A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation

Abstract Zeolite imidazolate frameworks (ZIFs) are a subclass of metal–organic frameworks (MOFs) containing N element, which are always exploited to prepare N-incorporated carbon materials containing rich carbon nanotubes (CNTs) via the pyrolysis. Humic acid layers are regarded as a natural GO-like...
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Autor*in:	Yuan, Hua [verfasserIn] He, Fan Zhao, Jie Cong, Shaoling Wang, Qianyu Yang, Nana Wang, Xiaoqin Xiong, Shanxin Wu, Bohua Wu, Yan

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Humic acid ZIFs PtCoFe Nitrogen doping Carbon skeleton Electrocatalysis

Anmerkung:	© The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022

Übergeordnetes Werk:	Enthalten in: Ionics - Berlin : Springer, 1995, 28(2022), 7 vom: 13. Mai, Seite 3379-3388
Übergeordnetes Werk:	volume:28 ; year:2022 ; number:7 ; day:13 ; month:05 ; pages:3379-3388

Links:	Volltext

DOI / URN:	10.1007/s11581-022-04600-9

Katalog-ID:	SPR047308974

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520			\|a Abstract Zeolite imidazolate frameworks (ZIFs) are a subclass of metal–organic frameworks (MOFs) containing N element, which are always exploited to prepare N-incorporated carbon materials containing rich carbon nanotubes (CNTs) via the pyrolysis. Humic acid layers are regarded as a natural GO-like material due to similar laminate size and thickness, physical and chemical structures, surface polarity, and activity to graphene oxide (GO). Here, a layered humate-ZIF (HA-CoFe-ZIF) composite template is elaborately designed and first constructed by a hydrothermal method using sodium humate as the substrate. An N-incorporated carbon skeleton (NCS) support assembled by CNTs and graphene layers is then achieved after the segmented pyrolysis and acid etching. Afterwards, a PtCoFe/NCS electrocatalyst with high catalytic activity and cycling stability for methanol oxidation reaction (MOR) is purposefully synthesized by loading PtCoFe nanoparticles on the NCS surface via ethylene glycol-sodium borohydride (EG-$ NaBH_{4} $) double reduction. The supported catalyst constructs a composite structure with good dispersibility of metal nanoparticles on the NCS surface due to the oriented coordination bonding between metal and nitrogen incorporated in the NCS. The large specific surface and good electrical conductivity of the NCS support together guarantee high MOR electrocatalytic activity, stability, and CO tolerance ability of PtCoFe nanoparticles.
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700	1		\|a Yang, Nana \|4 aut
700	1		\|a Wang, Xiaoqin \|4 aut
700	1		\|a Xiong, Shanxin \|4 aut
700	1		\|a Wu, Bohua \|4 aut
700	1		\|a Wu, Yan \|4 aut
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912			\|a GBV_ILN_151
912			\|a GBV_ILN_152
912			\|a GBV_ILN_161
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912			\|a GBV_ILN_171
912			\|a GBV_ILN_187
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912			\|a GBV_ILN_224
912			\|a GBV_ILN_230
912			\|a GBV_ILN_250
912			\|a GBV_ILN_281
912			\|a GBV_ILN_285
912			\|a GBV_ILN_293
912			\|a GBV_ILN_370
912			\|a GBV_ILN_602
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912			\|a GBV_ILN_2025
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912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2037
912			\|a GBV_ILN_2038
912			\|a GBV_ILN_2039
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2055
912			\|a GBV_ILN_2056
912			\|a GBV_ILN_2057
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
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912			\|a GBV_ILN_2068
912			\|a GBV_ILN_2088
912			\|a GBV_ILN_2093
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912			\|a GBV_ILN_2108
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912			\|a GBV_ILN_2112
