Selective Decolorization of Methylene Blue from Methyl Orange in Heterogeneous Fenton-like Reaction
Abstract Selective decolorization of mixed dyestuffs was realized by heterogeneous catalyst. A series of Cu/Febiochar composites containing different amounts of copper and iron were fabricated and all exhibited excellent catalytic performance in the degradation of methyl orange and methylene blue. T...
Ausführliche Beschreibung
Autor*in: |
Wang, Xue [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
Erschienen: |
2023 |
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Anmerkung: |
© University of Tehran 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
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Übergeordnetes Werk: |
Enthalten in: International journal of environmental research - [Cham] : Springer International Publishing, 2007, 17(2023), 1 vom: 13. Jan. |
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Übergeordnetes Werk: |
volume:17 ; year:2023 ; number:1 ; day:13 ; month:01 |
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DOI / URN: |
10.1007/s41742-023-00509-x |
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Katalog-ID: |
SPR04942887X |
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520 | |a Abstract Selective decolorization of mixed dyestuffs was realized by heterogeneous catalyst. A series of Cu/Febiochar composites containing different amounts of copper and iron were fabricated and all exhibited excellent catalytic performance in the degradation of methyl orange and methylene blue. The composite containing the highest metal component with 294.44 mg/g iron and 16.22 mg/g copper could decolorize 97.35% methyl orange in 60 min and 100% methylene blue in 10 min when the composite loading amount was 100 mg/L with 64 mM $ H_{2} %$ O_{2} $ in a 500 mg/L dyestuff solution at pH 3.0. In a solution containing methyl orange and methylene blue both in 200 mg/L and 100 mg/L the composite could decolorize almost 100% methylene blue in 10 min with 48 mM $ H_{2} %$ O_{2} $ while 74.9% methyl orange was left. Investigation revealed that methyl orange was mainly degraded on the catalyst surface and methylene blue in the solution. The selectivity was related to competitive adsorption and phase where dyestuff was degraded and depended on the performance of catalyst. Factors influencing degradation would also impact selectivity. This finding might be viable in application to reuse dyeing wastewater. HighlightsA Cu/Fe@biochar composite was fabricated to be an efficient heterogeneous catalyst.Decolorization rates of MB and MO were different.Selective decolorization of MB and MO happened on the composite.Selective decolorization was carried out at high dyestuff concentration.Mechanism of selective decolorization was discussed. | ||
650 | 4 | |a Heterogeneous Fenton-like catalysis |7 (dpeaa)DE-He213 | |
650 | 4 | |a Selective decolorization |7 (dpeaa)DE-He213 | |
650 | 4 | |a Cu/Fe@biochar |7 (dpeaa)DE-He213 | |
650 | 4 | |a Adsorption |7 (dpeaa)DE-He213 | |
650 | 4 | |a Methyl orange |7 (dpeaa)DE-He213 | |
650 | 4 | |a Methylene blue |7 (dpeaa)DE-He213 | |
700 | 1 | |a Liu, Xiurui |4 aut | |
700 | 1 | |a Yuan, Fang |4 aut | |
700 | 1 | |a Wang, Buyun |4 aut | |
700 | 1 | |a Peng, Qi’an |4 aut | |
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10.1007/s41742-023-00509-x doi (DE-627)SPR04942887X (SPR)s41742-023-00509-x-e DE-627 ger DE-627 rakwb eng Wang, Xue verfasserin aut Selective Decolorization of Methylene Blue from Methyl Orange in Heterogeneous Fenton-like Reaction 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © University of Tehran 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Abstract Selective decolorization of mixed dyestuffs was realized by heterogeneous catalyst. A series of Cu/Febiochar composites containing different amounts of copper and iron were fabricated and all exhibited excellent catalytic performance in the degradation of methyl orange and methylene blue. The composite containing the highest metal component with 294.44 mg/g iron and 16.22 mg/g copper could decolorize 97.35% methyl orange in 60 min and 100% methylene blue in 10 min when the composite loading amount was 100 mg/L with 64 mM $ H_{2} %$ O_{2} $ in a 500 mg/L dyestuff solution at pH 3.0. In a solution containing methyl orange and methylene blue both in 200 mg/L and 100 mg/L the composite could decolorize almost 100% methylene blue in 10 min with 48 mM $ H_{2} %$ O_{2} $ while 74.9% methyl orange was left. Investigation revealed that methyl orange was mainly degraded on the catalyst