Construction of Z-scheme Ti/Ga co-doped ZnO heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation
Innovative solar-driven heterostructure photocatalysts are promising for removing the organic contaminants in the water environment. In this work, a sequence of well-defined Z-scheme Ti-Ga co-doped ZnO/g-$ C_{3} %$ N_{4} $ (TGZ/CN) heterostructure photocatalysts were developed via a simple sol–gel m...
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| Autor*in: |
Guo, Jin [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
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2023 |
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© The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
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Enthalten in: Environmental science and pollution research - Berlin : Springer, 1994, 30(2023), 15 vom: 20. Jan., Seite 43702-43713 |
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| Übergeordnetes Werk: |
volume:30 ; year:2023 ; number:15 ; day:20 ; month:01 ; pages:43702-43713 |
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| DOI / URN: |
10.1007/s11356-023-25276-2 |
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SPR049956884 |
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| 520 | |a Innovative solar-driven heterostructure photocatalysts are promising for removing the organic contaminants in the water environment. In this work, a sequence of well-defined Z-scheme Ti-Ga co-doped ZnO/g-$ C_{3} %$ N_{4} $ (TGZ/CN) heterostructure photocatalysts were developed via a simple sol–gel method and the single-phase dispersion method in order to realize the cooperative improvement from the Ti/Ga co-doping and construction of heterostructure. The synthesized samples were analyzed by a variety of characterization techniques, and the photocatalytic activity was assessed by photodegradation of methylene blue (MB) under visible light irradiation. Compared to the ZnO and g-$ C_{3} %$ N_{4} $, the TGZ/CN composite demonstrated higher photocatalytic performance for the degradation of MB indicating an efficient photocatalytic degradation rate of 95.4% in 105 min under visible light. Moreover, the TGZ/CN photocatalyst exhibited excellent stability after five cycles of MB photodegradation. Furthermore, the as-prepared composites’ possible photocatalytic mechanism was discussed in detail. The improved photocatalytic performance primarily resulted from the effectively reduced band gap of ZnO after Ti/Ga co-doping and the facilitated separation of photoexcited $ e^{−} $/$ h^{+} $ pairs caused by the construction of Z-scheme heterojunction. This work offers novel insights in developing hybrids with highly efficient photocatalytic activity towards future environmental applications. Graphical abstract | ||
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| 650 | 4 | |a Sol–gel |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Graphitic carbon nitride |7 (dpeaa)DE-He213 | |
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| 700 | 1 | |a Zhang, Jiangyu |4 aut | |
| 700 | 1 | |a Fang, Liang |4 aut | |
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10.1007/s11356-023-25276-2 doi (DE-627)SPR049956884 (SPR)s11356-023-25276-2-e DE-627 ger DE-627 rakwb eng Guo, Jin verfasserin aut Construction of Z-scheme Ti/Ga co-doped ZnO heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Innovative solar-driven heterostructure photocatalysts are promising for removing the organic contaminants in the water environment. In this work, a sequence of well-defined Z-scheme Ti-Ga co-doped ZnO/g-$ C_{3} %$ N_{4} $ (TGZ/CN) heterostructure photocatalysts were developed via a simple sol–gel method and the single-phase dispersion method in order to realize the cooperative improvement from the Ti/Ga co-doping and construction of heterostructure. The synthesized samples were analyzed by a variety of characterization techniques, and the photocatalytic activity was assessed by photodegradation of methylene blue (MB) under visible light irradiation. Compared to the ZnO and g-$ C_{3} %$ N_{4} $, the TGZ/CN composite demonstrated higher photocatalytic performance for the degradation of MB indicating an efficient photocatalytic degradation rate of 95.4% in 105 