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allfields	10.1007/s11581-022-04600-9 doi (DE-627)SPR047308974 (SPR)s11581-022-04600-9-e DE-627 ger DE-627 rakwb eng Yuan, Hua verfasserin aut A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract Zeolite imidazolate frameworks (ZIFs) are a subclass of metal–organic frameworks (MOFs) containing N element, which are always exploited to prepare N-incorporated carbon materials containing rich carbon nanotubes (CNTs) via the pyrolysis. Humic acid layers are regarded as a natural GO-like material due to similar laminate size and thickness, physical and chemical structures, surface polarity, and activity to graphene oxide (GO). Here, a layered humate-ZIF (HA-CoFe-ZIF) composite template is elaborately designed and first constructed by a hydrothermal method using sodium humate as the substrate. An N-incorporated carbon skeleton (NCS) support assembled by CNTs and graphene layers is then achieved after the segmented pyrolysis and acid etching. Afterwards, a PtCoFe/NCS electrocatalyst with high catalytic activity and cycling stability for methanol oxidation reaction (MOR) is purposefully synthesized by loading PtCoFe nanoparticles on the NCS surface via ethylene glycol-sodium borohydride (EG-$ NaBH_{4} $) double reduction. The supported catalyst constructs a composite structure with good dispersibility of metal nanoparticles on the NCS surface due to the oriented coordination bonding between metal and nitrogen incorporated in the NCS. The large specific surface and good electrical conductivity of the NCS support together guarantee high MOR electrocatalytic activity, stability, and CO tolerance ability of PtCoFe nanoparticles. Humic acid (dpeaa)DE-He213 ZIFs (dpeaa)DE-He213 PtCoFe (dpeaa)DE-He213 Nitrogen doping (dpeaa)DE-He213 Carbon skeleton (dpeaa)DE-He213 Electrocatalysis (dpeaa)DE-He213 He, Fan aut Zhao, Jie aut Cong, Shaoling aut Wang, Qianyu aut Yang, Nana aut Wang, Xiaoqin aut Xiong, Shanxin aut Wu, Bohua aut Wu, Yan aut Enthalten in Ionics Berlin : Springer, 1995 28(2022), 7 vom: 13. Mai, Seite 3379-3388 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:28 year:2022 number:7 day:13 month:05 pages:3379-3388 https://dx.doi.org/10.1007/s11581-022-04600-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 28 2022 7 13 05 3379-3388
spelling	10.1007/s11581-022-04600-9 doi (DE-627)SPR047308974 (SPR)s11581-022-04600-9-e DE-627 ger DE-627 rakwb eng Yuan, Hua verfasserin aut A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract Zeolite imidazolate frameworks (ZIFs) are a subclass of metal–organic frameworks (MOFs) containing N element, which are always exploited to prepare N-incorporated carbon materials containing rich carbon nanotubes (CNTs) via the pyrolysis. Humic acid layers are regarded as a natural GO-like material due to similar laminate size and thickness, physical and chemical structures, surface polarity, and activity to graphene oxide (GO). Here, a layered humate-ZIF (HA-CoFe-ZIF) composite template is elaborately designed and first constructed by a hydrothermal method using sodium humate as the substrate. An N-incorporated carbon skeleton (NCS) support assembled by CNTs and graphene layers is then achieved after the segmented pyrolysis and acid etching. Afterwards, a PtCoFe/NCS electrocatalyst with high catalytic activity and cycling stability for methanol oxidation reaction (MOR) is purposefully synthesized by loading PtCoFe nanoparticles on the NCS surface via ethylene glycol-sodium borohydride (EG-$ NaBH_{4} $) double reduction. The supported catalyst constructs a composite structure with good dispersibility of metal nanoparticles on the NCS surface due to the oriented coordination bonding between metal and nitrogen incorporated in the NCS. The large specific surface and good electrical conductivity of the NCS support together guarantee high MOR electrocatalytic activity, stability, and CO tolerance ability of PtCoFe nanoparticles. Humic acid (dpeaa)DE-He213 ZIFs (dpeaa)DE-He213 PtCoFe (dpeaa)DE-He213 Nitrogen doping (dpeaa)DE-He213 Carbon skeleton (dpeaa)DE-He213 Electrocatalysis (dpeaa)DE-He213 He, Fan aut Zhao, Jie aut Cong, Shaoling aut Wang, Qianyu aut Yang, Nana aut Wang, Xiaoqin aut Xiong, Shanxin aut Wu, Bohua aut Wu, Yan aut Enthalten in Ionics Berlin : Springer, 1995 28(2022), 7 vom: 13. Mai, Seite 3379-3388 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:28 year:2022 number:7 day:13 month:05 pages:3379-3388 https://dx.doi.org/10.1007/s11581-022-04600-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 28 2022 7 13 05 3379-3388
