Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides
The novel hybrid materials of ZIF-8 with mesoporous SBA-15 were fabricated through a facile layer-by-layer assembly strategy, and their catalytic performances for cycloaddition reaction between $ CO_{2} $ and epoxide were also preliminarily explored. The structure features and physicochemical proper...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Su, Hongjing [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2022 |
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| Schlagwörter: |
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| Anmerkung: |
© The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 |
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| Übergeordnetes Werk: |
Enthalten in: Catalysis letters - Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988, 153(2022), 5 vom: 24. Juni, Seite 1410-1422 |
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| Übergeordnetes Werk: |
volume:153 ; year:2022 ; number:5 ; day:24 ; month:06 ; pages:1410-1422 |
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| DOI / URN: |
10.1007/s10562-022-03995-4 |
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| Katalog-ID: |
SPR049986805 |
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| 520 | |a The novel hybrid materials of ZIF-8 with mesoporous SBA-15 were fabricated through a facile layer-by-layer assembly strategy, and their catalytic performances for cycloaddition reaction between $ CO_{2} $ and epoxide were also preliminarily explored. The structure features and physicochemical properties of the obtained ZIF-8/SBA-15 by means of various characterizations demonstrated that SBA-15, acting as a structure-directing agent, could not only induce the nucleation of ZIF-8 directionally through the coordination interaction between $ Zn^{2+} $ and silanol groups, but also control the growth of the nanocrystals via the confined space of mesoporous channels. These results easily led to a sharp decrease in the crystal sizes of ZIF-8, accompanied with extensive exposure of the active sites. Particularly, the stability of ZIF-8 distributed in the mesopores of SBA-15 was improved significantly, despite their small size and low coordination. Therefore, the activity of the 5th recycled hybrid catalysts was almost twice that of ZIF-8. This strategy not only facilitates the preparation of a high-efficiency catalyst for cycloaddition reaction, but also opens up a path for synthesis of other metal–organic frameworks (MOFs)/silica materials, which is greatly anticipated for a wide variety of applications. Graphical Abstract | ||
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10.1007/s10562-022-03995-4 doi (DE-627)SPR049986805 (SPR)s10562-022-03995-4-e DE-627 ger DE-627 rakwb eng Su, Hongjing verfasserin aut Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 The novel hybrid materials of ZIF-8 with mesoporous SBA-15 were fabricated through a facile layer-by-layer assembly strategy, and their catalytic performances for cycloaddition reaction between $ CO_{2} $ and epoxide were also preliminarily explored. The structure features and physicochemical properties of the obtained ZIF-8/SBA-15 by means of various characterizations demonstrated that SBA-15, acting as a structure-directing agent, could not only induce the nucleation of ZIF-8 directionally through the coordination interaction between $ Zn^{2+} $ and silanol groups, but also control the growth of the nanocrystals via the confined space of mesoporous channels. These results easily led to a sharp decrease in the crystal sizes of ZIF-8, accompanied with extensive exposure of the active sites. Particularly, the stability of ZIF-8 distributed in the mesopores of SBA-15 was improved significantly, despite their small size and low coordination. Therefore, the activity of the 5th recycled hybrid catalysts was almost twice that of ZIF-8. This strategy not only facilitates the preparation of a high-efficiency catalyst for cycloaddition reaction, but also opens up a path for synthesis of other metal–organic frameworks (MOFs)/silica materials, which is greatly anticipated for a wide variety of applications. Graphical Abstract Hybrid (dpeaa)DE-He213 MOFs (dpeaa)DE-He213 Mesoporous silicas (dpeaa)DE-He213 Carbon dioxide (dpeaa)DE-He213 Cyclic carbonate (dpeaa)DE-He213 Bai, Shiyang (orcid)0000-0003-4694-9062 aut Bing, Liujie aut Deng, Han aut Zhuang, Yuanye aut Sun, Jihong aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 153(2022), 5 vom: 24. Juni, Seite 1410-1422 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:153 year:2022 number:5 day:24 month:06 pages:1410-1422 https://dx.doi.org/10.1007/s10562-022-03995-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 153 2022 5 24 06 1410-1422 |
