Laboratory Studies of Removal and Degradation of Galaxolide (HHCB) and Tonalide (AHTN) in Water by Ferrate(VI)
Abstract Synthetic musks (SMs), as a group of pharmaceutical and personal care products (PPCPs), have been widely detected in the environment at ng $ L^{−1} $ ~ μg $ L^{−1} $ levels and require our serious attention regarding their presence, toxicity and treatment technologies. In this study, ferrat...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Xu, Ying [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2022 |
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| Schlagwörter: |
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| Anmerkung: |
© The Author(s), under exclusive licence to Springer Nature Switzerland AG 2022 |
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| Übergeordnetes Werk: |
Enthalten in: Water, air & soil pollution - Dordrecht [u.a.] : Springer Science + Business Media B.V, 1971, 233(2022), 6 vom: Juni |
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| Übergeordnetes Werk: |
volume:233 ; year:2022 ; number:6 ; month:06 |
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| DOI / URN: |
10.1007/s11270-022-05686-7 |
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| Katalog-ID: |
SPR047213620 |
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| 520 | |a Abstract Synthetic musks (SMs), as a group of pharmaceutical and personal care products (PPCPs), have been widely detected in the environment at ng $ L^{−1} $ ~ μg $ L^{−1} $ levels and require our serious attention regarding their presence, toxicity and treatment technologies. In this study, ferrate ($ Fe_{2} %$ O_{4} $2−, Fe(VI)) was employed to treat two typical SMs, galaxolide (HHCB) and tonalide (AHTN), in water solutions. The treatment efficiencies of trace level HHCB and AHTN compounds (16 μg $ L^{−1} $ each) in individual and mixed solutions by Fe(VI) (0–45 mg $ L^{−1} $ as Fe) at pH 5.5–8.5 were assessed, and oxidation products of both compounds were also investigated by means of solid phase extraction coupled with gas chromatography-mass spectrometry (SPE-GC–MS). Results demonstrated that Fe(VI) was more suitable to remove HHCB than AHTN from test solutions. Specifically, when solution pH was 6.5 and Fe(VI) dose was 15–18 mg $ L^{−1} $ as Fe, the removal efficiencies of HHCB and AHTN in individual test solutions were up to 60% and 40%, respectively. Comparatively, much higher Fe(VI) doses were required (up to 38 mg $ L^{−1} $ as Fe) in order to achieve considerable removal efficiencies of both compounds in mixed test solutions. Solution pH played an important role and neutral conditions would benefit the removal of both compounds. In addition, several oxidation products (OPs) of both HHCB and AHTN were identified, and degradation pathways were then tentatively proposed. Finally, engineering aspects of Fe(VI) technology in full-scale water treatment applications were also discussed. | ||
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| 650 | 4 | |a Synthetic musks |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Galaxolide (HHCB) |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Tonalide (AHTN) |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Oxidation products |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Degradation pathways |7 (dpeaa)DE-He213 | |
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| 700 | 1 | |a Xue, Yingang |4 aut | |
| 700 | 1 | |a Wu, Jun |4 aut | |
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10.1007/s11270-022-05686-7 doi (DE-627)SPR047213620 (SPR)s11270-022-05686-7-e DE-627 ger DE-627 rakwb eng Xu, Ying verfasserin aut Laboratory Studies of Removal and Degradation of Galaxolide (HHCB) and Tonalide (AHTN) in Water by Ferrate(VI) 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature Switzerland AG 2022 Abstract Synthetic musks (SMs), as a group of pharmaceutical and personal care products (PPCPs), have been widely detected in the environment at ng $ L^{−1} $ ~ μg $ L^{−1} $ levels and require our serious attention regarding their presence, toxicity and treatment technologies. In this study, ferrate ($ Fe_{2} %$ O_{4} $2−, Fe(VI)) was employed to treat two typical SMs, galaxolide (HHCB) and tonalide (AHTN), in water solutions. The treatment efficiencies of trace level