDs via facile electrodeposition method. The performance of fabricated catalyst towards ORR is similar to Pt/C catalyst. The ORR onset potential for $ Mn_{3} %$ O_{4} $/GQDs-CP is − 0.1 V vs. (Hg/HgO), which is similar to that of the Pt/C-CP. The diffusion-limiting current density of the $ Mn_{3} %$ O_{4} $/GQDs-CP is approximately − 3.1 mA $ cm^{−2} $, which is higher than the $ Mn_{3} %$ O_{4} $/C-CP (− 2.5 mA $ cm^{−2} $) and GQDs/CP (− 2.01 mA $ cm^{−2} $). Moreover, the higher stability was obtained for $ Mn_{3} %$ O_{4} $/GQDs-CP in comparison to Pt/C-CP. The excellent catalytic activity of the $ Mn_{3} %$ O_{4} $/GQDs-CP electrode stemmed from the synergistic effect between $ Mn_{3} %$ O_{4} $ and the GQDs nanoparticles. Graphical abstract Kheirmand, Mehdi aut Enthalten in Journal of materials research Berlin : Springer, 1986 37(2022), 4 vom: 14. Feb., Seite 887-896 (DE-627)320527026 (DE-600)2015297-8 2044-5326 nnns volume:37 year:2022 number:4 day:14 month:02 pages:887-896 https://dx.doi.org/10.1557/s43578-021-00436-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 37 2022 4 14 02 887-896 |
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10.1557/s43578-021-00436-7 doi (DE-627)SPR046376534 (SPR)s43578-021-00436-7-e DE-627 ger DE-627 rakwb eng Akbarian, Parisa verfasserin aut $ Mn_{3} %$ O_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to The Materials Research Society 2022 The development of cost-effective, abundant, and durable catalyst accelerating oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) is of important significance for commercialization of fuel cells and metal–oxygen batteries. In this work, the nanostructure of $ Mn_{3} %$ O_{4} $/Graphene Quantum Dots (GQDs) was reported as a novel and high-performance ORR catalyst. The $ Mn_{3} %$ O_{4} $ nanoparticles were casted on GQDs via facile electrodeposition method. The performance of fabricated catalyst towards ORR is similar to Pt/C catalyst. The ORR onset potential for $ Mn_{3} %$ O_{4} $/GQDs-CP is − 0.1 V vs. (Hg/HgO), which is similar to that of the Pt/C-CP. The diffusion-limiting current density of the $ Mn_{3} %$ O_{4} $/GQDs-CP is approximately − 3.1 mA $ cm^{−2} $, which is higher than the $ Mn_{3} %$ O_{4} $/C-CP (− 2.5 mA $ cm^{−2} $) and GQDs/CP (− 2.01 mA $ cm^{−2} $). Moreover, the higher stability was obtained for $ Mn_{3} %$ O_{4} $/GQDs-CP in comparison to Pt/C-CP. The excellent catalytic activity of the $ Mn_{3} %$ O_{4} $/GQDs-CP electrode stemmed from the synergistic effect between $ Mn_{3} %$ O_{4} $ and the GQDs nanoparticles. Graphical abstract Kheirmand, Mehdi aut Enthalten in Journal of materials research Berlin : Springer, 1986 37(2022), 4 vom: 14. Feb., Seite 887-896 (DE-627)320527026 (DE-600)2015297-8 2044-5326 nnns volume:37 year:2022 number:4 day:14 month:02 pages:887-896 https://dx.doi.org/10.1557/s43578-021-00436-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 37 2022 4 14 02 887-896 |
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In this work, the nanostructure of $ Mn_{3} %$ O_{4} $/Graphene Quantum Dots (GQDs) was reported as a novel and high-performance ORR catalyst. The $ Mn_{3} %$ O_{4} $ nanoparticles were casted on GQDs via facile electrodeposition method. The performance of fabricated catalyst towards ORR is similar to Pt/C catalyst. The ORR onset potential for $ Mn_{3} %$ O_{4} $/GQDs-CP is − 0.1 V vs. (Hg/HgO), which is similar to that of the Pt/C-CP. The diffusion-limiting current density of the $ Mn_{3} %$ O_{4} $/GQDs-CP is approximately − 3.1 mA $ cm^{−2} $, which is higher than the $ Mn_{3} %$ O_{4} $/C-CP (− 2.5 mA $ cm^{−2} $) and GQDs/CP (− 2.01 mA $ cm^{−2} $). Moreover, the higher stability was obtained for $ Mn_{3} %$ O_{4} $/GQDs-CP in comparison to Pt/C-CP. The excellent catalytic activity of the $ Mn_{3} %$ O_{4} $/GQDs-CP electrode stemmed from the synergistic effect between $ Mn_{3} %$ O_{4} $ and the GQDs nanoparticles. 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Akbarian, Parisa |
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Akbarian, Parisa $ Mn_{3} %$ O_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media |
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$ Mn_{3} %$ O_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media |
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$ Mn_{3} %$ O_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media |
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$ Mn_{3} %$ O_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media |
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10.1557/s43578-021-00436-7 |