allfields_unstemmed	10.1007/s11581-022-04600-9 doi (DE-627)SPR047308974 (SPR)s11581-022-04600-9-e DE-627 ger DE-627 rakwb eng Yuan, Hua verfasserin aut A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract Zeolite imidazolate frameworks (ZIFs) are a subclass of metal–organic frameworks (MOFs) containing N element, which are always exploited to prepare N-incorporated carbon materials containing rich carbon nanotubes (CNTs) via the pyrolysis. Humic acid layers are regarded as a natural GO-like material due to similar laminate size and thickness, physical and chemical structures, surface polarity, and activity to graphene oxide (GO). Here, a layered humate-ZIF (HA-CoFe-ZIF) composite template is elaborately designed and first constructed by a hydrothermal method using sodium humate as the substrate. An N-incorporated carbon skeleton (NCS) support assembled by CNTs and graphene layers is then achieved after the segmented pyrolysis and acid etching. Afterwards, a PtCoFe/NCS electrocatalyst with high catalytic activity and cycling stability for methanol oxidation reaction (MOR) is purposefully synthesized by loading PtCoFe nanoparticles on the NCS surface via ethylene glycol-sodium borohydride (EG-$ NaBH_{4} $) double reduction. The supported catalyst constructs a composite structure with good dispersibility of metal nanoparticles on the NCS surface due to the oriented coordination bonding between metal and nitrogen incorporated in the NCS. The large specific surface and good electrical conductivity of the NCS support together guarantee high MOR electrocatalytic activity, stability, and CO tolerance ability of PtCoFe nanoparticles. Humic acid (dpeaa)DE-He213 ZIFs (dpeaa)DE-He213 PtCoFe (dpeaa)DE-He213 Nitrogen doping (dpeaa)DE-He213 Carbon skeleton (dpeaa)DE-He213 Electrocatalysis (dpeaa)DE-He213 He, Fan aut Zhao, Jie aut Cong, Shaoling aut Wang, Qianyu aut Yang, Nana aut Wang, Xiaoqin aut Xiong, Shanxin aut Wu, Bohua aut Wu, Yan aut Enthalten in Ionics Berlin : Springer, 1995 28(2022), 7 vom: 13. Mai, Seite 3379-3388 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:28 year:2022 number:7 day:13 month:05 pages:3379-3388 https://dx.doi.org/10.1007/s11581-022-04600-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 28 2022 7 13 05 3379-3388
allfieldsGer	10.1007/s11581-022-04600-9 doi (DE-627)SPR047308974 (SPR)s11581-022-04600-9-e DE-627 ger DE-627 rakwb eng Yuan, Hua verfasserin aut A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract Zeolite imidazolate frameworks (ZIFs) are a subclass of metal–organic frameworks (MOFs) containing N element, which are always exploited to prepare N-incorporated carbon materials containing rich carbon nanotubes (CNTs) via the pyrolysis. Humic acid layers are regarded as a natural GO-like material due to similar laminate size and thickness, physical and chemical structures, surface polarity, and activity to graphene oxide (GO). Here, a layered humate-ZIF (HA-CoFe-ZIF) composite template is elaborately designed and first constructed by a hydrothermal method using sodium humate as the substrate. An N-incorporated carbon skeleton (NCS) support assembled by CNTs and graphene layers is then achieved after the segmented pyrolysis and acid etching. Afterwards, a PtCoFe/NCS electrocatalyst with high catalytic activity and cycling stability for methanol oxidation reaction (MOR) is purposefully synthesized by loading PtCoFe nanoparticles on the NCS surface via ethylene glycol-sodium borohydride (EG-$ NaBH_{4} $) double reduction. The supported