surface and methylene blue in the solution. The selectivity was related to competitive adsorption and phase where dyestuff was degraded and depended on the performance of catalyst. Factors influencing degradation would also impact selectivity. This finding might be viable in application to reuse dyeing wastewater. HighlightsA Cu/Fe@biochar composite was fabricated to be an efficient heterogeneous catalyst.Decolorization rates of MB and MO were different.Selective decolorization of MB and MO happened on the composite.Selective decolorization was carried out at high dyestuff concentration.Mechanism of selective decolorization was discussed. Heterogeneous Fenton-like catalysis (dpeaa)DE-He213 Selective decolorization (dpeaa)DE-He213 Cu/Fe@biochar (dpeaa)DE-He213 Adsorption (dpeaa)DE-He213 Methyl orange (dpeaa)DE-He213 Methylene blue (dpeaa)DE-He213 Liu, Xiurui aut Yuan, Fang aut Wang, Buyun aut Peng, Qi’an aut Enthalten in International journal of environmental research [Cham] : Springer International Publishing, 2007 17(2023), 1 vom: 13. Jan. (DE-627)552252506 (DE-600)2399844-1 2008-2304 nnns volume:17 year:2023 number:1 day:13 month:01 https://dx.doi.org/10.1007/s41742-023-00509-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_266 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 17 2023 1 13 01 |
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10.1007/s41742-023-00509-x doi (DE-627)SPR04942887X (SPR)s41742-023-00509-x-e DE-627 ger DE-627 rakwb eng Wang, Xue verfasserin aut Selective Decolorization of Methylene Blue from Methyl Orange in Heterogeneous Fenton-like Reaction 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © University of Tehran 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Abstract Selective decolorization of mixed dyestuffs was realized by heterogeneous catalyst. A series of Cu/Febiochar composites containing different amounts of copper and iron were fabricated and all exhibited excellent catalytic performance in the degradation of methyl orange and methylene blue. The composite containing the highest metal component with 294.44 mg/g iron and 16.22 mg/g copper could decolorize 97.35% methyl orange in 60 min and 100% methylene blue in 10 min when the composite loading amount was 100 mg/L with 64 mM $ H_{2} %$ O_{2} $ in a 500 mg/L dyestuff solution at pH 3.0. In a solution containing methyl orange and methylene blue both in 200 mg/L and 100 mg/L the composite could decolorize almost 100% methylene blue in 10 min with 48 mM $ H_{2} %$ O_{2} $ while 74.9% methyl orange was left. Investigation revealed that methyl orange was mainly degraded on the catalyst surface and methylene blue in the solution. The selectivity was related to competitive adsorption and phase where dyestuff was degraded and depended on the performance of catalyst. Factors influencing degradation would also impact selectivity. This finding might be viable in application to reuse dyeing wastewater. HighlightsA Cu/Fe@biochar composite was fabricated to be an efficient heterogeneous catalyst.Decolorization rates of MB and MO were different.Selective decolorization of MB and MO happened on the composite.Selective decolorization was carried out at high dyestuff concentration.Mechanism of selective decolorization was discussed. Heterogeneous Fenton-like catalysis (dpeaa)DE-He213 Selective decolorization (dpeaa)DE-He213 Cu/Fe@biochar (dpeaa)DE-He213 Adsorption (dpeaa)DE-He213 Methyl orange (dpeaa)DE-He213 Methylene blue (dpeaa)DE-He213 Liu, Xiurui aut Yuan, Fang aut Wang, Buyun aut Peng, Qi’an aut Enthalten in International journal of environmental research [Cham] : Springer International Publishing, 2007 17(2023), 1 vom: 13. Jan. (DE-627)552252506 (DE-600)2399844-1 2008-2304 nnns volume:17 year:2023 number:1 day:13 month:01 https://dx.doi.org/10.1007/s41742-023-00509-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_266 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 17 2023 1 13 01 |
