Geometric constraints of molecular self-assembly of normal alkanes on graphite
Abstract An abrupt increase of $ CH_{3} $-groups brightness as well as $ CH_{2} $-groups modulation along alkyl skeleton were observed in scanning tunneling microscopy (STM) images of n-alkanes monolayers on graphite. Analysis of STM-patterns demonstrates that both effects strongly depend on deforma...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Kutsenko, V. Ye. [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2021 |
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| Schlagwörter: |
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| Anmerkung: |
© King Abdulaziz City for Science and Technology 2021 |
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| Übergeordnetes Werk: |
Enthalten in: Applied nanoscience - Berlin : Springer, 2011, 12(2021), 3 vom: 16. Feb., Seite 385-393 |
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| Übergeordnetes Werk: |
volume:12 ; year:2021 ; number:3 ; day:16 ; month:02 ; pages:385-393 |
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| DOI / URN: |
10.1007/s13204-021-01713-x |
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SPR046433422 |
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| 520 | |a Abstract An abrupt increase of $ CH_{3} $-groups brightness as well as $ CH_{2} $-groups modulation along alkyl skeleton were observed in scanning tunneling microscopy (STM) images of n-alkanes monolayers on graphite. Analysis of STM-patterns demonstrates that both effects strongly depend on deformations of molecules and scanning conditions. We have observed that due to deformations, the monolayer is going to be compressed, thus methylene units protrude away from the surface forming a corrugated structure. Moreover, the distance between adjacent lamellae narrows, leading to the absence of furrows and, in particular, to a significant increasing of tunneling current from peripheral groups. The whole monolayer has been conserving its anomalous brightness for a few hours. Moreover, when the scanning conditions are changed, the monolayer could undergo an instantaneous reordering from the structure with increased brightness to the uniform one. | ||
| 650 | 4 | |a Normal alkanes |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Scanning tunneling microscopy |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Self-assembled monolayers |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Molecular interactions |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Geometric constrains |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Vasko, A. A. |4 aut | |
| 773 | 0 | 8 | |i Enthalten in |t Applied nanoscience |d Berlin : Springer, 2011 |g 12(2021), 3 vom: 16. Feb., Seite 385-393 |w (DE-627)658009001 |w (DE-600)2607723-1 |x 2190-5517 |7 nnns |
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10.1007/s13204-021-01713-x doi (DE-627)SPR046433422 (SPR)s13204-021-01713-x-e DE-627 ger DE-627 rakwb eng Kutsenko, V. Ye. verfasserin (orcid)0000-0003-0245-0817 aut Geometric constraints of molecular self-assembly of normal alkanes on graphite 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © King Abdulaziz City for Science and Technology 2021 Abstract An abrupt increase of $ CH_{3} $-groups brightness as well as $ CH_{2} $-groups modulation along alkyl skeleton were observed in scanning tunneling microscopy (STM) images of n-alkanes monolayers on graphite. Analysis of STM-patterns demonstrates that both effects strongly depend on deformations of molecules and scanning conditions. We have observed that due to deformations, the monolayer is going to be compressed, thus methylene units protrude away from the surface forming a corrugated structure. Moreover, the distance between adjacent lamellae narrows, leading to the absence of furrows and, in particular, to a significant increasing of tunneling current from peripheral groups. The whole monolayer has been conserving its anomalous brightness for a few hours. Moreover, when the scanning conditions are changed, the monolayer could undergo an instantaneous reordering from the structure with increased brightness to the uniform one. Normal alkanes (dpeaa)DE-He213 Scanning tunneling microscopy (dpeaa)DE-He213 Self-assembled monolayers (dpeaa)DE-He213 Molecular interactions (dpeaa)DE-He213 Geometric constrains (dpeaa)DE-He213 Vasko, A. A. aut Enthalten in Applied nanoscience Berlin : Springer, 2011 12(2021), 3 vom: 16. Feb., Seite 385-393 (DE-627)658009001 (DE-600)2607723-1 2190-5517 nnns volume:12 year:2021 number:3 day:16 month:02 pages:385-393 https://dx.doi.org/10.1007/s13204-021-01713-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_266 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 12 2021 3 16 02 385-393 |
