Synthesis and Luminescent Properties of 1,4,5-Triphenylimidazole‒Phenothiazine Fluorophores
Abstract Two blue donor–acceptor fluorophores with 1,4,5-triphenylimidazole as the electron-transporting unit and phenothiazine as the hole-transporting unit were synthesized by grafting 1,4,5-triphenylimidazole moieties onto 3- and 3,7-position of the phenothiazine core and characterized by spectro...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Qian, Long [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2022 |
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| Schlagwörter: |
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| Anmerkung: |
© The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 |
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| Übergeordnetes Werk: |
Enthalten in: Journal of fluorescence - New York, NY : Springer Science + Business Media B.V., 1991, 32(2022), 5 vom: 21. Juni, Seite 1833-1842 |
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| Übergeordnetes Werk: |
volume:32 ; year:2022 ; number:5 ; day:21 ; month:06 ; pages:1833-1842 |
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| DOI / URN: |
10.1007/s10895-022-02989-0 |
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| Katalog-ID: |
SPR047935790 |
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| 520 | |a Abstract Two blue donor–acceptor fluorophores with 1,4,5-triphenylimidazole as the electron-transporting unit and phenothiazine as the hole-transporting unit were synthesized by grafting 1,4,5-triphenylimidazole moieties onto 3- and 3,7-position of the phenothiazine core and characterized by spectroscopic methods. Their thermal stability, photophysical, electrochemical and electroluminescence properties were systematically investigated. These compounds exhibit good thermal stability and show blue emission in dichloromethane solution and thin solid films. The solution-processed doped devices were fabricated by using these fluorophores as the emitting dopant in 1,3-bis(N-carbazolyl)benzene host, in which the device fabricated from the fluorophore containing two 1,4,5-triphenylimidazole moieties exhibited blue emission with a luminance of 648 cd/$ m^{2} $ and external quantum efficiency of 1.48%. | ||
| 650 | 4 | |a Imidazole derivative |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Phenothiazine |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Photoluminescence |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Electroluminescence |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Yang, Hongyan |4 aut | |
| 700 | 1 | |a Zhao, Yuling |4 aut | |
| 700 | 1 | |a Guo, Yongchun |4 aut | |
| 700 | 1 | |a Yu, Tianzhi |0 (orcid)0000-0001-8180-0445 |4 aut | |
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10.1007/s10895-022-02989-0 doi (DE-627)SPR047935790 (SPR)s10895-022-02989-0-e DE-627 ger DE-627 rakwb eng Qian, Long verfasserin aut Synthesis and Luminescent Properties of 1,4,5-Triphenylimidazole‒Phenothiazine Fluorophores 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 Abstract Two blue donor–acceptor fluorophores with 1,4,5-triphenylimidazole as the electron-transporting unit and phenothiazine as the hole-transporting unit were synthesized by grafting 1,4,5-triphenylimidazole moieties onto 3- and 3,7-position of the phenothiazine core and characterized by spectroscopic methods. Their thermal stability, photophysical, electrochemical and electroluminescence properties were systematically investigated. These compounds exhibit good thermal stability and show blue emission in dichloromethane solution and thin solid films. The solution-processed doped devices were fabricated by using these fluorophores as the emitting dopant in 1,3-bis(N-carbazolyl)benzene host, in which the device fabricated from the fluorophore containing two 1,4,5-triphenylimidazole moieties exhibited blue emission with a luminance of 648 cd/$ m^{2} $ and external quantum efficiency of 1.48%. Imidazole derivative (dpeaa)DE-He213 Phenothiazine (dpeaa)DE-He213 Photoluminescence (dpeaa)DE-He213 Electroluminescence (dpeaa)DE-He213 Yang, Hongyan aut Zhao, Yuling aut Guo, Yongchun aut Yu, Tianzhi (orcid)0000-0001-8180-0445 aut Enthalten in Journal of fluorescence New York, NY : Springer Science + Business Media B.V., 1991 32(2022), 5 vom: 21. Juni, Seite 1833-1842 (DE-627)32057461X (DE-600)2016892-5 1573-4994 nnns volume:32 year:2022 number:5 day:21 month:06 pages:1833-1842 https://dx.doi.org/10.1007/s10895-022-02989-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 32 2022 5 21 06 1833-1842 |