min under visible light. Moreover, the TGZ/CN photocatalyst exhibited excellent stability after five cycles of MB photodegradation. Furthermore, the as-prepared composites’ possible photocatalytic mechanism was discussed in detail. The improved photocatalytic performance primarily resulted from the effectively reduced band gap of ZnO after Ti/Ga co-doping and the facilitated separation of photoexcited $ e^{−} $/$ h^{+} $ pairs caused by the construction of Z-scheme heterojunction. This work offers novel insights in developing hybrids with highly efficient photocatalytic activity towards future environmental applications. Graphical abstract Ti/Ga co-doping ZnO (dpeaa)DE-He213 Sol–gel (dpeaa)DE-He213 Graphitic carbon nitride (dpeaa)DE-He213 Z-scheme heterostructure (dpeaa)DE-He213 Photocatalysis (dpeaa)DE-He213 MB degradation (dpeaa)DE-He213 Sun, Yihua (orcid)0000-0002-0480-7632 aut Luo, Qiuzi aut Zhang, Jiangyu aut Fang, Liang aut Enthalten in Environmental science and pollution research Berlin : Springer, 1994 30(2023), 15 vom: 20. Jan., Seite 43702-43713 (DE-627)320517926 (DE-600)2014192-0 1614-7499 nnns volume:30 year:2023 number:15 day:20 month:01 pages:43702-43713 https://dx.doi.org/10.1007/s11356-023-25276-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 30 2023 15 20 01 43702-43713 |
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10.1007/s11356-023-25276-2 doi (DE-627)SPR049956884 (SPR)s11356-023-25276-2-e DE-627 ger DE-627 rakwb eng Guo, Jin verfasserin aut Construction of Z-scheme Ti/Ga co-doped ZnO heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Innovative solar-driven heterostructure photocatalysts are promising for removing the organic contaminants in the water environment. In this work, a sequence of well-defined Z-scheme Ti-Ga co-doped ZnO/g-$ C_{3} %$ N_{4} $ (TGZ/CN) heterostructure photocatalysts were developed via a simple sol–gel method and the single-phase dispersion method in order to realize the cooperative improvement from the Ti/Ga co-doping and construction of heterostructure. The synthesized samples were analyzed by a variety of characterization techniques, and the photocatalytic activity was assessed by photodegradation of methylene blue (MB) under visible light irradiation. Compared to the ZnO and g-$ C_{3} %$ N_{4} $, the TGZ/CN composite demonstrated higher photocatalytic performance for the degradation of MB indicating an efficient photocatalytic degradation rate of 95.4% in 105 min under visible light. Moreover, the TGZ/CN photocatalyst exhibited excellent stability after five cycles of MB photodegradation. Furthermore, the as-prepared composites’ possible photocatalytic mechanism was discussed in detail. The improved photocatalytic performance primarily resulted from the effectively reduced band gap of ZnO after Ti/Ga co-doping and the facilitated separation of photoexcited $ e^{−} $/$ h^{+} $ pairs caused by the construction of Z-scheme heterojunction. This work offers novel insights in developing hybrids with highly efficient photocatalytic activity towards future environmental applications. Graphical abstract Ti/Ga co-doping ZnO (dpeaa)DE-He213 Sol–gel (dpeaa)DE-He213 Graphitic carbon nitride (dpeaa)DE-He213 Z-scheme heterostructure (dpeaa)DE-He213 Photocatalysis (dpeaa)DE-He213 MB degradation (dpeaa)DE-He213 Sun, Yihua (orcid)0000-0002-0480-7632 aut Luo, Qiuzi aut Zhang, Jiangyu aut Fang, Liang aut Enthalten in Environmental science and pollution research Berlin : Springer, 1994 30(2023), 15 vom: 20. Jan., Seite 43702-43713 (DE-627)320517926 (DE-600)2014192-0 1614-7499 nnns volume:30 year:2023 number:15 day:20 month:01 pages:43702-43713 https://dx.doi.org/10.1007/s11356-023-25276-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 30 2023 15 20 01 43702-43713 |