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10.1007/s13204-021-01713-x doi (DE-627)SPR046433422 (SPR)s13204-021-01713-x-e DE-627 ger DE-627 rakwb eng Kutsenko, V. Ye. verfasserin (orcid)0000-0003-0245-0817 aut Geometric constraints of molecular self-assembly of normal alkanes on graphite 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © King Abdulaziz City for Science and Technology 2021 Abstract An abrupt increase of $ CH_{3} $-groups brightness as well as $ CH_{2} $-groups modulation along alkyl skeleton were observed in scanning tunneling microscopy (STM) images of n-alkanes monolayers on graphite. Analysis of STM-patterns demonstrates that both effects strongly depend on deformations of molecules and scanning conditions. We have observed that due to deformations, the monolayer is going to be compressed, thus methylene units protrude away from the surface forming a corrugated structure. Moreover, the distance between adjacent lamellae narrows, leading to the absence of furrows and, in particular, to a significant increasing of tunneling current from peripheral groups. The whole monolayer has been conserving its anomalous brightness for a few hours. Moreover, when the scanning conditions are changed, the monolayer could undergo an instantaneous reordering from the structure with increased brightness to the uniform one. Normal alkanes (dpeaa)DE-He213 Scanning tunneling microscopy (dpeaa)DE-He213 Self-assembled monolayers (dpeaa)DE-He213 Molecular interactions (dpeaa)DE-He213 Geometric constrains (dpeaa)DE-He213 Vasko, A. A. aut Enthalten in Applied nanoscience Berlin : Springer, 2011 12(2021), 3 vom: 16. Feb., Seite 385-393 (DE-627)658009001 (DE-600)2607723-1 2190-5517 nnns volume:12 year:2021 number:3 day:16 month:02 pages:385-393 https://dx.doi.org/10.1007/s13204-021-01713-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_266 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 12 2021 3 16 02 385-393 |
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10.1007/s13204-021-01713-x doi (DE-627)SPR046433422 (SPR)s13204-021-01713-x-e DE-627 ger DE-627 rakwb eng Kutsenko, V. Ye. verfasserin (orcid)0000-0003-0245-0817 aut Geometric constraints of molecular self-assembly of normal alkanes on graphite 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © King Abdulaziz City for Science and Technology 2021 Abstract An abrupt increase of $ CH_{3} $-groups brightness as well as $ CH_{2} $-groups modulation along alkyl skeleton were observed in scanning tunneling microscopy (STM) images of n-alkanes monolayers on graphite. Analysis of STM-patterns demonstrates that both effects strongly depend on deformations of molecules and scanning conditions. We have observed that due to deformations, the monolayer is going to be compressed, thus methylene units protrude away from the surface forming a corrugated structure. Moreover, the distance between adjacent lamellae narrows, leading to the absence of furrows and, in particular, to a significant increasing of tunneling current from peripheral groups. The whole monolayer has been conserving its anomalous brightness for a few hours. Moreover, when the scanning conditions are changed, the monolayer could undergo an instantaneous reordering from the structure with increased brightness to the uniform one. Normal alkanes (dpeaa)DE-He213 Scanning tunneling microscopy (dpeaa)DE-He213 Self-assembled monolayers (dpeaa)DE-He213 Molecular interactions (dpeaa)DE-He213 Geometric constrains (dpeaa)DE-He213 Vasko, A. A. aut Enthalten in Applied nanoscience Berlin : Springer, 2011 12(2021), 3 vom: 16. Feb., Seite 385-393 (DE-627)658009001 (DE-600)2607723-1 2190-5517 nnns volume:12 year:2021 number:3 day:16 month:02 pages:385-393 https://dx.doi.org/10.1007/s13204-021-01713-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_266 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 12 2021 3 16 02 385-393 |
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10.1007/s13204-021-01713-x doi (DE-627)SPR046433422 (SPR)s13204-021-01713-x-e DE-627 ger DE-627 rakwb eng Kutsenko, V. Ye. verfasserin (orcid)0000-0003-0245-0817 aut Geometric constraints of molecular self-assembly of normal alkanes on graphite 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © King Abdulaziz City for Science and Technology 2021 Abstract An abrupt increase of $ CH_{3} $-groups brightness as well as $ CH_{2} $-groups modulation along alkyl skeleton were observed in scanning tunneling microscopy (STM) images of n-alkanes monolayers on graphite. Analysis of STM-patterns demonstrates that both effects strongly depend on deformations of molecules and scanning conditions. We have observed that due to deformations, the monolayer is going to be compressed, thus methylene units protrude away from the surface forming a corrugated structure. Moreover, the distance between adjacent lamellae narrows, leading to the absence of furrows and, in particular, to a significant increasing of tunneling current from peripheral groups. The whole monolayer has been conserving its anomalous brightness for a few hours. Moreover, when the scanning conditions are changed, the monolayer could undergo an instantaneous reordering from the structure with increased brightness to the uniform one. Normal alkanes (dpeaa)DE-He213 Scanning tunneling microscopy (dpeaa)DE-He213 Self-assembled monolayers (dpeaa)DE-He213 Molecular interactions (dpeaa)DE-He213 Geometric constrains (dpeaa)DE-He213 Vasko, A. A. aut Enthalten in Applied nanoscience Berlin : Springer, 2011 12(2021), 3 vom: 16. Feb., Seite 385-393 (DE-627)658009001 (DE-600)2607723-1 2190-5517 nnns volume:12 year:2021 number:3 day:16 month:02 pages:385-393 https://dx.doi.org/10.1007/s13204-021-01713-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_266 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 12 2021 3 16 02 385-393 |
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Kutsenko, V. Ye. |
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Kutsenko, V. Ye. misc Normal alkanes misc Scanning tunneling microscopy misc Self-assembled monolayers misc Molecular interactions misc Geometric constrains Geometric constraints of molecular self-assembly of normal alkanes on graphite |