| spelling |
10.1007/s10895-022-02989-0 doi (DE-627)SPR047935790 (SPR)s10895-022-02989-0-e DE-627 ger DE-627 rakwb eng Qian, Long verfasserin aut Synthesis and Luminescent Properties of 1,4,5-Triphenylimidazole‒Phenothiazine Fluorophores 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 Abstract Two blue donor–acceptor fluorophores with 1,4,5-triphenylimidazole as the electron-transporting unit and phenothiazine as the hole-transporting unit were synthesized by grafting 1,4,5-triphenylimidazole moieties onto 3- and 3,7-position of the phenothiazine core and characterized by spectroscopic methods. Their thermal stability, photophysical, electrochemical and electroluminescence properties were systematically investigated. These compounds exhibit good thermal stability and show blue emission in dichloromethane solution and thin solid films. The solution-processed doped devices were fabricated by using these fluorophores as the emitting dopant in 1,3-bis(N-carbazolyl)benzene host, in which the device fabricated from the fluorophore containing two 1,4,5-triphenylimidazole moieties exhibited blue emission with a luminance of 648 cd/$ m^{2} $ and external quantum efficiency of 1.48%. Imidazole derivative (dpeaa)DE-He213 Phenothiazine (dpeaa)DE-He213 Photoluminescence (dpeaa)DE-He213 Electroluminescence (dpeaa)DE-He213 Yang, Hongyan aut Zhao, Yuling aut Guo, Yongchun aut Yu, Tianzhi (orcid)0000-0001-8180-0445 aut Enthalten in Journal of fluorescence New York, NY : Springer Science + Business Media B.V., 1991 32(2022), 5 vom: 21. Juni, Seite 1833-1842 (DE-627)32057461X (DE-600)2016892-5 1573-4994 nnns volume:32 year:2022 number:5 day:21 month:06 pages:1833-1842 https://dx.doi.org/10.1007/s10895-022-02989-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 32 2022 5 21 06 1833-1842 |
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10.1007/s10895-022-02989-0 doi (DE-627)SPR047935790 (SPR)s10895-022-02989-0-e DE-627 ger DE-627 rakwb eng Qian, Long verfasserin aut Synthesis and Luminescent Properties of 1,4,5-Triphenylimidazole‒Phenothiazine Fluorophores 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 Abstract Two blue donor–acceptor fluorophores with 1,4,5-triphenylimidazole as the electron-transporting unit and phenothiazine as the hole-transporting unit were synthesized by grafting 1,4,5-triphenylimidazole moieties onto 3- and 3,7-position of the phenothiazine core and characterized by spectroscopic methods. Their thermal stability, photophysical, electrochemical and electroluminescence properties were systematically investigated. These compounds exhibit good thermal stability and show blue emission in dichloromethane solution and thin solid films. The solution-processed doped devices were fabricated by using these fluorophores as the emitting dopant in 1,3-bis(N-carbazolyl)benzene host, in which the device fabricated from the fluorophore containing two 1,4,5-triphenylimidazole moieties exhibited blue emission with a luminance of 648 cd/$ m^{2} $ and external quantum efficiency of 1.48%. Imidazole derivative (dpeaa)DE-He213 Phenothiazine (dpeaa)DE-He213 Photoluminescence (dpeaa)DE-He213 Electroluminescence (dpeaa)DE-He213 Yang, Hongyan aut Zhao, Yuling aut Guo, Yongchun aut Yu, Tianzhi (orcid)0000-0001-8180-0445 aut Enthalten in Journal of fluorescence New York, NY : Springer Science + Business Media B.V., 1991 32(2022), 5 vom: 21. Juni, Seite 1833-1842 (DE-627)32057461X (DE-600)2016892-5 1573-4994 nnns volume:32 year:2022 number:5 day:21 month:06 pages:1833-1842 https://dx.doi.org/10.1007/s10895-022-02989-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 32 2022 5 21 06 1833-1842 |