catalyst constructs a composite structure with good dispersibility of metal nanoparticles on the NCS surface due to the oriented coordination bonding between metal and nitrogen incorporated in the NCS. The large specific surface and good electrical conductivity of the NCS support together guarantee high MOR electrocatalytic activity, stability, and CO tolerance ability of PtCoFe nanoparticles. Humic acid (dpeaa)DE-He213 ZIFs (dpeaa)DE-He213 PtCoFe (dpeaa)DE-He213 Nitrogen doping (dpeaa)DE-He213 Carbon skeleton (dpeaa)DE-He213 Electrocatalysis (dpeaa)DE-He213 He, Fan aut Zhao, Jie aut Cong, Shaoling aut Wang, Qianyu aut Yang, Nana aut Wang, Xiaoqin aut Xiong, Shanxin aut Wu, Bohua aut Wu, Yan aut Enthalten in Ionics Berlin : Springer, 1995 28(2022), 7 vom: 13. Mai, Seite 3379-3388 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:28 year:2022 number:7 day:13 month:05 pages:3379-3388 https://dx.doi.org/10.1007/s11581-022-04600-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 28 2022 7 13 05 3379-3388
allfieldsSound	10.1007/s11581-022-04600-9 doi (DE-627)SPR047308974 (SPR)s11581-022-04600-9-e DE-627 ger DE-627 rakwb eng Yuan, Hua verfasserin aut A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract Zeolite imidazolate frameworks (ZIFs) are a subclass of metal–organic frameworks (MOFs) containing N element, which are always exploited to prepare N-incorporated carbon materials containing rich carbon nanotubes (CNTs) via the pyrolysis. Humic acid layers are regarded as a natural GO-like material due to similar laminate size and thickness, physical and chemical structures, surface polarity, and activity to graphene oxide (GO). Here, a layered humate-ZIF (HA-CoFe-ZIF) composite template is elaborately designed and first constructed by a hydrothermal method using sodium humate as the substrate. An N-incorporated carbon skeleton (NCS) support assembled by CNTs and graphene layers is then achieved after the segmented pyrolysis and acid etching. Afterwards, a PtCoFe/NCS electrocatalyst with high catalytic activity and cycling stability for methanol oxidation reaction (MOR) is purposefully synthesized by loading PtCoFe nanoparticles on the NCS surface via ethylene glycol-sodium borohydride (EG-$ NaBH_{4} $) double reduction. The supported catalyst constructs a composite structure with good dispersibility of metal nanoparticles on the NCS surface due to the oriented coordination bonding between metal and nitrogen incorporated in the NCS. The large specific surface and good electrical conductivity of the NCS support together guarantee high MOR electrocatalytic activity, stability, and CO tolerance ability of PtCoFe nanoparticles. Humic acid (dpeaa)DE-He213 ZIFs (dpeaa)DE-He213 PtCoFe (dpeaa)DE-He213 Nitrogen doping (dpeaa)DE-He213 Carbon skeleton (dpeaa)DE-He213 Electrocatalysis (dpeaa)DE-He213 He, Fan aut Zhao, Jie aut Cong, Shaoling aut Wang, Qianyu aut Yang, Nana aut Wang, Xiaoqin aut Xiong, Shanxin aut Wu, Bohua aut Wu, Yan aut Enthalten in Ionics Berlin : Springer, 1995 28(2022), 7 vom: 13. Mai, Seite 3379-3388 (DE-627)509398944 (DE-600)2226746-3 1862-0760 nnns volume:28 year:2022 number:7 day:13 month:05 pages:3379-3388 https://dx.doi.org/10.1007/s11581-022-04600-9 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 28 2022 7 13 05 3379-3388
language	English
source	Enthalten in Ionics 28(2022), 7 vom: 13. Mai, Seite 3379-3388 volume:28 year:2022 number:7 day:13 month:05 pages:3379-3388
sourceStr	Enthalten in Ionics 28(2022), 7 vom: 13. Mai, Seite 3379-3388 volume:28 year:2022 number:7 day:13 month:05 pages:3379-3388
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Humic acid ZIFs PtCoFe Nitrogen doping Carbon skeleton Electrocatalysis
isfreeaccess_bool	false
container_title	Ionics
authorswithroles_txt_mv	Yuan, Hua @@aut@@ He, Fan @@aut@@ Zhao, Jie @@aut@@ Cong, Shaoling @@aut@@ Wang, Qianyu @@aut@@ Yang, Nana @@aut@@ Wang, Xiaoqin @@aut@@ Xiong, Shanxin @@aut@@ Wu, Bohua @@aut@@ Wu, Yan @@aut@@
publishDateDaySort_date	2022-05-13T00:00:00Z