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10.1007/s41742-023-00509-x doi (DE-627)SPR04942887X (SPR)s41742-023-00509-x-e DE-627 ger DE-627 rakwb eng Wang, Xue verfasserin aut Selective Decolorization of Methylene Blue from Methyl Orange in Heterogeneous Fenton-like Reaction 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © University of Tehran 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Abstract Selective decolorization of mixed dyestuffs was realized by heterogeneous catalyst. A series of Cu/Febiochar composites containing different amounts of copper and iron were fabricated and all exhibited excellent catalytic performance in the degradation of methyl orange and methylene blue. The composite containing the highest metal component with 294.44 mg/g iron and 16.22 mg/g copper could decolorize 97.35% methyl orange in 60 min and 100% methylene blue in 10 min when the composite loading amount was 100 mg/L with 64 mM $ H_{2} %$ O_{2} $ in a 500 mg/L dyestuff solution at pH 3.0. In a solution containing methyl orange and methylene blue both in 200 mg/L and 100 mg/L the composite could decolorize almost 100% methylene blue in 10 min with 48 mM $ H_{2} %$ O_{2} $ while 74.9% methyl orange was left. Investigation revealed that methyl orange was mainly degraded on the catalyst surface and methylene blue in the solution. The selectivity was related to competitive adsorption and phase where dyestuff was degraded and depended on the performance of catalyst. Factors influencing degradation would also impact selectivity. This finding might be viable in application to reuse dyeing wastewater. HighlightsA Cu/Fe@biochar composite was fabricated to be an efficient heterogeneous catalyst.Decolorization rates of MB and MO were different.Selective decolorization of MB and MO happened on the composite.Selective decolorization was carried out at high dyestuff concentration.Mechanism of selective decolorization was discussed. Heterogeneous Fenton-like catalysis (dpeaa)DE-He213 Selective decolorization (dpeaa)DE-He213 Cu/Fe@biochar (dpeaa)DE-He213 Adsorption (dpeaa)DE-He213 Methyl orange (dpeaa)DE-He213 Methylene blue (dpeaa)DE-He213 Liu, Xiurui aut Yuan, Fang aut Wang, Buyun aut Peng, Qi’an aut Enthalten in International journal of environmental research [Cham] : Springer International Publishing, 2007 17(2023), 1 vom: 13. Jan. (DE-627)552252506 (DE-600)2399844-1 2008-2304 nnns volume:17 year:2023 number:1 day:13 month:01 https://dx.doi.org/10.1007/s41742-023-00509-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_266 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 17 2023 1 13 01 |
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10.1007/s41742-023-00509-x doi (DE-627)SPR04942887X (SPR)s41742-023-00509-x-e DE-627 ger DE-627 rakwb eng Wang, Xue verfasserin aut Selective Decolorization of Methylene Blue from Methyl Orange in Heterogeneous Fenton-like Reaction 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © University of Tehran 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Abstract Selective decolorization of mixed dyestuffs was realized by heterogeneous catalyst. A series of Cu/Febiochar composites containing different amounts of copper and iron were fabricated and all exhibited excellent catalytic performance in the degradation of methyl orange and methylene blue. The composite containing the highest metal component with 294.44 mg/g iron and 16.22 mg/g copper could decolorize 97.35% methyl orange in 60 min and 100% methylene blue in 10 min when the composite loading amount was 100 mg/L with 64 mM $ H_{2} %$ O_{2} $ in a 500 mg/L dyestuff solution at pH 3.0. In a solution containing methyl orange and methylene blue both in 200 mg/L and 100 mg/L the composite could decolorize almost 100% methylene blue in 10 min with 48 mM $ H_{2} %$ O_{2} $ while 74.9% methyl orange was left. Investigation revealed that methyl orange was mainly degraded on the catalyst surface and methylene blue in the solution. The selectivity was related to competitive adsorption and phase where dyestuff was degraded and depended on the performance of catalyst. Factors influencing degradation would also impact selectivity. This finding might be viable in application to reuse dyeing wastewater. HighlightsA Cu/Fe@biochar composite was fabricated to be an efficient heterogeneous catalyst.Decolorization rates of MB and MO were different.Selective decolorization of MB and MO happened on the composite.Selective decolorization was carried out at high dyestuff concentration.Mechanism of selective decolorization was discussed. Heterogeneous Fenton-like catalysis (dpeaa)DE-He213 Selective decolorization (dpeaa)DE-He213 Cu/Fe@biochar (dpeaa)DE-He213 Adsorption (dpeaa)DE-He213 Methyl orange (dpeaa)DE-He213 Methylene blue (dpeaa)DE-He213 Liu, Xiurui aut Yuan, Fang aut Wang, Buyun aut Peng, Qi’an aut Enthalten in International journal of environmental research [Cham] : Springer International Publishing, 2007 17(2023), 1 vom: 13. Jan. (DE-627)552252506 (DE-600)2399844-1 2008-2304 nnns volume:17 year:2023 number:1 day:13 month:01 https://dx.doi.org/10.1007/s41742-023-00509-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_266 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 17 2023 1 13 01 |
