An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light

A novel dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(dmbpy)2]·$ H_{2} $O ($ Fe_{2} $-DMBPY) with 4,4′-dimethyl-2,2′-bipyridine (dmbpy) as ligand are reported on the photocatalytic reduction of $ CO_{2} $, and another easy-to-prepare dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(bpy)2] (...
Ausführliche Beschreibung

Gespeichert in:

Autor*in:	Li, Niang-Xiu [verfasserIn] Lu, Xi-Bo Xu, Quan-Qing Mu, Wei-Hua

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2022

Schlagwörter:	Photocatalytic CO -CO reduction Iron (III)-based

Anmerkung:	© The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022

Übergeordnetes Werk:	Enthalten in: Catalysis letters - Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988, 153(2022), 1 vom: 03. März, Seite 74-82
Übergeordnetes Werk:	volume:153 ; year:2022 ; number:1 ; day:03 ; month:03 ; pages:74-82

Links:	Volltext

DOI / URN:	10.1007/s10562-022-03953-0

Katalog-ID:	SPR048976679

Internformat


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245	1	3	\|a An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light
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520			\|a A novel dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(dmbpy)2]·$ H_{2} $O ($ Fe_{2} $-DMBPY) with 4,4′-dimethyl-2,2′-bipyridine (dmbpy) as ligand are reported on the photocatalytic reduction of $ CO_{2} $, and another easy-to-prepare dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(bpy)2] ($ Fe_{2} $-BPY) with 2,2′-bipyridine (bpy) as ligand is used to make a comparison. The catalytic activity of $ Fe_{2} $-DMBPY is greater than that reported previously, in addition to favorable stability and selectivity. Based on the two intermediates that derived from high-resolution mass spectrometry, density functional theory calculations well confirmed these intermediates can be stable during the experimental process. Graphical Abstract
650		4	\|a Photocatalytic \|7 (dpeaa)DE-He213
650		4	\|a CO \|7 (dpeaa)DE-He213
650		4	\|a -CO reduction \|7 (dpeaa)DE-He213
650		4	\|a Iron (III)-based \|7 (dpeaa)DE-He213
700	1		\|a Lu, Xi-Bo \|4 aut
700	1		\|a Xu, Quan-Qing \|0 (orcid)0000-0001-5377-901X \|4 aut
700	1		\|a Mu, Wei-Hua \|4 aut
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912			\|a GBV_ILN_151
912			\|a GBV_ILN_152
912			\|a GBV_ILN_161
912			\|a GBV_ILN_170
912			\|a GBV_ILN_171
912			\|a GBV_ILN_187
912			\|a GBV_ILN_213
912			\|a GBV_ILN_224
912			\|a GBV_ILN_230
912			\|a GBV_ILN_250
912			\|a GBV_ILN_281
912			\|a GBV_ILN_285
912			\|a GBV_ILN_293
912			\|a GBV_ILN_370
912			\|a GBV_ILN_602
912			\|a GBV_ILN_636
912			\|a GBV_ILN_702
912			\|a GBV_ILN_2001
912			\|a GBV_ILN_2003
912			\|a GBV_ILN_2004
912			\|a GBV_ILN_2005
912			\|a GBV_ILN_2006
912			\|a GBV_ILN_2007
912			\|a GBV_ILN_2008
912			\|a GBV_ILN_2009
912			\|a GBV_ILN_2010
912			\|a GBV_ILN_2011
912			\|a GBV_ILN_2014
912			\|a GBV_ILN_2015
912			\|a GBV_ILN_2020
912			\|a GBV_ILN_2021
912			\|a GBV_ILN_2025
912			\|a GBV_ILN_2026
912			\|a GBV_ILN_2027
912			\|a GBV_ILN_2031
912			\|a GBV_ILN_2034
912			\|a GBV_ILN_2037
912			\|a GBV_ILN_2038
912			\|a GBV_ILN_2039
912			\|a GBV_ILN_2044
912			\|a GBV_ILN_2048
912			\|a GBV_ILN_2049
912			\|a GBV_ILN_2050
912			\|a GBV_ILN_2055
912			\|a GBV_ILN_2056
912			\|a GBV_ILN_2057
912			\|a GBV_ILN_2059
912			\|a GBV_ILN_2061
912			\|a GBV_ILN_2064
912			\|a GBV_ILN_2065
912			\|a GBV_ILN_2068
912			\|a GBV_ILN_2088
912			\|a GBV_ILN_2093
912			\|a GBV_ILN_2106
912			\|a GBV_ILN_2107
912			\|a GBV_ILN_2108
912			\|a GBV_ILN_2110
912			\|a GBV_ILN_2111
912			\|a GBV_ILN_2112
912			\|a GBV_ILN_2113
912			\|a GBV_ILN_2118
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912			\|a GBV_ILN_2147
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912			\|a GBV_ILN_2152
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912			\|a GBV_ILN_2446
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912			\|a GBV_ILN_2522
912			\|a GBV_ILN_2548
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912			\|a GBV_ILN_4037
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912			\|a GBV_ILN_4112
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author_variant	n x l nxl x b l xbl q q x qqx w h m whm