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10.1007/s10895-022-02989-0 doi (DE-627)SPR047935790 (SPR)s10895-022-02989-0-e DE-627 ger DE-627 rakwb eng Qian, Long verfasserin aut Synthesis and Luminescent Properties of 1,4,5-Triphenylimidazole‒Phenothiazine Fluorophores 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 Abstract Two blue donor–acceptor fluorophores with 1,4,5-triphenylimidazole as the electron-transporting unit and phenothiazine as the hole-transporting unit were synthesized by grafting 1,4,5-triphenylimidazole moieties onto 3- and 3,7-position of the phenothiazine core and characterized by spectroscopic methods. Their thermal stability, photophysical, electrochemical and electroluminescence properties were systematically investigated. These compounds exhibit good thermal stability and show blue emission in dichloromethane solution and thin solid films. The solution-processed doped devices were fabricated by using these fluorophores as the emitting dopant in 1,3-bis(N-carbazolyl)benzene host, in which the device fabricated from the fluorophore containing two 1,4,5-triphenylimidazole moieties exhibited blue emission with a luminance of 648 cd/$ m^{2} $ and external quantum efficiency of 1.48%. Imidazole derivative (dpeaa)DE-He213 Phenothiazine (dpeaa)DE-He213 Photoluminescence (dpeaa)DE-He213 Electroluminescence (dpeaa)DE-He213 Yang, Hongyan aut Zhao, Yuling aut Guo, Yongchun aut Yu, Tianzhi (orcid)0000-0001-8180-0445 aut Enthalten in Journal of fluorescence New York, NY : Springer Science + Business Media B.V., 1991 32(2022), 5 vom: 21. Juni, Seite 1833-1842 (DE-627)32057461X (DE-600)2016892-5 1573-4994 nnns volume:32 year:2022 number:5 day:21 month:06 pages:1833-1842 https://dx.doi.org/10.1007/s10895-022-02989-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 32 2022 5 21 06 1833-1842 |
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10.1007/s10895-022-02989-0 doi (DE-627)SPR047935790 (SPR)s10895-022-02989-0-e DE-627 ger DE-627 rakwb eng Qian, Long verfasserin aut Synthesis and Luminescent Properties of 1,4,5-Triphenylimidazole‒Phenothiazine Fluorophores 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 Abstract Two blue donor–acceptor fluorophores with 1,4,5-triphenylimidazole as the electron-transporting unit and phenothiazine as the hole-transporting unit were synthesized by grafting 1,4,5-triphenylimidazole moieties onto 3- and 3,7-position of the phenothiazine core and characterized by spectroscopic methods. Their thermal stability, photophysical, electrochemical and electroluminescence properties were systematically investigated. These compounds exhibit good thermal stability and show blue emission in dichloromethane solution and thin solid films. The solution-processed doped devices were fabricated by using these fluorophores as the emitting dopant in 1,3-bis(N-carbazolyl)benzene host, in which the device fabricated from the fluorophore containing two 1,4,5-triphenylimidazole moieties exhibited blue emission with a luminance of 648 cd/$ m^{2} $ and external quantum efficiency of 1.48%. Imidazole derivative (dpeaa)DE-He213 Phenothiazine (dpeaa)DE-He213 Photoluminescence (dpeaa)DE-He213 Electroluminescence (dpeaa)DE-He213 Yang, Hongyan aut Zhao, Yuling aut Guo, Yongchun aut Yu, Tianzhi (orcid)0000-0001-8180-0445 aut Enthalten in Journal of fluorescence New York, NY : Springer Science + Business Media B.V., 1991 32(2022), 5 vom: 21. Juni, Seite 1833-1842 (DE-627)32057461X (DE-600)2016892-5 1573-4994 nnns volume:32 year:2022 number:5 day:21 month:06 pages:1833-1842 https://dx.doi.org/10.1007/s10895-022-02989-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 32 2022 5 21 06 1833-1842 |
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Enthalten in Journal of fluorescence 32(2022), 5 vom: 21. Juni, Seite 1833-1842 volume:32 year:2022 number:5 day:21 month:06 pages:1833-1842 |
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Imidazole derivative Phenothiazine Photoluminescence Electroluminescence |
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Qian, Long @@aut@@ Yang, Hongyan @@aut@@ Zhao, Yuling @@aut@@ Guo, Yongchun @@aut@@ Yu, Tianzhi @@aut@@ |
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Qian, Long |
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Qian, Long misc Imidazole derivative misc Phenothiazine misc Photoluminescence misc Electroluminescence Synthesis and Luminescent Properties of 1,4,5-Triphenylimidazole‒Phenothiazine Fluorophores |