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10.1007/s11356-023-25276-2 doi (DE-627)SPR049956884 (SPR)s11356-023-25276-2-e DE-627 ger DE-627 rakwb eng Guo, Jin verfasserin aut Construction of Z-scheme Ti/Ga co-doped ZnO heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Innovative solar-driven heterostructure photocatalysts are promising for removing the organic contaminants in the water environment. In this work, a sequence of well-defined Z-scheme Ti-Ga co-doped ZnO/g-$ C_{3} %$ N_{4} $ (TGZ/CN) heterostructure photocatalysts were developed via a simple sol–gel method and the single-phase dispersion method in order to realize the cooperative improvement from the Ti/Ga co-doping and construction of heterostructure. The synthesized samples were analyzed by a variety of characterization techniques, and the photocatalytic activity was assessed by photodegradation of methylene blue (MB) under visible light irradiation. Compared to the ZnO and g-$ C_{3} %$ N_{4} $, the TGZ/CN composite demonstrated higher photocatalytic performance for the degradation of MB indicating an efficient photocatalytic degradation rate of 95.4% in 105 min under visible light. Moreover, the TGZ/CN photocatalyst exhibited excellent stability after five cycles of MB photodegradation. Furthermore, the as-prepared composites’ possible photocatalytic mechanism was discussed in detail. The improved photocatalytic performance primarily resulted from the effectively reduced band gap of ZnO after Ti/Ga co-doping and the facilitated separation of photoexcited $ e^{−} $/$ h^{+} $ pairs caused by the construction of Z-scheme heterojunction. This work offers novel insights in developing hybrids with highly efficient photocatalytic activity towards future environmental applications. Graphical abstract Ti/Ga co-doping ZnO (dpeaa)DE-He213 Sol–gel (dpeaa)DE-He213 Graphitic carbon nitride (dpeaa)DE-He213 Z-scheme heterostructure (dpeaa)DE-He213 Photocatalysis (dpeaa)DE-He213 MB degradation (dpeaa)DE-He213 Sun, Yihua (orcid)0000-0002-0480-7632 aut Luo, Qiuzi aut Zhang, Jiangyu aut Fang, Liang aut Enthalten in Environmental science and pollution research Berlin : Springer, 1994 30(2023), 15 vom: 20. Jan., Seite 43702-43713 (DE-627)320517926 (DE-600)2014192-0 1614-7499 nnns volume:30 year:2023 number:15 day:20 month:01 pages:43702-43713 https://dx.doi.org/10.1007/s11356-023-25276-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 30 2023 15 20 01 43702-43713 |
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10.1007/s11356-023-25276-2 doi (DE-627)SPR049956884 (SPR)s11356-023-25276-2-e DE-627 ger DE-627 rakwb eng Guo, Jin verfasserin aut Construction of Z-scheme Ti/Ga co-doped ZnO heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Innovative solar-driven heterostructure photocatalysts are promising for removing the organic contaminants in the water environment. In this work, a sequence of well-defined Z-scheme Ti-Ga co-doped ZnO/g-$ C_{3} %$ N_{4} $ (TGZ/CN) heterostructure photocatalysts were developed via a simple sol–gel method and the single-phase dispersion method in order to realize the cooperative improvement from the Ti/Ga co-doping and construction of heterostructure. The synthesized samples were analyzed by a variety of characterization techniques, and the photocatalytic activity was assessed by photodegradation of methylene blue (MB) under visible light irradiation. Compared to the ZnO and g-$ C_{3} %$ N_{4} $, the TGZ/CN composite demonstrated higher photocatalytic performance for the degradation of MB indicating an efficient photocatalytic degradation rate of 95.4% in 105 min under visible light. Moreover, the TGZ/CN photocatalyst exhibited excellent stability after five cycles of MB photodegradation. Furthermore, the as-prepared composites’ possible photocatalytic mechanism was discussed in detail. The improved photocatalytic performance primarily resulted from the effectively reduced band gap of ZnO after Ti/Ga co-doping and the facilitated separation of photoexcited $ e^{−} $/$ h^{+} $ pairs caused by the construction of Z-scheme heterojunction. This work offers novel insights in developing hybrids with highly efficient photocatalytic activity towards future environmental applications. Graphical abstract Ti/Ga co-doping ZnO (dpeaa)DE-He213 Sol–gel (dpeaa)DE-He213 Graphitic carbon nitride (dpeaa)DE-He213 Z-scheme heterostructure (dpeaa)DE-He213 Photocatalysis (dpeaa)DE-He213 MB degradation (dpeaa)DE-He213 Sun, Yihua (orcid)0000-0002-0480-7632 aut Luo, Qiuzi aut Zhang, Jiangyu aut Fang, Liang aut Enthalten in Environmental science and pollution research Berlin : Springer, 1994 30(2023), 15 vom: 20. Jan., Seite 43702-43713 (DE-627)320517926 (DE-600)2014192-0 1614-7499 nnns volume:30 year:2023 number:15 day:20 month:01 pages:43702-43713 https://dx.doi.org/10.1007/s11356-023-25276-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 30 2023 15 20 01 43702-43713 |