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allfields	10.1007/s10562-022-03953-0 doi (DE-627)SPR048976679 (SPR)s10562-022-03953-0-e DE-627 ger DE-627 rakwb eng Li, Niang-Xiu verfasserin aut An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 A novel dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(dmbpy)2]·$ H_{2} $O ($ Fe_{2} $-DMBPY) with 4,4′-dimethyl-2,2′-bipyridine (dmbpy) as ligand are reported on the photocatalytic reduction of $ CO_{2} $, and another easy-to-prepare dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(bpy)2] ($ Fe_{2} $-BPY) with 2,2′-bipyridine (bpy) as ligand is used to make a comparison. The catalytic activity of $ Fe_{2} $-DMBPY is greater than that reported previously, in addition to favorable stability and selectivity. Based on the two intermediates that derived from high-resolution mass spectrometry, density functional theory calculations well confirmed these intermediates can be stable during the experimental process. Graphical Abstract Photocatalytic (dpeaa)DE-He213 CO (dpeaa)DE-He213 -CO reduction (dpeaa)DE-He213 Iron (III)-based (dpeaa)DE-He213 Lu, Xi-Bo aut Xu, Quan-Qing (orcid)0000-0001-5377-901X aut Mu, Wei-Hua aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 153(2022), 1 vom: 03. März, Seite 74-82 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:153 year:2022 number:1 day:03 month:03 pages:74-82 https://dx.doi.org/10.1007/s10562-022-03953-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 153 2022 1 03 03 74-82
spelling	10.1007/s10562-022-03953-0 doi (DE-627)SPR048976679 (SPR)s10562-022-03953-0-e DE-627 ger DE-627 rakwb eng Li, Niang-Xiu verfasserin aut An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 A novel dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(dmbpy)2]·$ H_{2} $O ($ Fe_{2} $-DMBPY) with 4,4′-dimethyl-2,2′-bipyridine (dmbpy) as ligand are reported on the photocatalytic reduction of $ CO_{2} $, and another easy-to-prepare dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(bpy)2] ($ Fe_{2} $-BPY) with 2,2′-bipyridine (bpy) as ligand is used to make a comparison. The catalytic activity of $ Fe_{2} $-DMBPY is greater than that reported previously, in addition to favorable stability and selectivity. Based on the two intermediates that derived from high-resolution mass spectrometry, density functional theory calculations well confirmed these intermediates can be stable during the experimental process. Graphical Abstract Photocatalytic (dpeaa)DE-He213 CO (dpeaa)DE-He213 -CO reduction (dpeaa)DE-He213 Iron (III)-based (dpeaa)DE-He213 Lu, Xi-Bo aut Xu, Quan-Qing (orcid)0000-0001-5377-901X aut Mu, Wei-Hua aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 153(2022), 1 vom: 03. März, Seite 74-82 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:153 year:2022 number:1 day:03 month:03 pages:74-82 https://dx.doi.org/10.1007/s10562-022-03953-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 153 2022 1 03 03 74-82
allfields_unstemmed	10.1007/s10562-022-03953-0 doi (DE-627)SPR048976679 (SPR)s10562-022-03953-0-e DE-627 ger DE-627 rakwb eng Li, Niang-Xiu verfasserin aut An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 A novel dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(dmbpy)2]·$ H_{2} $O ($ Fe_{2} $-DMBPY) with 4,4′-dimethyl-2,2′-bipyridine (dmbpy) as ligand are reported on the photocatalytic reduction of $ CO_{2} $, and another easy-to-prepare dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(bpy)2] ($ Fe_{2} $-BPY) with 2,2′-bipyridine (bpy) as ligand is used to make a comparison. The catalytic activity of $ Fe_{2} $-DMBPY is greater than that reported previously, in addition to favorable stability and selectivity. Based on the two intermediates that derived from high-resolution mass spectrometry, density functional theory calculations well confirmed these intermediates can be stable during the experimental process. Graphical Abstract Photocatalytic (dpeaa)DE-He213 CO (dpeaa)DE-He213 -CO reduction (dpeaa)DE-He213 Iron (III)-based (dpeaa)DE-He213 Lu, Xi-Bo aut Xu, Quan-Qing (orcid)0000-0001-5377-901X aut Mu, Wei-Hua aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 153(2022), 1 vom: 03. März, Seite 74-82 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:153 year:2022 number:1 day:03 month:03 pages:74-82 https://dx.doi.org/10.1007/s10562-022-03953-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 153 2022 1 03 03 74-82