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10.1007/s41742-023-00509-x doi (DE-627)SPR04942887X (SPR)s41742-023-00509-x-e DE-627 ger DE-627 rakwb eng Wang, Xue verfasserin aut Selective Decolorization of Methylene Blue from Methyl Orange in Heterogeneous Fenton-like Reaction 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © University of Tehran 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Abstract Selective decolorization of mixed dyestuffs was realized by heterogeneous catalyst. A series of Cu/Febiochar composites containing different amounts of copper and iron were fabricated and all exhibited excellent catalytic performance in the degradation of methyl orange and methylene blue. The composite containing the highest metal component with 294.44 mg/g iron and 16.22 mg/g copper could decolorize 97.35% methyl orange in 60 min and 100% methylene blue in 10 min when the composite loading amount was 100 mg/L with 64 mM $ H_{2} %$ O_{2} $ in a 500 mg/L dyestuff solution at pH 3.0. In a solution containing methyl orange and methylene blue both in 200 mg/L and 100 mg/L the composite could decolorize almost 100% methylene blue in 10 min with 48 mM $ H_{2} %$ O_{2} $ while 74.9% methyl orange was left. Investigation revealed that methyl orange was mainly degraded on the catalyst surface and methylene blue in the solution. The selectivity was related to competitive adsorption and phase where dyestuff was degraded and depended on the performance of catalyst. Factors influencing degradation would also impact selectivity. This finding might be viable in application to reuse dyeing wastewater. HighlightsA Cu/Fe@biochar composite was fabricated to be an efficient heterogeneous catalyst.Decolorization rates of MB and MO were different.Selective decolorization of MB and MO happened on the composite.Selective decolorization was carried out at high dyestuff concentration.Mechanism of selective decolorization was discussed. Heterogeneous Fenton-like catalysis (dpeaa)DE-He213 Selective decolorization (dpeaa)DE-He213 Cu/Fe@biochar (dpeaa)DE-He213 Adsorption (dpeaa)DE-He213 Methyl orange (dpeaa)DE-He213 Methylene blue (dpeaa)DE-He213 Liu, Xiurui aut Yuan, Fang aut Wang, Buyun aut Peng, Qi’an aut Enthalten in International journal of environmental research [Cham] : Springer International Publishing, 2007 17(2023), 1 vom: 13. Jan. (DE-627)552252506 (DE-600)2399844-1 2008-2304 nnns volume:17 year:2023 number:1 day:13 month:01 https://dx.doi.org/10.1007/s41742-023-00509-x lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_266 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 17 2023 1 13 01 |
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Wang, Xue @@aut@@ Liu, Xiurui @@aut@@ Yuan, Fang @@aut@@ Wang, Buyun @@aut@@ Peng, Qi’an @@aut@@ |
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Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Abstract Selective decolorization of mixed dyestuffs was realized by heterogeneous catalyst. A series of Cu/Febiochar composites containing different amounts of copper and iron were fabricated and all exhibited excellent catalytic performance in the degradation of methyl orange and methylene blue. The composite containing the highest metal component with 294.44 mg/g iron and 16.22 mg/g copper could decolorize 97.35% methyl orange in 60 min and 100% methylene blue in 10 min when the composite loading amount was 100 mg/L with 64 mM $ H_{2} %$ O_{2} $ in a 500 mg/L dyestuff solution at pH 3.0. In a solution containing methyl orange and methylene blue both in 200 mg/L and 100 mg/L the composite could decolorize almost 100% methylene blue in 10 min with 48 mM $ H_{2} %$ O_{2} $ while 74.9% methyl orange was left. Investigation revealed that methyl orange was mainly degraded on the catalyst surface and methylene blue in the solution. The selectivity was related to competitive adsorption and phase where dyestuff was degraded and depended on the performance of catalyst. Factors influencing degradation would also impact selectivity. This finding might be viable in application to reuse dyeing wastewater. HighlightsA Cu/Fe@biochar composite was fabricated to be an efficient heterogeneous catalyst.Decolorization rates of MB and MO were different.Selective decolorization of MB and MO happened on the composite.Selective decolorization was carried out at high dyestuff concentration.Mechanism of selective decolorization was discussed.