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10.1007/s11356-023-25276-2 doi (DE-627)SPR049956884 (SPR)s11356-023-25276-2-e DE-627 ger DE-627 rakwb eng Guo, Jin verfasserin aut Construction of Z-scheme Ti/Ga co-doped ZnO heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Innovative solar-driven heterostructure photocatalysts are promising for removing the organic contaminants in the water environment. In this work, a sequence of well-defined Z-scheme Ti-Ga co-doped ZnO/g-$ C_{3} %$ N_{4} $ (TGZ/CN) heterostructure photocatalysts were developed via a simple sol–gel method and the single-phase dispersion method in order to realize the cooperative improvement from the Ti/Ga co-doping and construction of heterostructure. The synthesized samples were analyzed by a variety of characterization techniques, and the photocatalytic activity was assessed by photodegradation of methylene blue (MB) under visible light irradiation. Compared to the ZnO and g-$ C_{3} %$ N_{4} $, the TGZ/CN composite demonstrated higher photocatalytic performance for the degradation of MB indicating an efficient photocatalytic degradation rate of 95.4% in 105 min under visible light. Moreover, the TGZ/CN photocatalyst exhibited excellent stability after five cycles of MB photodegradation. Furthermore, the as-prepared composites’ possible photocatalytic mechanism was discussed in detail. The improved photocatalytic performance primarily resulted from the effectively reduced band gap of ZnO after Ti/Ga co-doping and the facilitated separation of photoexcited $ e^{−} $/$ h^{+} $ pairs caused by the construction of Z-scheme heterojunction. This work offers novel insights in developing hybrids with highly efficient photocatalytic activity towards future environmental applications. Graphical abstract Ti/Ga co-doping ZnO (dpeaa)DE-He213 Sol–gel (dpeaa)DE-He213 Graphitic carbon nitride (dpeaa)DE-He213 Z-scheme heterostructure (dpeaa)DE-He213 Photocatalysis (dpeaa)DE-He213 MB degradation (dpeaa)DE-He213 Sun, Yihua (orcid)0000-0002-0480-7632 aut Luo, Qiuzi aut Zhang, Jiangyu aut Fang, Liang aut Enthalten in Environmental science and pollution research Berlin : Springer, 1994 30(2023), 15 vom: 20. Jan., Seite 43702-43713 (DE-627)320517926 (DE-600)2014192-0 1614-7499 nnns volume:30 year:2023 number:15 day:20 month:01 pages:43702-43713 https://dx.doi.org/10.1007/s11356-023-25276-2 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_381 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2360 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 30 2023 15 20 01 43702-43713 |
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Enthalten in Environmental science and pollution research 30(2023), 15 vom: 20. Jan., Seite 43702-43713 volume:30 year:2023 number:15 day:20 month:01 pages:43702-43713 |
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Ti/Ga co-doping ZnO Sol–gel Graphitic carbon nitride Z-scheme heterostructure Photocatalysis MB degradation |
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Guo, Jin @@aut@@ Sun, Yihua @@aut@@ Luo, Qiuzi @@aut@@ Zhang, Jiangyu @@aut@@ Fang, Liang @@aut@@ |
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Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Innovative solar-driven heterostructure photocatalysts are promising for removing the organic contaminants in the water environment. In this work, a sequence of well-defined Z-scheme Ti-Ga co-doped ZnO/g-$ C_{3} %$ N_{4} $ (TGZ/CN) heterostructure photocatalysts were developed via a simple sol–gel method and the single-phase dispersion method in order to realize the cooperative improvement from the Ti/Ga co-doping and construction of heterostructure. The synthesized samples were analyzed by a variety of characterization techniques, and the photocatalytic activity was assessed by photodegradation of methylene blue (MB) under visible light irradiation. Compared to the ZnO and g-$ C_{3} %$ N_{4} $, the TGZ/CN composite demonstrated higher photocatalytic performance for the degradation of MB indicating an efficient photocatalytic degradation rate