hierarchy_top_id	509398944
id	SPR047308974
language_de	englisch
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author	Yuan, Hua
spellingShingle	Yuan, Hua misc Humic acid misc ZIFs misc PtCoFe misc Nitrogen doping misc Carbon skeleton misc Electrocatalysis A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation
authorStr	Yuan, Hua
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topic_title	A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation Humic acid (dpeaa)DE-He213 ZIFs (dpeaa)DE-He213 PtCoFe (dpeaa)DE-He213 Nitrogen doping (dpeaa)DE-He213 Carbon skeleton (dpeaa)DE-He213 Electrocatalysis (dpeaa)DE-He213
topic	misc Humic acid misc ZIFs misc PtCoFe misc Nitrogen doping misc Carbon skeleton misc Electrocatalysis
topic_unstemmed	misc Humic acid misc ZIFs misc PtCoFe misc Nitrogen doping misc Carbon skeleton misc Electrocatalysis
topic_browse	misc Humic acid misc ZIFs misc PtCoFe misc Nitrogen doping misc Carbon skeleton misc Electrocatalysis
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title	A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation
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title_full	A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation
author_sort	Yuan, Hua
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author_browse	Yuan, Hua He, Fan Zhao, Jie Cong, Shaoling Wang, Qianyu Yang, Nana Wang, Xiaoqin Xiong, Shanxin Wu, Bohua Wu, Yan
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doi_str_mv	10.1007/s11581-022-04600-9
title_sort	highly active and durable ptcofe/nitrogen-incorporated carbon skeleton catalyst evolved from ha-cofe-zif template for methanol electrooxidation
title_auth	A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation
abstract	Abstract Zeolite imidazolate frameworks (ZIFs) are a subclass of metal–organic frameworks (MOFs) containing N element, which are always exploited to prepare N-incorporated carbon materials containing rich carbon nanotubes (CNTs) via the pyrolysis. Humic acid layers are regarded as a natural GO-like material due to similar laminate size and thickness, physical and chemical structures, surface polarity, and activity to graphene oxide (GO). Here, a layered humate-ZIF (HA-CoFe-ZIF) composite template is elaborately designed and first constructed by a hydrothermal method using sodium humate as the substrate. An N-incorporated carbon skeleton (NCS) support assembled by CNTs and graphene layers is then achieved after the segmented pyrolysis and acid etching. Afterwards, a PtCoFe/NCS electrocatalyst with high catalytic activity and cycling stability for methanol oxidation reaction (MOR) is purposefully synthesized by loading PtCoFe nanoparticles on the NCS surface via ethylene glycol-sodium borohydride (EG-$ NaBH_{4} $) double reduction. The supported catalyst constructs a composite structure with good dispersibility of metal nanoparticles on the NCS surface due to the oriented coordination bonding between metal and nitrogen incorporated in the NCS. The large specific surface and good electrical conductivity of the NCS support together guarantee high MOR electrocatalytic activity, stability, and CO tolerance ability of PtCoFe nanoparticles. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022
abstractGer	Abstract Zeolite imidazolate frameworks (ZIFs) are a subclass of metal–organic frameworks (MOFs) containing N element, which are always exploited to prepare N-incorporated carbon materials containing rich carbon nanotubes (CNTs) via the pyrolysis. Humic acid layers are regarded as a natural GO-like material due to similar laminate size and thickness, physical and chemical structures, surface polarity, and activity to graphene oxide (GO). Here, a layered humate-ZIF (HA-CoFe-ZIF) composite template is elaborately designed and first constructed by a hydrothermal method using sodium humate as the substrate. An N-incorporated carbon skeleton (NCS) support assembled by CNTs and graphene layers is then achieved after