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10.1007/s10562-022-03995-4 doi (DE-627)SPR049986805 (SPR)s10562-022-03995-4-e DE-627 ger DE-627 rakwb eng Su, Hongjing verfasserin aut Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 The novel hybrid materials of ZIF-8 with mesoporous SBA-15 were fabricated through a facile layer-by-layer assembly strategy, and their catalytic performances for cycloaddition reaction between $ CO_{2} $ and epoxide were also preliminarily explored. The structure features and physicochemical properties of the obtained ZIF-8/SBA-15 by means of various characterizations demonstrated that SBA-15, acting as a structure-directing agent, could not only induce the nucleation of ZIF-8 directionally through the coordination interaction between $ Zn^{2+} $ and silanol groups, but also control the growth of the nanocrystals via the confined space of mesoporous channels. These results easily led to a sharp decrease in the crystal sizes of ZIF-8, accompanied with extensive exposure of the active sites. Particularly, the stability of ZIF-8 distributed in the mesopores of SBA-15 was improved significantly, despite their small size and low coordination. Therefore, the activity of the 5th recycled hybrid catalysts was almost twice that of ZIF-8. This strategy not only facilitates the preparation of a high-efficiency catalyst for cycloaddition reaction, but also opens up a path for synthesis of other metal–organic frameworks (MOFs)/silica materials, which is greatly anticipated for a wide variety of applications. Graphical Abstract Hybrid (dpeaa)DE-He213 MOFs (dpeaa)DE-He213 Mesoporous silicas (dpeaa)DE-He213 Carbon dioxide (dpeaa)DE-He213 Cyclic carbonate (dpeaa)DE-He213 Bai, Shiyang (orcid)0000-0003-4694-9062 aut Bing, Liujie aut Deng, Han aut Zhuang, Yuanye aut Sun, Jihong aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 153(2022), 5 vom: 24. Juni, Seite 1410-1422 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:153 year:2022 number:5 day:24 month:06 pages:1410-1422 https://dx.doi.org/10.1007/s10562-022-03995-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 153 2022 5 24 06 1410-1422 |
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10.1007/s10562-022-03995-4 doi (DE-627)SPR049986805 (SPR)s10562-022-03995-4-e DE-627 ger DE-627 rakwb eng Su, Hongjing verfasserin aut Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 The novel hybrid materials of ZIF-8 with mesoporous SBA-15 were fabricated through a facile layer-by-layer assembly strategy, and their catalytic performances for cycloaddition reaction between $ CO_{2} $ and epoxide were also preliminarily explored. The structure features and physicochemical properties of the obtained ZIF-8/SBA-15 by means of various characterizations demonstrated that SBA-15, acting as a structure-directing agent, could not only induce the nucleation of ZIF-8 directionally through the coordination interaction between $ Zn^{2+} $ and silanol groups, but also control the growth of the nanocrystals via the confined space of mesoporous channels. These results easily led to a sharp decrease in the crystal sizes of ZIF-8, accompanied with extensive exposure of the active sites. Particularly, the stability of ZIF-8 distributed in the mesopores of SBA-15 was improved significantly, despite their small size and low coordination. Therefore, the activity of the 5th recycled hybrid catalysts was almost twice that of ZIF-8. This strategy not only facilitates the preparation of a high-efficiency catalyst for cycloaddition reaction, but also opens up a path for synthesis of other metal–organic frameworks (MOFs)/silica materials, which is greatly anticipated for a wide variety of applications. Graphical Abstract Hybrid (dpeaa)DE-He213 MOFs (dpeaa)DE-He213 Mesoporous silicas (dpeaa)DE-He213 Carbon dioxide (dpeaa)DE-He213 Cyclic carbonate (dpeaa)DE-He213 Bai, Shiyang (orcid)0000-0003-4694-9062 aut Bing, Liujie aut Deng, Han aut Zhuang, Yuanye aut Sun, Jihong aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 153(2022), 5 vom: 24. Juni, Seite 1410-1422 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:153 year:2022 number:5 day:24 month:06 pages:1410-1422 https://dx.doi.org/10.1007/s10562-022-03995-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 153 2022 5 24 06 1410-1422 |