of 95.4% in 105 min under visible light. Moreover, the TGZ/CN photocatalyst exhibited excellent stability after five cycles of MB photodegradation. Furthermore, the as-prepared composites’ possible photocatalytic mechanism was discussed in detail. The improved photocatalytic performance primarily resulted from the effectively reduced band gap of ZnO after Ti/Ga co-doping and the facilitated separation of photoexcited $ e^{−} $/$ h^{+} $ pairs caused by the construction of Z-scheme heterojunction. This work offers novel insights in developing hybrids with highly efficient photocatalytic activity towards future environmental applications. 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|
| author |
Guo, Jin |
| spellingShingle |
Guo, Jin misc Ti/Ga co-doping ZnO misc Sol–gel misc Graphitic carbon nitride misc Z-scheme heterostructure misc Photocatalysis misc MB degradation Construction of Z-scheme Ti/Ga co-doped ZnO heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation |
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1614-7499 |
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Construction of Z-scheme Ti/Ga co-doped ZnO heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation Ti/Ga co-doping ZnO (dpeaa)DE-He213 Sol–gel (dpeaa)DE-He213 Graphitic carbon nitride (dpeaa)DE-He213 Z-scheme heterostructure (dpeaa)DE-He213 Photocatalysis (dpeaa)DE-He213 MB degradation (dpeaa)DE-He213 |
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misc Ti/Ga co-doping ZnO misc Sol–gel misc Graphitic carbon nitride misc Z-scheme heterostructure misc Photocatalysis misc MB degradation |
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misc Ti/Ga co-doping ZnO misc Sol–gel misc Graphitic carbon nitride misc Z-scheme heterostructure misc Photocatalysis misc MB degradation |
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Construction of Z-scheme Ti/Ga co-doped ZnO heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation |
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(DE-627)SPR049956884 (SPR)s11356-023-25276-2-e |
| title_full |
Construction of Z-scheme Ti/Ga co-doped ZnO heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation |
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Guo, Jin |
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Environmental science and pollution research |
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Guo, Jin Sun, Yihua Luo, Qiuzi Zhang, Jiangyu Fang, Liang |
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Elektronische Aufsätze |
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Guo, Jin |
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10.1007/s11356-023-25276-2 |
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construction of z-scheme ti/ga co-doped zno heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation |
| title_auth |
Construction of Z-scheme Ti/Ga co-doped ZnO heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation |
| abstract |
Innovative solar-driven heterostructure photocatalysts are promising for removing the organic contaminants in the water environment. In this work, a sequence of well-defined Z-scheme Ti-Ga co-doped ZnO/g-$ C_{3} %$ N_{4} $ (TGZ/CN) heterostructure photocatalysts were developed via a simple sol–gel method and the single-phase dispersion method in order to realize the cooperative improvement from the Ti/Ga co-doping and construction of heterostructure. The synthesized samples were analyzed by a variety of characterization techniques, and the photocatalytic activity was assessed by photodegradation of methylene blue (MB) under visible light irradiation. Compared to the ZnO and g-$ C_{3} %$ N_{4} $, the TGZ/CN composite demonstrated higher photocatalytic performance for the degradation of MB indicating an efficient photocatalytic degradation rate of 95.4% in 105 min under visible light. Moreover, the TGZ/CN photocatalyst exhibited excellent stability after five cycles of MB photodegradation. Furthermore, the as-prepared composites’ possible photocatalytic mechanism was discussed in detail. The improved photocatalytic performance primarily resulted from the effectively reduced band gap of ZnO after Ti/Ga co-doping and the facilitated separation of photoexcited $ e^{−} $/$ h^{+} $ pairs caused by the construction of Z-scheme heterojunction. This work offers novel insights in developing hybrids with highly efficient photocatalytic activity towards future environmental applications. Graphical abstract © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