HHCB and AHTN compounds (16 μg $ L^{−1} $ each) in individual and mixed solutions by Fe(VI) (0–45 mg $ L^{−1} $ as Fe) at pH 5.5–8.5 were assessed, and oxidation products of both compounds were also investigated by means of solid phase extraction coupled with gas chromatography-mass spectrometry (SPE-GC–MS). Results demonstrated that Fe(VI) was more suitable to remove HHCB than AHTN from test solutions. Specifically, when solution pH was 6.5 and Fe(VI) dose was 15–18 mg $ L^{−1} $ as Fe, the removal efficiencies of HHCB and AHTN in individual test solutions were up to 60% and 40%, respectively. Comparatively, much higher Fe(VI) doses were required (up to 38 mg $ L^{−1} $ as Fe) in order to achieve considerable removal efficiencies of both compounds in mixed test solutions. Solution pH played an important role and neutral conditions would benefit the removal of both compounds. In addition, several oxidation products (OPs) of both HHCB and AHTN were identified, and degradation pathways were then tentatively proposed. Finally, engineering aspects of Fe(VI) technology in full-scale water treatment applications were also discussed. Ferrate(VI) (dpeaa)DE-He213 Synthetic musks (dpeaa)DE-He213 Galaxolide (HHCB) (dpeaa)DE-He213 Tonalide (AHTN) (dpeaa)DE-He213 Oxidation products (dpeaa)DE-He213 Degradation pathways (dpeaa)DE-He213 Zhou, Zhengwei (orcid)0000-0001-9014-5139 aut Xue, Yingang aut Wu, Jun aut Enthalten in Water, air & soil pollution Dordrecht [u.a.] : Springer Science + Business Media B.V, 1971 233(2022), 6 vom: Juni (DE-627)271349417 (DE-600)1479824-4 1573-2932 nnns volume:233 year:2022 number:6 month:06 https://dx.doi.org/10.1007/s11270-022-05686-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 233 2022 6 06 |
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10.1007/s11270-022-05686-7 doi (DE-627)SPR047213620 (SPR)s11270-022-05686-7-e DE-627 ger DE-627 rakwb eng Xu, Ying verfasserin aut Laboratory Studies of Removal and Degradation of Galaxolide (HHCB) and Tonalide (AHTN) in Water by Ferrate(VI) 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature Switzerland AG 2022 Abstract Synthetic musks (SMs), as a group of pharmaceutical and personal care products (PPCPs), have been widely detected in the environment at ng $ L^{−1} $ ~ μg $ L^{−1} $ levels and require our serious attention regarding their presence, toxicity and treatment technologies. In this study, ferrate ($ Fe_{2} %$ O_{4} $2−, Fe(VI)) was employed to treat two typical SMs, galaxolide (HHCB) and tonalide (AHTN), in water solutions. The treatment efficiencies of trace level HHCB and AHTN compounds (16 μg $ L^{−1} $ each) in individual and mixed solutions by Fe(VI) (0–45 mg $ L^{−1} $ as Fe) at pH 5.5–8.5 were assessed, and oxidation products of both compounds were also investigated by means of solid phase extraction coupled with gas chromatography-mass spectrometry (SPE-GC–MS). Results demonstrated that Fe(VI) was more suitable to remove HHCB than AHTN from test solutions. Specifically, when solution pH was 6.5 and Fe(VI) dose was 15–18 mg $ L^{−1} $ as Fe, the removal efficiencies of HHCB and AHTN in individual test solutions were up to 60% and 40%, respectively. Comparatively, much higher Fe(VI) doses were required (up to 38 mg $ L^{−1} $ as Fe) in order to achieve considerable removal efficiencies of both compounds in mixed test solutions. Solution pH played an important role and neutral conditions would benefit the removal of both compounds. In addition, several oxidation products (OPs) of both HHCB and AHTN were identified, and degradation pathways were then tentatively proposed. Finally, engineering aspects of Fe(VI) technology in full-scale water treatment applications were also discussed. Ferrate(VI) (dpeaa)DE-He213 Synthetic musks (dpeaa)DE-He213 Galaxolide (HHCB) (dpeaa)DE-He213 Tonalide (AHTN) (dpeaa)DE-He213 Oxidation products (dpeaa)DE-He213 Degradation pathways (dpeaa)DE-He213 Zhou, Zhengwei (orcid)0000-0001-9014-5139 aut Xue, Yingang aut Wu, Jun aut Enthalten in Water, air & soil pollution Dordrecht [u.a.] : Springer Science + Business Media B.V, 1971 233(2022), 6 vom: Juni (DE-627)271349417 (DE-600)1479824-4 1573-2932 nnns volume:233 year:2022 number:6 month:06 https://dx.doi.org/10.1007/s11270-022-05686-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 233 2022 6 06 |