the segmented pyrolysis and acid etching. Afterwards, a PtCoFe/NCS electrocatalyst with high catalytic activity and cycling stability for methanol oxidation reaction (MOR) is purposefully synthesized by loading PtCoFe nanoparticles on the NCS surface via ethylene glycol-sodium borohydride (EG-$ NaBH_{4} $) double reduction. The supported catalyst constructs a composite structure with good dispersibility of metal nanoparticles on the NCS surface due to the oriented coordination bonding between metal and nitrogen incorporated in the NCS. The large specific surface and good electrical conductivity of the NCS support together guarantee high MOR electrocatalytic activity, stability, and CO tolerance ability of PtCoFe nanoparticles. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022
abstract_unstemmed	Abstract Zeolite imidazolate frameworks (ZIFs) are a subclass of metal–organic frameworks (MOFs) containing N element, which are always exploited to prepare N-incorporated carbon materials containing rich carbon nanotubes (CNTs) via the pyrolysis. Humic acid layers are regarded as a natural GO-like material due to similar laminate size and thickness, physical and chemical structures, surface polarity, and activity to graphene oxide (GO). Here, a layered humate-ZIF (HA-CoFe-ZIF) composite template is elaborately designed and first constructed by a hydrothermal method using sodium humate as the substrate. An N-incorporated carbon skeleton (NCS) support assembled by CNTs and graphene layers is then achieved after the segmented pyrolysis and acid etching. Afterwards, a PtCoFe/NCS electrocatalyst with high catalytic activity and cycling stability for methanol oxidation reaction (MOR) is purposefully synthesized by loading PtCoFe nanoparticles on the NCS surface via ethylene glycol-sodium borohydride (EG-$ NaBH_{4} $) double reduction. The supported catalyst constructs a composite structure with good dispersibility of metal nanoparticles on the NCS surface due to the oriented coordination bonding between metal and nitrogen incorporated in the NCS. The large specific surface and good electrical conductivity of the NCS support together guarantee high MOR electrocatalytic activity, stability, and CO tolerance ability of PtCoFe nanoparticles. © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2022
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title_short	A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation
url	https://dx.doi.org/10.1007/s11581-022-04600-9
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author2	He, Fan Zhao, Jie Cong, Shaoling Wang, Qianyu Yang, Nana Wang, Xiaoqin Xiong, Shanxin Wu, Bohua Wu, Yan
author2Str	He, Fan Zhao, Jie Cong, Shaoling Wang, Qianyu Yang, Nana Wang, Xiaoqin Xiong, Shanxin Wu, Bohua Wu, Yan
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doi_str	10.1007/s11581-022-04600-9
up_date	2024-07-04T02:41:01.071Z
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Humic acid layers are regarded as a natural GO-like material due to similar laminate size and thickness, physical and chemical structures, surface polarity, and activity to graphene oxide (GO). Here, a layered humate-ZIF (HA-CoFe-ZIF) composite template is elaborately designed and first constructed by a hydrothermal method using sodium humate as the substrate. An N-incorporated carbon skeleton (NCS) support assembled by CNTs and graphene layers is then achieved after the segmented pyrolysis and acid etching. Afterwards, a PtCoFe/NCS electrocatalyst with high catalytic activity and cycling stability for methanol oxidation reaction (MOR) is purposefully synthesized by loading PtCoFe nanoparticles on the NCS surface via ethylene glycol-sodium borohydride (EG-$ NaBH_{4} $) double reduction. 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A highly active and durable PtCoFe/nitrogen-incorporated carbon skeleton catalyst evolved from HA-CoFe-ZIF template for methanol electrooxidation

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