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$ mn_{3} %$ o_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media |
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$ Mn_{3} %$ O_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media |
| abstract |
The development of cost-effective, abundant, and durable catalyst accelerating oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) is of important significance for commercialization of fuel cells and metal–oxygen batteries. In this work, the nanostructure of $ Mn_{3} %$ O_{4} $/Graphene Quantum Dots (GQDs) was reported as a novel and high-performance ORR catalyst. The $ Mn_{3} %$ O_{4} $ nanoparticles were casted on GQDs via facile electrodeposition method. The performance of fabricated catalyst towards ORR is similar to Pt/C catalyst. The ORR onset potential for $ Mn_{3} %$ O_{4} $/GQDs-CP is − 0.1 V vs. (Hg/HgO), which is similar to that of the Pt/C-CP. The diffusion-limiting current density of the $ Mn_{3} %$ O_{4} $/GQDs-CP is approximately − 3.1 mA $ cm^{−2} $, which is higher than the $ Mn_{3} %$ O_{4} $/C-CP (− 2.5 mA $ cm^{−2} $) and GQDs/CP (− 2.01 mA $ cm^{−2} $). Moreover, the higher stability was obtained for $ Mn_{3} %$ O_{4} $/GQDs-CP in comparison to Pt/C-CP. The excellent catalytic activity of the $ Mn_{3} %$ O_{4} $/GQDs-CP electrode stemmed from the synergistic effect between $ Mn_{3} %$ O_{4} $ and the GQDs nanoparticles. Graphical abstract © The Author(s), under exclusive licence to The Materials Research Society 2022 |
| abstractGer |
The development of cost-effective, abundant, and durable catalyst accelerating oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) is of important significance for commercialization of fuel cells and metal–oxygen batteries. In this work, the nanostructure of $ Mn_{3} %$ O_{4} $/Graphene Quantum Dots (GQDs) was reported as a novel and high-performance ORR catalyst. The $ Mn_{3} %$ O_{4} $ nanoparticles were casted on GQDs via facile electrodeposition method. The performance of fabricated catalyst towards ORR is similar to Pt/C catalyst. The ORR onset potential for $ Mn_{3} %$ O_{4} $/GQDs-CP is − 0.1 V vs. (Hg/HgO), which is similar to that of the Pt/C-CP. The diffusion-limiting current density of the $ Mn_{3} %$ O_{4} $/GQDs-CP is approximately − 3.1 mA $ cm^{−2} $, which is higher than the $ Mn_{3} %$ O_{4} $/C-CP (− 2.5 mA $ cm^{−2} $) and GQDs/CP (− 2.01 mA $ cm^{−2} $). Moreover, the higher stability was obtained for $ Mn_{3} %$ O_{4} $/GQDs-CP in comparison to Pt/C-CP. The excellent catalytic activity of the $ Mn_{3} %$ O_{4} $/GQDs-CP electrode stemmed from the synergistic effect between $ Mn_{3} %$ O_{4} $ and the GQDs nanoparticles. Graphical abstract © The Author(s), under exclusive licence to The Materials Research Society 2022 |
| abstract_unstemmed |
The development of cost-effective, abundant, and durable catalyst accelerating oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) is of important significance for commercialization of fuel cells and metal–oxygen batteries. In this work, the nanostructure of $ Mn_{3} %$ O_{4} $/Graphene Quantum Dots (GQDs) was reported as a novel and high-performance ORR catalyst. The $ Mn_{3} %$ O_{4} $ nanoparticles were casted on GQDs via facile electrodeposition method. The performance of fabricated catalyst towards ORR is similar to Pt/C catalyst. The ORR onset potential for $ Mn_{3} %$ O_{4} $/GQDs-CP is − 0.1 V vs. (Hg/HgO), which is similar to that of the Pt/C-CP. The diffusion-limiting current density of the $ Mn_{3} %$ O_{4} $/GQDs-CP is approximately − 3.1 mA $ cm^{−2} $, which is higher than the $ Mn_{3} %$ O_{4} $/C-CP (− 2.5 mA $ cm^{−2} $) and GQDs/CP (− 2.01 mA $ cm^{−2} $). Moreover, the higher stability was obtained for $ Mn_{3} %$ O_{4} $/GQDs-CP in comparison to Pt/C-CP. The excellent catalytic activity of the $ Mn_{3} %$ O_{4} $/GQDs-CP electrode stemmed from the synergistic effect between $ Mn_{3} %$ O_{4} $ and the GQDs nanoparticles. Graphical abstract © The Author(s), under exclusive licence to The Materials Research Society 2022 |
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$ Mn_{3} %$ O_{4} $/graphene quantum dots hybrid nanoparticles for enhanced oxygen reduction reaction in alkaline media |
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https://dx.doi.org/10.1557/s43578-021-00436-7 |
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Kheirmand, Mehdi |
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10.1557/s43578-021-00436-7 |
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