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10.1007/s10562-022-03995-4 doi (DE-627)SPR049986805 (SPR)s10562-022-03995-4-e DE-627 ger DE-627 rakwb eng Su, Hongjing verfasserin aut Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 The novel hybrid materials of ZIF-8 with mesoporous SBA-15 were fabricated through a facile layer-by-layer assembly strategy, and their catalytic performances for cycloaddition reaction between $ CO_{2} $ and epoxide were also preliminarily explored. The structure features and physicochemical properties of the obtained ZIF-8/SBA-15 by means of various characterizations demonstrated that SBA-15, acting as a structure-directing agent, could not only induce the nucleation of ZIF-8 directionally through the coordination interaction between $ Zn^{2+} $ and silanol groups, but also control the growth of the nanocrystals via the confined space of mesoporous channels. These results easily led to a sharp decrease in the crystal sizes of ZIF-8, accompanied with extensive exposure of the active sites. Particularly, the stability of ZIF-8 distributed in the mesopores of SBA-15 was improved significantly, despite their small size and low coordination. Therefore, the activity of the 5th recycled hybrid catalysts was almost twice that of ZIF-8. This strategy not only facilitates the preparation of a high-efficiency catalyst for cycloaddition reaction, but also opens up a path for synthesis of other metal–organic frameworks (MOFs)/silica materials, which is greatly anticipated for a wide variety of applications. Graphical Abstract Hybrid (dpeaa)DE-He213 MOFs (dpeaa)DE-He213 Mesoporous silicas (dpeaa)DE-He213 Carbon dioxide (dpeaa)DE-He213 Cyclic carbonate (dpeaa)DE-He213 Bai, Shiyang (orcid)0000-0003-4694-9062 aut Bing, Liujie aut Deng, Han aut Zhuang, Yuanye aut Sun, Jihong aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 153(2022), 5 vom: 24. Juni, Seite 1410-1422 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:153 year:2022 number:5 day:24 month:06 pages:1410-1422 https://dx.doi.org/10.1007/s10562-022-03995-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 153 2022 5 24 06 1410-1422 |
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10.1007/s10562-022-03995-4 doi (DE-627)SPR049986805 (SPR)s10562-022-03995-4-e DE-627 ger DE-627 rakwb eng Su, Hongjing verfasserin aut Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 The novel hybrid materials of ZIF-8 with mesoporous SBA-15 were fabricated through a facile layer-by-layer assembly strategy, and their catalytic performances for cycloaddition reaction between $ CO_{2} $ and epoxide were also preliminarily explored. The structure features and physicochemical properties of the obtained ZIF-8/SBA-15 by means of various characterizations demonstrated that SBA-15, acting as a structure-directing agent, could not only induce the nucleation of ZIF-8 directionally through the coordination interaction between $ Zn^{2+} $ and silanol groups, but also control the growth of the nanocrystals via the confined space of mesoporous channels. These results easily led to a sharp decrease in the crystal sizes of ZIF-8, accompanied with extensive exposure of the active sites. Particularly, the stability of ZIF-8 distributed in the mesopores of SBA-15 was improved significantly, despite their small size and low coordination. Therefore, the activity of the 5th recycled hybrid catalysts was almost twice that of ZIF-8. This strategy not only facilitates the preparation of a high-efficiency catalyst for cycloaddition reaction, but also opens up a path for synthesis of other metal–organic frameworks (MOFs)/silica materials, which is greatly anticipated for a wide variety of applications. Graphical Abstract Hybrid (dpeaa)DE-He213 MOFs (dpeaa)DE-He213 Mesoporous silicas (dpeaa)DE-He213 Carbon dioxide (dpeaa)DE-He213 Cyclic carbonate (dpeaa)DE-He213 Bai, Shiyang (orcid)0000-0003-4694-9062 aut Bing, Liujie aut Deng, Han aut Zhuang, Yuanye aut Sun, Jihong aut Enthalten in Catalysis letters Dordrecht [u.a.] : Springer Science + Business Media B.V, 1988 153(2022), 5 vom: 24. Juni, Seite 1410-1422 (DE-627)306717638 (DE-600)1501518-X 1572-879X nnns volume:153 year:2022 number:5 day:24 month:06 pages:1410-1422 https://dx.doi.org/10.1007/s10562-022-03995-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 153 2022 5 24 06 1410-1422 |