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10.1007/s11270-022-05686-7 doi (DE-627)SPR047213620 (SPR)s11270-022-05686-7-e DE-627 ger DE-627 rakwb eng Xu, Ying verfasserin aut Laboratory Studies of Removal and Degradation of Galaxolide (HHCB) and Tonalide (AHTN) in Water by Ferrate(VI) 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature Switzerland AG 2022 Abstract Synthetic musks (SMs), as a group of pharmaceutical and personal care products (PPCPs), have been widely detected in the environment at ng $ L^{−1} $ ~ μg $ L^{−1} $ levels and require our serious attention regarding their presence, toxicity and treatment technologies. In this study, ferrate ($ Fe_{2} %$ O_{4} $2−, Fe(VI)) was employed to treat two typical SMs, galaxolide (HHCB) and tonalide (AHTN), in water solutions. The treatment efficiencies of trace level HHCB and AHTN compounds (16 μg $ L^{−1} $ each) in individual and mixed solutions by Fe(VI) (0–45 mg $ L^{−1} $ as Fe) at pH 5.5–8.5 were assessed, and oxidation products of both compounds were also investigated by means of solid phase extraction coupled with gas chromatography-mass spectrometry (SPE-GC–MS). Results demonstrated that Fe(VI) was more suitable to remove HHCB than AHTN from test solutions. Specifically, when solution pH was 6.5 and Fe(VI) dose was 15–18 mg $ L^{−1} $ as Fe, the removal efficiencies of HHCB and AHTN in individual test solutions were up to 60% and 40%, respectively. Comparatively, much higher Fe(VI) doses were required (up to 38 mg $ L^{−1} $ as Fe) in order to achieve considerable removal efficiencies of both compounds in mixed test solutions. Solution pH played an important role and neutral conditions would benefit the removal of both compounds. In addition, several oxidation products (OPs) of both HHCB and AHTN were identified, and degradation pathways were then tentatively proposed. Finally, engineering aspects of Fe(VI) technology in full-scale water treatment applications were also discussed. Ferrate(VI) (dpeaa)DE-He213 Synthetic musks (dpeaa)DE-He213 Galaxolide (HHCB) (dpeaa)DE-He213 Tonalide (AHTN) (dpeaa)DE-He213 Oxidation products (dpeaa)DE-He213 Degradation pathways (dpeaa)DE-He213 Zhou, Zhengwei (orcid)0000-0001-9014-5139 aut Xue, Yingang aut Wu, Jun aut Enthalten in Water, air & soil pollution Dordrecht [u.a.] : Springer Science + Business Media B.V, 1971 233(2022), 6 vom: Juni (DE-627)271349417 (DE-600)1479824-4 1573-2932 nnns volume:233 year:2022 number:6 month:06 https://dx.doi.org/10.1007/s11270-022-05686-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 233 2022 6 06 |
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10.1007/s11270-022-05686-7 doi (DE-627)SPR047213620 (SPR)s11270-022-05686-7-e DE-627 ger DE-627 rakwb eng Xu, Ying verfasserin aut Laboratory Studies of Removal and Degradation of Galaxolide (HHCB) and Tonalide (AHTN) in Water by Ferrate(VI) 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature Switzerland AG 2022 Abstract Synthetic musks (SMs), as a group of pharmaceutical and personal care products (PPCPs), have been widely detected in the environment at ng $ L^{−1} $ ~ μg $ L^{−1} $ levels and require our serious attention regarding their presence, toxicity and treatment technologies. In this study, ferrate ($ Fe_{2} %$ O_{4} $2−, Fe(VI)) was employed to treat two typical SMs, galaxolide (HHCB) and tonalide (AHTN), in water solutions. The treatment efficiencies of trace level HHCB and AHTN compounds (16 μg $ L^{−1} $ each) in individual and mixed solutions by Fe(VI) (0–45 mg $ L^{−1} $ as Fe) at pH 5.5–8.5 were assessed, and oxidation products of both compounds were also investigated by means of solid phase extraction coupled with gas chromatography-mass spectrometry (SPE-GC–MS). Results demonstrated that Fe(VI) was more suitable to remove HHCB than AHTN from test solutions. Specifically, when solution pH was 6.5 and Fe(VI) dose was 15–18 mg $ L^{−1} $ as Fe, the removal efficiencies of HHCB and AHTN in individual test solutions were up to 60% and 40%, respectively. Comparatively, much higher Fe(VI) doses were required (up to 38 mg $ L^{−1} $ as Fe) in order to achieve considerable removal efficiencies of both compounds in mixed test solutions. Solution pH played an important role and neutral conditions would benefit the removal of both