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Synthesis and Luminescent Properties of 1,4,5-Triphenylimidazole‒Phenothiazine Fluorophores Imidazole derivative (dpeaa)DE-He213 Phenothiazine (dpeaa)DE-He213 Photoluminescence (dpeaa)DE-He213 Electroluminescence (dpeaa)DE-He213 |
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synthesis and luminescent properties of 1,4,5-triphenylimidazole‒phenothiazine fluorophores |
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Synthesis and Luminescent Properties of 1,4,5-Triphenylimidazole‒Phenothiazine Fluorophores |
| abstract |
Abstract Two blue donor–acceptor fluorophores with 1,4,5-triphenylimidazole as the electron-transporting unit and phenothiazine as the hole-transporting unit were synthesized by grafting 1,4,5-triphenylimidazole moieties onto 3- and 3,7-position of the phenothiazine core and characterized by spectroscopic methods. Their thermal stability, photophysical, electrochemical and electroluminescence properties were systematically investigated. These compounds exhibit good thermal stability and show blue emission in dichloromethane solution and thin solid films. The solution-processed doped devices were fabricated by using these fluorophores as the emitting dopant in 1,3-bis(N-carbazolyl)benzene host, in which the device fabricated from the fluorophore containing two 1,4,5-triphenylimidazole moieties exhibited blue emission with a luminance of 648 cd/$ m^{2} $ and external quantum efficiency of 1.48%. © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 |
| abstractGer |
Abstract Two blue donor–acceptor fluorophores with 1,4,5-triphenylimidazole as the electron-transporting unit and phenothiazine as the hole-transporting unit were synthesized by grafting 1,4,5-triphenylimidazole moieties onto 3- and 3,7-position of the phenothiazine core and characterized by spectroscopic methods. Their thermal stability, photophysical, electrochemical and electroluminescence properties were systematically investigated. These compounds exhibit good thermal stability and show blue emission in dichloromethane solution and thin solid films. The solution-processed doped devices were fabricated by using these fluorophores as the emitting dopant in 1,3-bis(N-carbazolyl)benzene host, in which the device fabricated from the fluorophore containing two 1,4,5-triphenylimidazole moieties exhibited blue emission with a luminance of 648 cd/$ m^{2} $ and external quantum efficiency of 1.48%. © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 |
| abstract_unstemmed |
Abstract Two blue donor–acceptor fluorophores with 1,4,5-triphenylimidazole as the electron-transporting unit and phenothiazine as the hole-transporting unit were synthesized by grafting 1,4,5-triphenylimidazole moieties onto 3- and 3,7-position of the phenothiazine core and characterized by spectroscopic methods. Their thermal stability, photophysical, electrochemical and electroluminescence properties were systematically investigated. These compounds exhibit good thermal stability and show blue emission in dichloromethane solution and thin solid films. The solution-processed doped devices were fabricated by using these fluorophores as the emitting dopant in 1,3-bis(N-carbazolyl)benzene host, in which the device fabricated from the fluorophore containing two 1,4,5-triphenylimidazole moieties exhibited blue emission with a luminance of 648 cd/$ m^{2} $ and external quantum efficiency of 1.48%. © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 |
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5 |
| title_short |
Synthesis and Luminescent Properties of 1,4,5-Triphenylimidazole‒Phenothiazine Fluorophores |
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https://dx.doi.org/10.1007/s10895-022-02989-0 |
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Yang, Hongyan Zhao, Yuling Guo, Yongchun Yu, Tianzhi |
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| doi_str |
10.1007/s10895-022-02989-0 |
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2024-07-03T15:58:28.230Z |
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