allfieldsGer	10.1007/s10562-022-03953-0 doi (DE-627)SPR048976679 (SPR)s10562-022-03953-0-e DE-627 ger DE-627 rakwb eng Li, Niang-Xiu verfasserin aut An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 A novel dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(dmbpy)2]·$ H_{2} $O ($ Fe_{2} $-DMBPY) with 4,4′-dimethyl-2,2′-bipyridine (dmbpy) as ligand are reported on the photocatalytic reduction of $ CO_{2} $, and another easy-to-prepare dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(bpy)2] ($ Fe_{2} $-BPY) with 2,2′-bipyridine (bpy) as ligand is used to make a comparison. The catalytic activity of $ Fe_{2} $-DMBPY is greater than that reported previously, in addition to favorable stability and selectivity. Based on the two intermediates that derived from high-resolution mass spectrometry, density functional theory calculations well confirmed these intermediates can be stable during the experimental process. Graphical Abstract Photocatalytic (dpeaa)DE-He213 CO (dpeaa)DE-He213 -CO reduction (dpeaa)DE-He213 Iron (III)-based (dpeaa)DE-He213 Lu, Xi-Bo aut Xu, Quan-Qing (orcid)0000-0001-5377-901X aut Mu, Wei-Hua aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 153(2022), 1 vom: 03. März, Seite 74-82 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:153 year:2022 number:1 day:03 month:03 pages:74-82 https://dx.doi.org/10.1007/s10562-022-03953-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 153 2022 1 03 03 74-82
allfieldsSound	10.1007/s10562-022-03953-0 doi (DE-627)SPR048976679 (SPR)s10562-022-03953-0-e DE-627 ger DE-627 rakwb eng Li, Niang-Xiu verfasserin aut An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 A novel dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(dmbpy)2]·$ H_{2} $O ($ Fe_{2} $-DMBPY) with 4,4′-dimethyl-2,2′-bipyridine (dmbpy) as ligand are reported on the photocatalytic reduction of $ CO_{2} $, and another easy-to-prepare dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(bpy)2] ($ Fe_{2} $-BPY) with 2,2′-bipyridine (bpy) as ligand is used to make a comparison. The catalytic activity of $ Fe_{2} $-DMBPY is greater than that reported previously, in addition to favorable stability and selectivity. Based on the two intermediates that derived from high-resolution mass spectrometry, density functional theory calculations well confirmed these intermediates can be stable during the experimental process. Graphical Abstract Photocatalytic (dpeaa)DE-He213 CO (dpeaa)DE-He213 -CO reduction (dpeaa)DE-He213 Iron (III)-based (dpeaa)DE-He213 Lu, Xi-Bo aut Xu, Quan-Qing (orcid)0000-0001-5377-901X aut Mu, Wei-Hua aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 153(2022), 1 vom: 03. März, Seite 74-82 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:153 year:2022 number:1 day:03 month:03 pages:74-82 https://dx.doi.org/10.1007/s10562-022-03953-0 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 153 2022 1 03 03 74-82
language	English
source	Enthalten in Catalysis letters 153(2022), 1 vom: 03. März, Seite 74-82 volume:153 year:2022 number:1 day:03 month:03 pages:74-82
sourceStr	Enthalten in Catalysis letters 153(2022), 1 vom: 03. März, Seite 74-82 volume:153 year:2022 number:1 day:03 month:03 pages:74-82
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Photocatalytic CO -CO reduction Iron (III)-based
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container_title	Catalysis letters
authorswithroles_txt_mv	Li, Niang-Xiu @@aut@@ Lu, Xi-Bo @@aut@@ Xu, Quan-Qing @@aut@@ Mu, Wei-Hua @@aut@@
publishDateDaySort_date	2022-03-03T00:00:00Z
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author	Li, Niang-Xiu
spellingShingle	Li, Niang-Xiu misc Photocatalytic misc CO misc -CO reduction misc Iron (III)-based An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light
authorStr	Li, Niang-Xiu
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topic_title	An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light Photocatalytic (dpeaa)DE-He213 CO (dpeaa)DE-He213 -CO reduction (dpeaa)DE-He213 Iron (III)-based (dpeaa)DE-He213