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Su, Hongjing @@aut@@ Bai, Shiyang @@aut@@ Bing, Liujie @@aut@@ Deng, Han @@aut@@ Zhuang, Yuanye @@aut@@ Sun, Jihong @@aut@@ |
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<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000naa a22002652 4500</leader><controlfield tag="001">SPR049986805</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20230409064652.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">230409s2022 xx |||||o 00| ||eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1007/s10562-022-03995-4</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)SPR049986805</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(SPR)s10562-022-03995-4-e</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Su, Hongjing</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2022</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="500" ind1=" " ind2=" "><subfield code="a">© The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">The novel hybrid materials of ZIF-8 with mesoporous SBA-15 were fabricated through a facile layer-by-layer assembly strategy, and their catalytic performances for cycloaddition reaction between $ CO_{2} $ and epoxide were also preliminarily explored. The structure features and physicochemical properties of the obtained ZIF-8/SBA-15 by means of various characterizations demonstrated that SBA-15, acting as a structure-directing agent, could not only induce the nucleation of ZIF-8 directionally through the coordination interaction between $ Zn^{2+} $ and silanol groups, but also control the growth of the nanocrystals via the confined space of mesoporous channels. These results easily led to a sharp decrease in the crystal sizes of ZIF-8, accompanied with extensive exposure of the active sites. Particularly, the stability of ZIF-8 distributed in the mesopores of SBA-15 was improved significantly, despite their small size and low coordination. Therefore, the activity of the 5th recycled hybrid catalysts was almost twice that of ZIF-8. This strategy not only facilitates the preparation of a high-efficiency catalyst for cycloaddition reaction, but also opens up a path for synthesis of other metal–organic frameworks (MOFs)/silica materials, which is greatly anticipated for a wide variety of applications. 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Su, Hongjing |
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Su, Hongjing misc Hybrid misc MOFs misc Mesoporous silicas misc Carbon dioxide misc Cyclic carbonate Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides |
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Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides Hybrid (dpeaa)DE-He213 MOFs (dpeaa)DE-He213 Mesoporous silicas (dpeaa)DE-He213 Carbon dioxide (dpeaa)DE-He213 Cyclic carbonate (dpeaa)DE-He213 |
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Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides |
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Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides |
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Su, Hongjing Bai, Shiyang Bing, Liujie Deng, Han Zhuang, Yuanye Sun, Jihong |
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fabrication of small-sized zif-8 confined in the mesoporous sba-15 with synergistic enhancement for $ co_{2} $ fixation with epoxides |
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Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides |
| abstract |