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Geometric constraints of molecular self-assembly of normal alkanes on graphite Normal alkanes (dpeaa)DE-He213 Scanning tunneling microscopy (dpeaa)DE-He213 Self-assembled monolayers (dpeaa)DE-He213 Molecular interactions (dpeaa)DE-He213 Geometric constrains (dpeaa)DE-He213 |
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geometric constraints of molecular self-assembly of normal alkanes on graphite |
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Geometric constraints of molecular self-assembly of normal alkanes on graphite |
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Abstract An abrupt increase of $ CH_{3} $-groups brightness as well as $ CH_{2} $-groups modulation along alkyl skeleton were observed in scanning tunneling microscopy (STM) images of n-alkanes monolayers on graphite. Analysis of STM-patterns demonstrates that both effects strongly depend on deformations of molecules and scanning conditions. We have observed that due to deformations, the monolayer is going to be compressed, thus methylene units protrude away from the surface forming a corrugated structure. Moreover, the distance between adjacent lamellae narrows, leading to the absence of furrows and, in particular, to a significant increasing of tunneling current from peripheral groups. The whole monolayer has been conserving its anomalous brightness for a few hours. Moreover, when the scanning conditions are changed, the monolayer could undergo an instantaneous reordering from the structure with increased brightness to the uniform one. © King Abdulaziz City for Science and Technology 2021 |
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Abstract An abrupt increase of $ CH_{3} $-groups brightness as well as $ CH_{2} $-groups modulation along alkyl skeleton were observed in scanning tunneling microscopy (STM) images of n-alkanes monolayers on graphite. Analysis of STM-patterns demonstrates that both effects strongly depend on deformations of molecules and scanning conditions. We have observed that due to deformations, the monolayer is going to be compressed, thus methylene units protrude away from the surface forming a corrugated structure. Moreover, the distance between adjacent lamellae narrows, leading to the absence of furrows and, in particular, to a significant increasing of tunneling current from peripheral groups. The whole monolayer has been conserving its anomalous brightness for a few hours. Moreover, when the scanning conditions are changed, the monolayer could undergo an instantaneous reordering from the structure with increased brightness to the uniform one. © King Abdulaziz City for Science and Technology 2021 |
| abstract_unstemmed |
Abstract An abrupt increase of $ CH_{3} $-groups brightness as well as $ CH_{2} $-groups modulation along alkyl skeleton were observed in scanning tunneling microscopy (STM) images of n-alkanes monolayers on graphite. Analysis of STM-patterns demonstrates that both effects strongly depend on deformations of molecules and scanning conditions. We have observed that due to deformations, the monolayer is going to be compressed, thus methylene units protrude away from the surface forming a corrugated structure. Moreover, the distance between adjacent lamellae narrows, leading to the absence of furrows and, in particular, to a significant increasing of tunneling current from peripheral groups. The whole monolayer has been conserving its anomalous brightness for a few hours. Moreover, when the scanning conditions are changed, the monolayer could undergo an instantaneous reordering from the structure with increased brightness to the uniform one. © King Abdulaziz City for Science and Technology 2021 |
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<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000caa a22002652 4500</leader><controlfield tag="001">SPR046433422</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230507125432.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">220310s2021 xx |||||o 00| ||eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1007/s13204-021-01713-x</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)SPR046433422</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(SPR)s13204-021-01713-x-e</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Kutsenko, V. Ye.</subfield><subfield code="e">verfasserin</subfield><subfield code="0">(orcid)0000-0003-0245-0817</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Geometric constraints of molecular self-assembly of normal alkanes on graphite</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2021</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="500" ind1=" " ind2=" "><subfield code="a">© King Abdulaziz City for Science and Technology 2021</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Abstract An abrupt increase of $ CH_{3} $-groups brightness as well as $ CH_{2} $-groups modulation along alkyl skeleton were observed in scanning tunneling microscopy (STM) images of n-alkanes monolayers on graphite. Analysis of STM-patterns demonstrates that both effects strongly depend on deformations of molecules and scanning conditions. We have observed that due to deformations, the monolayer is going to be compressed, thus methylene units protrude away from the surface forming a corrugated structure. Moreover, the distance between adjacent lamellae narrows, leading to the absence of furrows and, in particular, to a significant increasing of tunneling current from peripheral groups. The whole monolayer has been conserving its anomalous brightness for a few hours. 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