topic	misc Photocatalytic misc CO misc -CO reduction misc Iron (III)-based
topic_unstemmed	misc Photocatalytic misc CO misc -CO reduction misc Iron (III)-based
topic_browse	misc Photocatalytic misc CO misc -CO reduction misc Iron (III)-based
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title	An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light
ctrlnum	(DE-627)SPR048976679 (SPR)s10562-022-03953-0-e
title_full	An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light
author_sort	Li, Niang-Xiu
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author_browse	Li, Niang-Xiu Lu, Xi-Bo Xu, Quan-Qing Mu, Wei-Hua
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author-letter	Li, Niang-Xiu
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title_sort	dinuclear iron (iii)-based homogeneous catalytic system: robust, efficient and highly selective $ co_{2} $-to-co conversion under visible light
title_auth	An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light
abstract	A novel dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(dmbpy)2]·$ H_{2} $O ($ Fe_{2} $-DMBPY) with 4,4′-dimethyl-2,2′-bipyridine (dmbpy) as ligand are reported on the photocatalytic reduction of $ CO_{2} $, and another easy-to-prepare dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(bpy)2] ($ Fe_{2} $-BPY) with 2,2′-bipyridine (bpy) as ligand is used to make a comparison. The catalytic activity of $ Fe_{2} $-DMBPY is greater than that reported previously, in addition to favorable stability and selectivity. Based on the two intermediates that derived from high-resolution mass spectrometry, density functional theory calculations well confirmed these intermediates can be stable during the experimental process. Graphical Abstract © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022
abstractGer	A novel dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(dmbpy)2]·$ H_{2} $O ($ Fe_{2} $-DMBPY) with 4,4′-dimethyl-2,2′-bipyridine (dmbpy) as ligand are reported on the photocatalytic reduction of $ CO_{2} $, and another easy-to-prepare dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(bpy)2] ($ Fe_{2} $-BPY) with 2,2′-bipyridine (bpy) as ligand is used to make a comparison. The catalytic activity of $ Fe_{2} $-DMBPY is greater than that reported previously, in addition to favorable stability and selectivity. Based on the two intermediates that derived from high-resolution mass spectrometry, density functional theory calculations well confirmed these intermediates can be stable during the experimental process. Graphical Abstract © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022
abstract_unstemmed	A novel dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(dmbpy)2]·$ H_{2} $O ($ Fe_{2} $-DMBPY) with 4,4′-dimethyl-2,2′-bipyridine (dmbpy) as ligand are reported on the photocatalytic reduction of $ CO_{2} $, and another easy-to-prepare dinuclear Fe (III) complex $ Fe_{2} $O($ NO_{3} $)4(bpy)2] ($ Fe_{2} $-BPY) with 2,2′-bipyridine (bpy) as ligand is used to make a comparison. The catalytic activity of $ Fe_{2} $-DMBPY is greater than that reported previously, in addition to favorable stability and selectivity. Based on the two intermediates that derived from high-resolution mass spectrometry, density functional theory calculations well confirmed these intermediates can be stable during the experimental process. Graphical Abstract © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022
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container_issue	1
title_short	An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light
url	https://dx.doi.org/10.1007/s10562-022-03953-0
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author2	Lu, Xi-Bo Xu, Quan-Qing Mu, Wei-Hua
author2Str	Lu, Xi-Bo Xu, Quan-Qing Mu, Wei-Hua
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doi_str	10.1007/s10562-022-03953-0
up_date	2024-07-03T22:35:19.077Z
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An Dinuclear Iron (III)-Based Homogeneous Catalytic System: Robust, Efficient and Highly Selective $ CO_{2} $-to-CO Conversion under Visible Light

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