The novel hybrid materials of ZIF-8 with mesoporous SBA-15 were fabricated through a facile layer-by-layer assembly strategy, and their catalytic performances for cycloaddition reaction between $ CO_{2} $ and epoxide were also preliminarily explored. The structure features and physicochemical properties of the obtained ZIF-8/SBA-15 by means of various characterizations demonstrated that SBA-15, acting as a structure-directing agent, could not only induce the nucleation of ZIF-8 directionally through the coordination interaction between $ Zn^{2+} $ and silanol groups, but also control the growth of the nanocrystals via the confined space of mesoporous channels. These results easily led to a sharp decrease in the crystal sizes of ZIF-8, accompanied with extensive exposure of the active sites. Particularly, the stability of ZIF-8 distributed in the mesopores of SBA-15 was improved significantly, despite their small size and low coordination. Therefore, the activity of the 5th recycled hybrid catalysts was almost twice that of ZIF-8. This strategy not only facilitates the preparation of a high-efficiency catalyst for cycloaddition reaction, but also opens up a path for synthesis of other metal–organic frameworks (MOFs)/silica materials, which is greatly anticipated for a wide variety of applications. Graphical Abstract © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 |
| abstractGer |
The novel hybrid materials of ZIF-8 with mesoporous SBA-15 were fabricated through a facile layer-by-layer assembly strategy, and their catalytic performances for cycloaddition reaction between $ CO_{2} $ and epoxide were also preliminarily explored. The structure features and physicochemical properties of the obtained ZIF-8/SBA-15 by means of various characterizations demonstrated that SBA-15, acting as a structure-directing agent, could not only induce the nucleation of ZIF-8 directionally through the coordination interaction between $ Zn^{2+} $ and silanol groups, but also control the growth of the nanocrystals via the confined space of mesoporous channels. These results easily led to a sharp decrease in the crystal sizes of ZIF-8, accompanied with extensive exposure of the active sites. Particularly, the stability of ZIF-8 distributed in the mesopores of SBA-15 was improved significantly, despite their small size and low coordination. Therefore, the activity of the 5th recycled hybrid catalysts was almost twice that of ZIF-8. This strategy not only facilitates the preparation of a high-efficiency catalyst for cycloaddition reaction, but also opens up a path for synthesis of other metal–organic frameworks (MOFs)/silica materials, which is greatly anticipated for a wide variety of applications. Graphical Abstract © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 |
| abstract_unstemmed |
The novel hybrid materials of ZIF-8 with mesoporous SBA-15 were fabricated through a facile layer-by-layer assembly strategy, and their catalytic performances for cycloaddition reaction between $ CO_{2} $ and epoxide were also preliminarily explored. The structure features and physicochemical properties of the obtained ZIF-8/SBA-15 by means of various characterizations demonstrated that SBA-15, acting as a structure-directing agent, could not only induce the nucleation of ZIF-8 directionally through the coordination interaction between $ Zn^{2+} $ and silanol groups, but also control the growth of the nanocrystals via the confined space of mesoporous channels. These results easily led to a sharp decrease in the crystal sizes of ZIF-8, accompanied with extensive exposure of the active sites. Particularly, the stability of ZIF-8 distributed in the mesopores of SBA-15 was improved significantly, despite their small size and low coordination. Therefore, the activity of the 5th recycled hybrid catalysts was almost twice that of ZIF-8. This strategy not only facilitates the preparation of a high-efficiency catalyst for cycloaddition reaction, but also opens up a path for synthesis of other metal–organic frameworks (MOFs)/silica materials, which is greatly anticipated for a wide variety of applications. Graphical Abstract © The Author(s), under exclusive licence to Springer Science+Business Media, LLC, part of Springer Nature 2022 |
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5 |
| title_short |
Fabrication of Small-Sized ZIF-8 Confined in the Mesoporous SBA-15 with Synergistic Enhancement for $ CO_{2} $ Fixation with Epoxides |
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https://dx.doi.org/10.1007/s10562-022-03995-4 |
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Bai, Shiyang Bing, Liujie Deng, Han Zhuang, Yuanye Sun, Jihong |
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2024-07-04T03:01:30.923Z |
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| score |
7.401229 |