compounds. In addition, several oxidation products (OPs) of both HHCB and AHTN were identified, and degradation pathways were then tentatively proposed. Finally, engineering aspects of Fe(VI) technology in full-scale water treatment applications were also discussed. Ferrate(VI) (dpeaa)DE-He213 Synthetic musks (dpeaa)DE-He213 Galaxolide (HHCB) (dpeaa)DE-He213 Tonalide (AHTN) (dpeaa)DE-He213 Oxidation products (dpeaa)DE-He213 Degradation pathways (dpeaa)DE-He213 Zhou, Zhengwei (orcid)0000-0001-9014-5139 aut Xue, Yingang aut Wu, Jun aut Enthalten in Water, air & soil pollution Dordrecht [u.a.] : Springer Science + Business Media B.V, 1971 233(2022), 6 vom: Juni (DE-627)271349417 (DE-600)1479824-4 1573-2932 nnns volume:233 year:2022 number:6 month:06 https://dx.doi.org/10.1007/s11270-022-05686-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 233 2022 6 06 |
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10.1007/s11270-022-05686-7 doi (DE-627)SPR047213620 (SPR)s11270-022-05686-7-e DE-627 ger DE-627 rakwb eng Xu, Ying verfasserin aut Laboratory Studies of Removal and Degradation of Galaxolide (HHCB) and Tonalide (AHTN) in Water by Ferrate(VI) 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature Switzerland AG 2022 Abstract Synthetic musks (SMs), as a group of pharmaceutical and personal care products (PPCPs), have been widely detected in the environment at ng $ L^{−1} $ ~ μg $ L^{−1} $ levels and require our serious attention regarding their presence, toxicity and treatment technologies. In this study, ferrate ($ Fe_{2} %$ O_{4} $2−, Fe(VI)) was employed to treat two typical SMs, galaxolide (HHCB) and tonalide (AHTN), in water solutions. The treatment efficiencies of trace level HHCB and AHTN compounds (16 μg $ L^{−1} $ each) in individual and mixed solutions by Fe(VI) (0–45 mg $ L^{−1} $ as Fe) at pH 5.5–8.5 were assessed, and oxidation products of both compounds were also investigated by means of solid phase extraction coupled with gas chromatography-mass spectrometry (SPE-GC–MS). Results demonstrated that Fe(VI) was more suitable to remove HHCB than AHTN from test solutions. Specifically, when solution pH was 6.5 and Fe(VI) dose was 15–18 mg $ L^{−1} $ as Fe, the removal efficiencies of HHCB and AHTN in individual test solutions were up to 60% and 40%, respectively. Comparatively, much higher Fe(VI) doses were required (up to 38 mg $ L^{−1} $ as Fe) in order to achieve considerable removal efficiencies of both compounds in mixed test solutions. Solution pH played an important role and neutral conditions would benefit the removal of both compounds. In addition, several oxidation products (OPs) of both HHCB and AHTN were identified, and degradation pathways were then tentatively proposed. Finally, engineering aspects of Fe(VI) technology in full-scale water treatment applications were also discussed. Ferrate(VI) (dpeaa)DE-He213 Synthetic musks (dpeaa)DE-He213 Galaxolide (HHCB) (dpeaa)DE-He213 Tonalide (AHTN) (dpeaa)DE-He213 Oxidation products (dpeaa)DE-He213 Degradation pathways (dpeaa)DE-He213 Zhou, Zhengwei (orcid)0000-0001-9014-5139 aut Xue, Yingang aut Wu, Jun aut Enthalten in Water, air & soil pollution Dordrecht [u.a.] : Springer Science + Business Media B.V, 1971 233(2022), 6 vom: Juni (DE-627)271349417 (DE-600)1479824-4 1573-2932 nnns volume:233 year:2022 number:6 month:06 https://dx.doi.org/10.1007/s11270-022-05686-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 233 2022 6 06 |
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Enthalten in Water, air & soil pollution 233(2022), 6 vom: Juni volume:233 year:2022 number:6 month:06 |
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Ferrate(VI) Synthetic musks Galaxolide (HHCB) Tonalide (AHTN) Oxidation products Degradation pathways |
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Xu, Ying @@aut@@ Zhou, Zhengwei @@aut@@ Xue, Yingang @@aut@@ Wu, Jun @@aut@@ |