</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Heterogeneous Fenton-like catalysis</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Selective decolorization</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Cu/Fe@biochar</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Adsorption</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Methyl orange</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="650" ind1=" " ind2="4"><subfield code="a">Methylene blue</subfield><subfield code="7">(dpeaa)DE-He213</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Liu, Xiurui</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Yuan, Fang</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Wang, Buyun</subfield><subfield code="4">aut</subfield></datafield><datafield tag="700" ind1="1" ind2=" "><subfield code="a">Peng, Qi’an</subfield><subfield code="4">aut</subfield></datafield><datafield tag="773" ind1="0" ind2="8"><subfield code="i">Enthalten in</subfield><subfield code="t">International journal of environmental research</subfield><subfield code="d">[Cham] : Springer International Publishing, 2007</subfield><subfield code="g">17(2023), 1 vom: 13. 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|
author |
Wang, Xue |
spellingShingle |
Wang, Xue misc Heterogeneous Fenton-like catalysis misc Selective decolorization misc Cu/Fe@biochar misc Adsorption misc Methyl orange misc Methylene blue Selective Decolorization of Methylene Blue from Methyl Orange in Heterogeneous Fenton-like Reaction |
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Wang, Xue |
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2008-2304 |
topic_title |
Selective Decolorization of Methylene Blue from Methyl Orange in Heterogeneous Fenton-like Reaction Heterogeneous Fenton-like catalysis (dpeaa)DE-He213 Selective decolorization (dpeaa)DE-He213 Cu/Fe@biochar (dpeaa)DE-He213 Adsorption (dpeaa)DE-He213 Methyl orange (dpeaa)DE-He213 Methylene blue (dpeaa)DE-He213 |
topic |
misc Heterogeneous Fenton-like catalysis misc Selective decolorization misc Cu/Fe@biochar misc Adsorption misc Methyl orange misc Methylene blue |
topic_unstemmed |
misc Heterogeneous Fenton-like catalysis misc Selective decolorization misc Cu/Fe@biochar misc Adsorption misc Methyl orange misc Methylene blue |
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misc Heterogeneous Fenton-like catalysis misc Selective decolorization misc Cu/Fe@biochar misc Adsorption misc Methyl orange misc Methylene blue |
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Elektronische Aufsätze Aufsätze Elektronische Ressource |
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Selective Decolorization of Methylene Blue from Methyl Orange in Heterogeneous Fenton-like Reaction |
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title_full |
Selective Decolorization of Methylene Blue from Methyl Orange in Heterogeneous Fenton-like Reaction |
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Wang, Xue |
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International journal of environmental research |
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International journal of environmental research |
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Wang, Xue Liu, Xiurui Yuan, Fang Wang, Buyun Peng, Qi’an |
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Wang, Xue |
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10.1007/s41742-023-00509-x |
title_sort |
selective decolorization of methylene blue from methyl orange in heterogeneous fenton-like reaction |
title_auth |
Selective Decolorization of Methylene Blue from Methyl Orange in Heterogeneous Fenton-like Reaction |
abstract |
Abstract Selective decolorization of mixed dyestuffs was realized by heterogeneous catalyst. A series of Cu/Febiochar composites containing different amounts of copper and iron were fabricated and all exhibited excellent catalytic performance in the degradation of methyl orange and methylene blue. The composite containing the highest metal component with 294.44 mg/g iron and 16.22 mg/g copper could decolorize 97.35% methyl orange in 60 min and 100% methylene blue in 10 min when the composite loading amount was 100 mg/L with 64 mM $ H_{2} %$ O_{2} $ in a 500 mg/L dyestuff solution at pH 3.0. In a solution containing methyl orange and methylene blue both in 200 mg/L and 100 mg/L the composite could decolorize almost 100% methylene blue in 10 min with 48 mM $ H_{2} %$ O_{2} $ while 74.9% methyl orange was left. Investigation revealed that methyl orange was mainly degraded on the catalyst surface and methylene blue in the solution. The selectivity was related to competitive adsorption and phase where dyestuff was degraded and depended on the performance of catalyst. Factors influencing degradation would also impact selectivity. This finding might be viable in application to reuse dyeing wastewater. HighlightsA Cu/Fe@biochar composite was fabricated to be an efficient heterogeneous catalyst.Decolorization rates of MB and MO were different.Selective decolorization of MB and MO happened on the composite.Selective decolorization was carried out at high dyestuff concentration.Mechanism of selective decolorization was discussed. © University of Tehran 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
