A novel coral-like garnet for high-performance PEO-based all solid-state batteries
Abstract As one of the most promising next-generation energy storage devices, the lithium-metal battery has been extensively investigated. However, safety issues and undesired lithium dendrite growth hinder its development. The application of solid-state electrolytes has attracted increasing attenti...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Cheng, Jun [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2021 |
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| Schlagwörter: |
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| Anmerkung: |
© Science China Press and Springer-Verlag GmbH Germany, part of Springer Nature 2022 |
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| Übergeordnetes Werk: |
Enthalten in: Science China materials - Beijing : Science China Press, 2014, 65(2021), 2 vom: 26. Aug., Seite 364-372 |
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| Übergeordnetes Werk: |
volume:65 ; year:2021 ; number:2 ; day:26 ; month:08 ; pages:364-372 |
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| DOI / URN: |
10.1007/s40843-021-1748-7 |
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| Katalog-ID: |
SPR050455885 |
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| 245 | 1 | 2 | |a A novel coral-like garnet for high-performance PEO-based all solid-state batteries |
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| 520 | |a Abstract As one of the most promising next-generation energy storage devices, the lithium-metal battery has been extensively investigated. However, safety issues and undesired lithium dendrite growth hinder its development. The application of solid-state electrolytes has attracted increasing attention as they can solve safety issues and show great potential to inhibit the growth of lithium dendrites. Polyethylene oxide (PEO)-based electrolytes are very promising due to their enhanced safety and excellent flexibility. However, they suffer from low ionic conductivity at room temperature and cannot effectively inhibit lithium dendrites at high temperatures due to the intrinsic semicrystalline properties and poor mechanical strength. In this work, a novel coral-like $ Li_{6.25} %$ Al_{0.25} %$ La_{3} %$ Zr_{2} $-$ O_{12} $ (C-LALZO) is synthesized to serve as an active ceramic filler in PEO. The PEO with LALZO coral (PLC) exhibits increased ionic conductivity and mechanical strength, which leads to uniform deposition/stripping of lithium metal. The Li symmetric cells with PLC do not cause a short circuit after cycling for 1500 h at 60°C. The assembled $ LiFePO_{4} $/PLC/Li batteries display excellent cycling stability at both 60 and 50°C. This work reveals that the electrochemical properties of the composite electrolyte can be effectively improved by tuning the microstructure of the filler, such as the C-LALZO architecture. | ||
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| 650 | 4 | |a composite solid-state electrolyte |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a all-solid-state battery |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Hou, Guangmei |4 aut | |
| 700 | 1 | |a Sun, Qing |4 aut | |
| 700 | 1 | |a Chen, Qiong |4 aut | |
| 700 | 1 | |a Li, Deping |4 aut | |
| 700 | 1 | |a Li, Jianwei |4 aut | |
| 700 | 1 | |a Zeng, Zhen |4 aut | |
| 700 | 1 | |a Li, Kaikai |4 aut | |
| 700 | 1 | |a Yuan, Qunhui |4 aut | |
| 700 | 1 | |a Wang, Jiajun |4 aut | |
| 700 | 1 | |a Ci, Lijie |4 aut | |
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10.1007/s40843-021-1748-7 doi (DE-627)SPR050455885 (SPR)s40843-021-1748-7-e DE-627 ger DE-627 rakwb eng Cheng, Jun verfasserin aut A novel coral-like garnet for high-performance PEO-based all solid-state batteries 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Science China Press and Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract As one of the most promising next-generation energy storage devices, the lithium-metal battery has been extensively investigated. However, safety issues and undesired lithium dendrite growth hinder its development. The application of solid-state electrolytes has attracted increasing attention as they can solve safety issues and show great potential to inhibit the growth of lithium dendrites. Polyethylene oxide (PEO)-based electrolytes are very promising due to their enhanced safety and excellent flexibility. However, they suffer from low ionic conductivity at room temperature and cannot effectively inhibit lithium dendrites at high temperatures due to the intrinsic semicrystalline properties and poor mechanical strength. In this work, a novel coral-like $ Li_{6.25} %$ Al_{0.25} %$ La_{3} %$ Zr_{2} $-$ O_{12} $ (C-LALZO) is synthesized to serve as an active ceramic filler in PEO. The PEO with LALZO coral (PLC) exhibits increased ionic conductivity and mechanical strength, which leads to uniform deposition/stripping of lithium metal. The Li symmetric cells with PLC do not cause a short circuit after cycling for 1500 h at 60°C. The assembled $ LiFePO_{4} $/PLC/Li batteries display excellent cycling stability at both 60 and 50°C. This work reveals that the electrochemical properties of the composite electrolyte can be effectively improved by tuning the microstructure of the filler, such as the C-LALZO architecture. coral-like garnet (dpeaa)DE-He213 composite solid-state electrolyte (dpeaa)DE-He213 all-solid-state battery (dpeaa)DE-He213 Hou, Guangmei aut Sun, Qing aut Chen, Qiong aut Li, Deping aut Li, Jianwei aut Zeng, Zhen aut Li, Kaikai aut Yuan, Qunhui aut Wang, Jiajun aut Ci, Lijie aut Enthalten in Science China materials Beijing : Science China Press, 2014 65(2021), 2 vom: 26. Aug., Seite 364-372 (DE-627)815914733 (DE-600)2806677-7 2199-4501 nnns volume:65 year:2021 number:2 day:26 month:08 pages:364-372 https://dx.doi.org/10.1007/s40843-021-1748-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 65 2021 2 26 08 364-372 |