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In this study, ferrate ($ Fe_{2} %$ O_{4} $2−, Fe(VI)) was employed to treat two typical SMs, galaxolide (HHCB) and tonalide (AHTN), in water solutions. The treatment efficiencies of trace level HHCB and AHTN compounds (16 μg $ L^{−1} $ each) in individual and mixed solutions by Fe(VI) (0–45 mg $ L^{−1} $ as Fe) at pH 5.5–8.5 were assessed, and oxidation products of both compounds were also investigated by means of solid phase extraction coupled with gas chromatography-mass spectrometry (SPE-GC–MS). Results demonstrated that Fe(VI) was more suitable to remove HHCB than AHTN from test solutions. Specifically, when solution pH was 6.5 and Fe(VI) dose was 15–18 mg $ L^{−1} $ as Fe, the removal efficiencies of HHCB and AHTN in individual test solutions were up to 60% and 40%, respectively. Comparatively, much higher Fe(VI) doses were required (up to 38 mg $ L^{−1} $ as Fe) in order to achieve considerable removal efficiencies of both compounds in mixed test solutions. Solution pH played an important role and neutral conditions would benefit the removal of both compounds. In addition, several oxidation products (OPs) of both HHCB and AHTN were identified, and degradation pathways were then tentatively proposed. 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|
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Xu, Ying |
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Xu, Ying misc Ferrate(VI) misc Synthetic musks misc Galaxolide (HHCB) misc Tonalide (AHTN) misc Oxidation products misc Degradation pathways Laboratory Studies of Removal and Degradation of Galaxolide (HHCB) and Tonalide (AHTN) in Water by Ferrate(VI) |
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Laboratory Studies of Removal and Degradation of Galaxolide (HHCB) and Tonalide (AHTN) in Water by Ferrate(VI) Ferrate(VI) (dpeaa)DE-He213 Synthetic musks (dpeaa)DE-He213 Galaxolide (HHCB) (dpeaa)DE-He213 Tonalide (AHTN) (dpeaa)DE-He213 Oxidation products (dpeaa)DE-He213 Degradation pathways (dpeaa)DE-He213 |
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misc Ferrate(VI) misc Synthetic musks misc Galaxolide (HHCB) misc Tonalide (AHTN) misc Oxidation products misc Degradation pathways |
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misc Ferrate(VI) misc Synthetic musks misc Galaxolide (HHCB) misc Tonalide (AHTN) misc Oxidation products misc Degradation pathways |
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Laboratory Studies of Removal and Degradation of Galaxolide (HHCB) and Tonalide (AHTN) in Water by Ferrate(VI) |
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Laboratory Studies of Removal and Degradation of Galaxolide (HHCB) and Tonalide (AHTN) in Water by Ferrate(VI) |
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Xu, Ying |
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Xu, Ying Zhou, Zhengwei Xue, Yingang Wu, Jun |
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Xu, Ying |
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laboratory studies of removal and degradation of galaxolide (hhcb) and tonalide (ahtn) in water by ferrate(vi) |
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Laboratory Studies of Removal and Degradation of Galaxolide (HHCB) and Tonalide (AHTN) in Water by Ferrate(VI) |
| abstract |
Abstract Synthetic musks (SMs), as a group of pharmaceutical and personal care products (PPCPs), have been widely detected in the environment at ng $ L^{−1} $ ~ μg $ L^{−1} $ levels and require our serious attention regarding their presence, toxicity and treatment technologies. In this study, ferrate ($ Fe_{2} %$ O_{4} $2−, Fe(VI)) was employed to treat two typical SMs, galaxolide (HHCB) and tonalide (AHTN), in water solutions. The treatment efficiencies of trace level HHCB and AHTN compounds (16 μg $ L^{−1} $ each) in individual and mixed solutions by Fe(VI) (0–45 mg $ L^{−1} $ as Fe) at pH 5.5–8.5 were assessed, and oxidation products of both compounds were also investigated by means of solid phase extraction coupled with gas chromatography-mass spectrometry (SPE-GC–MS). Results demonstrated that Fe(VI) was more suitable to remove HHCB than AHTN from test solutions. Specifically, when solution pH was 6.5 and Fe(VI) dose was 15–18 mg $ L^{−1} $ as Fe, the removal efficiencies of HHCB and AHTN in individual test solutions were up to 60% and 40%, respectively. Comparatively, much higher Fe(VI) doses were required (up to 38 mg $ L^{−1} $ as Fe) in order to achieve considerable removal efficiencies of both compounds in mixed test solutions. Solution pH played an important role and neutral conditions would benefit the removal of both compounds. In addition, several oxidation products (OPs) of both HHCB and AHTN were identified, and degradation pathways were then tentatively proposed. Finally, engineering aspects of Fe(VI) technology in full-scale water treatment applications were also discussed. © The Author(s), under exclusive licence to Springer Nature Switzerland AG 2022 |