abstractGer |
Abstract Selective decolorization of mixed dyestuffs was realized by heterogeneous catalyst. A series of Cu/Febiochar composites containing different amounts of copper and iron were fabricated and all exhibited excellent catalytic performance in the degradation of methyl orange and methylene blue. The composite containing the highest metal component with 294.44 mg/g iron and 16.22 mg/g copper could decolorize 97.35% methyl orange in 60 min and 100% methylene blue in 10 min when the composite loading amount was 100 mg/L with 64 mM $ H_{2} %$ O_{2} $ in a 500 mg/L dyestuff solution at pH 3.0. In a solution containing methyl orange and methylene blue both in 200 mg/L and 100 mg/L the composite could decolorize almost 100% methylene blue in 10 min with 48 mM $ H_{2} %$ O_{2} $ while 74.9% methyl orange was left. Investigation revealed that methyl orange was mainly degraded on the catalyst surface and methylene blue in the solution. The selectivity was related to competitive adsorption and phase where dyestuff was degraded and depended on the performance of catalyst. Factors influencing degradation would also impact selectivity. This finding might be viable in application to reuse dyeing wastewater. HighlightsA Cu/Fe@biochar composite was fabricated to be an efficient heterogeneous catalyst.Decolorization rates of MB and MO were different.Selective decolorization of MB and MO happened on the composite.Selective decolorization was carried out at high dyestuff concentration.Mechanism of selective decolorization was discussed. © University of Tehran 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
abstract_unstemmed |
Abstract Selective decolorization of mixed dyestuffs was realized by heterogeneous catalyst. A series of Cu/Febiochar composites containing different amounts of copper and iron were fabricated and all exhibited excellent catalytic performance in the degradation of methyl orange and methylene blue. The composite containing the highest metal component with 294.44 mg/g iron and 16.22 mg/g copper could decolorize 97.35% methyl orange in 60 min and 100% methylene blue in 10 min when the composite loading amount was 100 mg/L with 64 mM $ H_{2} %$ O_{2} $ in a 500 mg/L dyestuff solution at pH 3.0. In a solution containing methyl orange and methylene blue both in 200 mg/L and 100 mg/L the composite could decolorize almost 100% methylene blue in 10 min with 48 mM $ H_{2} %$ O_{2} $ while 74.9% methyl orange was left. Investigation revealed that methyl orange was mainly degraded on the catalyst surface and methylene blue in the solution. The selectivity was related to competitive adsorption and phase where dyestuff was degraded and depended on the performance of catalyst. Factors influencing degradation would also impact selectivity. This finding might be viable in application to reuse dyeing wastewater. HighlightsA Cu/Fe@biochar composite was fabricated to be an efficient heterogeneous catalyst.Decolorization rates of MB and MO were different.Selective decolorization of MB and MO happened on the composite.Selective decolorization was carried out at high dyestuff concentration.Mechanism of selective decolorization was discussed. © University of Tehran 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
collection_details |
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container_issue |
1 |
title_short |
Selective Decolorization of Methylene Blue from Methyl Orange in Heterogeneous Fenton-like Reaction |
url |
https://dx.doi.org/10.1007/s41742-023-00509-x |
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author2 |
Liu, Xiurui Yuan, Fang Wang, Buyun Peng, Qi’an |
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Liu, Xiurui Yuan, Fang Wang, Buyun Peng, Qi’an |
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doi_str |
10.1007/s41742-023-00509-x |
up_date |
2024-07-04T00:46:16.236Z |
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|
score |
7.400585 |