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10.1007/s40843-021-1748-7 doi (DE-627)SPR050455885 (SPR)s40843-021-1748-7-e DE-627 ger DE-627 rakwb eng Cheng, Jun verfasserin aut A novel coral-like garnet for high-performance PEO-based all solid-state batteries 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Science China Press and Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract As one of the most promising next-generation energy storage devices, the lithium-metal battery has been extensively investigated. However, safety issues and undesired lithium dendrite growth hinder its development. The application of solid-state electrolytes has attracted increasing attention as they can solve safety issues and show great potential to inhibit the growth of lithium dendrites. Polyethylene oxide (PEO)-based electrolytes are very promising due to their enhanced safety and excellent flexibility. However, they suffer from low ionic conductivity at room temperature and cannot effectively inhibit lithium dendrites at high temperatures due to the intrinsic semicrystalline properties and poor mechanical strength. In this work, a novel coral-like $ Li_{6.25} %$ Al_{0.25} %$ La_{3} %$ Zr_{2} $-$ O_{12} $ (C-LALZO) is synthesized to serve as an active ceramic filler in PEO. The PEO with LALZO coral (PLC) exhibits increased ionic conductivity and mechanical strength, which leads to uniform deposition/stripping of lithium metal. The Li symmetric cells with PLC do not cause a short circuit after cycling for 1500 h at 60°C. The assembled $ LiFePO_{4} $/PLC/Li batteries display excellent cycling stability at both 60 and 50°C. This work reveals that the electrochemical properties of the composite electrolyte can be effectively improved by tuning the microstructure of the filler, such as the C-LALZO architecture. coral-like garnet (dpeaa)DE-He213 composite solid-state electrolyte (dpeaa)DE-He213 all-solid-state battery (dpeaa)DE-He213 Hou, Guangmei aut Sun, Qing aut Chen, Qiong aut Li, Deping aut Li, Jianwei aut Zeng, Zhen aut Li, Kaikai aut Yuan, Qunhui aut Wang, Jiajun aut Ci, Lijie aut Enthalten in Science China materials Beijing : Science China Press, 2014 65(2021), 2 vom: 26. Aug., Seite 364-372 (DE-627)815914733 (DE-600)2806677-7 2199-4501 nnns volume:65 year:2021 number:2 day:26 month:08 pages:364-372 https://dx.doi.org/10.1007/s40843-021-1748-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 65 2021 2 26 08 364-372 |
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10.1007/s40843-021-1748-7 doi (DE-627)SPR050455885 (SPR)s40843-021-1748-7-e DE-627 ger DE-627 rakwb eng Cheng, Jun verfasserin aut A novel coral-like garnet for high-performance PEO-based all solid-state batteries 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Science China Press and Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract As one of the most promising next-generation energy storage devices, the lithium-metal battery has been extensively investigated. However, safety issues and undesired lithium dendrite growth hinder its development. The application of solid-state electrolytes has attracted increasing attention as they can solve safety issues and show great potential to inhibit the growth of lithium dendrites. Polyethylene oxide (PEO)-based electrolytes are very promising due to their enhanced safety and excellent flexibility. However, they suffer from low ionic conductivity at room temperature and cannot effectively inhibit lithium dendrites at high temperatures due to the intrinsic semicrystalline properties and poor mechanical strength. In this work, a novel coral-like $ Li_{6.25} %$ Al_{0.25} %$ La_{3} %$ Zr_{2} $-$ O_{12} $ (C-LALZO) is synthesized to serve as an active ceramic filler in PEO. The PEO with LALZO coral (PLC) exhibits increased ionic conductivity and mechanical strength, which leads to uniform deposition/stripping of lithium metal. The Li symmetric cells with PLC do not cause a short circuit after cycling for 1500 h at 60°C. The assembled $ LiFePO_{4} $/PLC/Li batteries display excellent cycling stability at both 60 and 50°C. This work reveals that the electrochemical properties of the composite electrolyte can be effectively improved by tuning the microstructure of the filler, such as the C-LALZO architecture. coral-like garnet (dpeaa)DE-He213 composite solid-state electrolyte (dpeaa)DE-He213 all-solid-state battery (dpeaa)DE-He213 Hou, Guangmei aut Sun, Qing aut Chen, Qiong aut Li, Deping aut Li, Jianwei aut Zeng, Zhen aut Li, Kaikai aut Yuan, Qunhui aut Wang, Jiajun aut Ci, Lijie aut Enthalten in Science China materials Beijing : Science China Press, 2014 65(2021), 2 vom: 26. Aug., Seite 364-372 (DE-627)815914733 (DE-600)2806677-7 2199-4501 nnns volume:65 year:2021 number:2 day:26 month:08 pages:364-372 https://dx.doi.org/10.1007/s40843-021-1748-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 65 2021 2 26 08 364-372 |