| abstractGer |
Abstract Synthetic musks (SMs), as a group of pharmaceutical and personal care products (PPCPs), have been widely detected in the environment at ng $ L^{−1} $ ~ μg $ L^{−1} $ levels and require our serious attention regarding their presence, toxicity and treatment technologies. In this study, ferrate ($ Fe_{2} %$ O_{4} $2−, Fe(VI)) was employed to treat two typical SMs, galaxolide (HHCB) and tonalide (AHTN), in water solutions. The treatment efficiencies of trace level HHCB and AHTN compounds (16 μg $ L^{−1} $ each) in individual and mixed solutions by Fe(VI) (0–45 mg $ L^{−1} $ as Fe) at pH 5.5–8.5 were assessed, and oxidation products of both compounds were also investigated by means of solid phase extraction coupled with gas chromatography-mass spectrometry (SPE-GC–MS). Results demonstrated that Fe(VI) was more suitable to remove HHCB than AHTN from test solutions. Specifically, when solution pH was 6.5 and Fe(VI) dose was 15–18 mg $ L^{−1} $ as Fe, the removal efficiencies of HHCB and AHTN in individual test solutions were up to 60% and 40%, respectively. Comparatively, much higher Fe(VI) doses were required (up to 38 mg $ L^{−1} $ as Fe) in order to achieve considerable removal efficiencies of both compounds in mixed test solutions. Solution pH played an important role and neutral conditions would benefit the removal of both compounds. In addition, several oxidation products (OPs) of both HHCB and AHTN were identified, and degradation pathways were then tentatively proposed. Finally, engineering aspects of Fe(VI) technology in full-scale water treatment applications were also discussed. © The Author(s), under exclusive licence to Springer Nature Switzerland AG 2022 |
| abstract_unstemmed |
Abstract Synthetic musks (SMs), as a group of pharmaceutical and personal care products (PPCPs), have been widely detected in the environment at ng $ L^{−1} $ ~ μg $ L^{−1} $ levels and require our serious attention regarding their presence, toxicity and treatment technologies. In this study, ferrate ($ Fe_{2} %$ O_{4} $2−, Fe(VI)) was employed to treat two typical SMs, galaxolide (HHCB) and tonalide (AHTN), in water solutions. The treatment efficiencies of trace level HHCB and AHTN compounds (16 μg $ L^{−1} $ each) in individual and mixed solutions by Fe(VI) (0–45 mg $ L^{−1} $ as Fe) at pH 5.5–8.5 were assessed, and oxidation products of both compounds were also investigated by means of solid phase extraction coupled with gas chromatography-mass spectrometry (SPE-GC–MS). Results demonstrated that Fe(VI) was more suitable to remove HHCB than AHTN from test solutions. Specifically, when solution pH was 6.5 and Fe(VI) dose was 15–18 mg $ L^{−1} $ as Fe, the removal efficiencies of HHCB and AHTN in individual test solutions were up to 60% and 40%, respectively. Comparatively, much higher Fe(VI) doses were required (up to 38 mg $ L^{−1} $ as Fe) in order to achieve considerable removal efficiencies of both compounds in mixed test solutions. Solution pH played an important role and neutral conditions would benefit the removal of both compounds. In addition, several oxidation products (OPs) of both HHCB and AHTN were identified, and degradation pathways were then tentatively proposed. Finally, engineering aspects of Fe(VI) technology in full-scale water treatment applications were also discussed. © The Author(s), under exclusive licence to Springer Nature Switzerland AG 2022 |
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| title_short |
Laboratory Studies of Removal and Degradation of Galaxolide (HHCB) and Tonalide (AHTN) in Water by Ferrate(VI) |
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https://dx.doi.org/10.1007/s11270-022-05686-7 |
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Zhou, Zhengwei Xue, Yingang Wu, Jun |
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10.1007/s11270-022-05686-7 |
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2024-07-04T02:19:55.846Z |
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| score |
7.3996973 |