| abstractGer |
Innovative solar-driven heterostructure photocatalysts are promising for removing the organic contaminants in the water environment. In this work, a sequence of well-defined Z-scheme Ti-Ga co-doped ZnO/g-$ C_{3} %$ N_{4} $ (TGZ/CN) heterostructure photocatalysts were developed via a simple sol–gel method and the single-phase dispersion method in order to realize the cooperative improvement from the Ti/Ga co-doping and construction of heterostructure. The synthesized samples were analyzed by a variety of characterization techniques, and the photocatalytic activity was assessed by photodegradation of methylene blue (MB) under visible light irradiation. Compared to the ZnO and g-$ C_{3} %$ N_{4} $, the TGZ/CN composite demonstrated higher photocatalytic performance for the degradation of MB indicating an efficient photocatalytic degradation rate of 95.4% in 105 min under visible light. Moreover, the TGZ/CN photocatalyst exhibited excellent stability after five cycles of MB photodegradation. Furthermore, the as-prepared composites’ possible photocatalytic mechanism was discussed in detail. The improved photocatalytic performance primarily resulted from the effectively reduced band gap of ZnO after Ti/Ga co-doping and the facilitated separation of photoexcited $ e^{−} $/$ h^{+} $ pairs caused by the construction of Z-scheme heterojunction. This work offers novel insights in developing hybrids with highly efficient photocatalytic activity towards future environmental applications. Graphical abstract © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
| abstract_unstemmed |
Innovative solar-driven heterostructure photocatalysts are promising for removing the organic contaminants in the water environment. In this work, a sequence of well-defined Z-scheme Ti-Ga co-doped ZnO/g-$ C_{3} %$ N_{4} $ (TGZ/CN) heterostructure photocatalysts were developed via a simple sol–gel method and the single-phase dispersion method in order to realize the cooperative improvement from the Ti/Ga co-doping and construction of heterostructure. The synthesized samples were analyzed by a variety of characterization techniques, and the photocatalytic activity was assessed by photodegradation of methylene blue (MB) under visible light irradiation. Compared to the ZnO and g-$ C_{3} %$ N_{4} $, the TGZ/CN composite demonstrated higher photocatalytic performance for the degradation of MB indicating an efficient photocatalytic degradation rate of 95.4% in 105 min under visible light. Moreover, the TGZ/CN photocatalyst exhibited excellent stability after five cycles of MB photodegradation. Furthermore, the as-prepared composites’ possible photocatalytic mechanism was discussed in detail. The improved photocatalytic performance primarily resulted from the effectively reduced band gap of ZnO after Ti/Ga co-doping and the facilitated separation of photoexcited $ e^{−} $/$ h^{+} $ pairs caused by the construction of Z-scheme heterojunction. This work offers novel insights in developing hybrids with highly efficient photocatalytic activity towards future environmental applications. Graphical abstract © The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
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15 |
| title_short |
Construction of Z-scheme Ti/Ga co-doped ZnO heterostructure photocatalyst with graphitic carbon nitride for efficient visible-light-driven dye degradation |
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https://dx.doi.org/10.1007/s11356-023-25276-2 |
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Sun, Yihua Luo, Qiuzi Zhang, Jiangyu Fang, Liang |
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Sun, Yihua Luo, Qiuzi Zhang, Jiangyu Fang, Liang |
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| doi_str |
10.1007/s11356-023-25276-2 |
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2024-07-04T02:55:13.827Z |
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| score |
7.4028063 |