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10.1007/s40843-021-1748-7 doi (DE-627)SPR050455885 (SPR)s40843-021-1748-7-e DE-627 ger DE-627 rakwb eng Cheng, Jun verfasserin aut A novel coral-like garnet for high-performance PEO-based all solid-state batteries 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Science China Press and Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract As one of the most promising next-generation energy storage devices, the lithium-metal battery has been extensively investigated. However, safety issues and undesired lithium dendrite growth hinder its development. The application of solid-state electrolytes has attracted increasing attention as they can solve safety issues and show great potential to inhibit the growth of lithium dendrites. Polyethylene oxide (PEO)-based electrolytes are very promising due to their enhanced safety and excellent flexibility. However, they suffer from low ionic conductivity at room temperature and cannot effectively inhibit lithium dendrites at high temperatures due to the intrinsic semicrystalline properties and poor mechanical strength. In this work, a novel coral-like $ Li_{6.25} %$ Al_{0.25} %$ La_{3} %$ Zr_{2} $-$ O_{12} $ (C-LALZO) is synthesized to serve as an active ceramic filler in PEO. The PEO with LALZO coral (PLC) exhibits increased ionic conductivity and mechanical strength, which leads to uniform deposition/stripping of lithium metal. The Li symmetric cells with PLC do not cause a short circuit after cycling for 1500 h at 60°C. The assembled $ LiFePO_{4} $/PLC/Li batteries display excellent cycling stability at both 60 and 50°C. This work reveals that the electrochemical properties of the composite electrolyte can be effectively improved by tuning the microstructure of the filler, such as the C-LALZO architecture. coral-like garnet (dpeaa)DE-He213 composite solid-state electrolyte (dpeaa)DE-He213 all-solid-state battery (dpeaa)DE-He213 Hou, Guangmei aut Sun, Qing aut Chen, Qiong aut Li, Deping aut Li, Jianwei aut Zeng, Zhen aut Li, Kaikai aut Yuan, Qunhui aut Wang, Jiajun aut Ci, Lijie aut Enthalten in Science China materials Beijing : Science China Press, 2014 65(2021), 2 vom: 26. Aug., Seite 364-372 (DE-627)815914733 (DE-600)2806677-7 2199-4501 nnns volume:65 year:2021 number:2 day:26 month:08 pages:364-372 https://dx.doi.org/10.1007/s40843-021-1748-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 65 2021 2 26 08 364-372 |
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10.1007/s40843-021-1748-7 doi (DE-627)SPR050455885 (SPR)s40843-021-1748-7-e DE-627 ger DE-627 rakwb eng Cheng, Jun verfasserin aut A novel coral-like garnet for high-performance PEO-based all solid-state batteries 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Science China Press and Springer-Verlag GmbH Germany, part of Springer Nature 2022 Abstract As one of the most promising next-generation energy storage devices, the lithium-metal battery has been extensively investigated. However, safety issues and undesired lithium dendrite growth hinder its development. The application of solid-state electrolytes has attracted increasing attention as they can solve safety issues and show great potential to inhibit the growth of lithium dendrites. Polyethylene oxide (PEO)-based electrolytes are very promising due to their enhanced safety and excellent flexibility. However, they suffer from low ionic conductivity at room temperature and cannot effectively inhibit lithium dendrites at high temperatures due to the intrinsic semicrystalline properties and poor mechanical strength. In this work, a novel coral-like $ Li_{6.25} %$ Al_{0.25} %$ La_{3} %$ Zr_{2} $-$ O_{12} $ (C-LALZO) is synthesized to serve as an active ceramic filler in PEO. The PEO with LALZO coral (PLC) exhibits increased ionic conductivity and mechanical strength, which leads to uniform deposition/stripping of lithium metal. The Li symmetric cells with PLC do not cause a short circuit after cycling for 1500 h at 60°C. The assembled $ LiFePO_{4} $/PLC/Li batteries display excellent cycling stability at both 60 and 50°C. This work reveals that the electrochemical properties of the composite electrolyte can be effectively improved by tuning the microstructure of the filler, such as the C-LALZO architecture. coral-like garnet (dpeaa)DE-He213 composite solid-state electrolyte (dpeaa)DE-He213 all-solid-state battery (dpeaa)DE-He213 Hou, Guangmei aut Sun, Qing aut Chen, Qiong aut Li, Deping aut Li, Jianwei aut Zeng, Zhen aut Li, Kaikai aut Yuan, Qunhui aut Wang, Jiajun aut Ci, Lijie aut Enthalten in Science China materials Beijing : Science China Press, 2014 65(2021), 2 vom: 26. Aug., Seite 364-372 (DE-627)815914733 (DE-600)2806677-7 2199-4501 nnns volume:65 year:2021 number:2 day:26 month:08 pages:364-372 https://dx.doi.org/10.1007/s40843-021-1748-7 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 65 2021 2 26 08 364-372 |
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Enthalten in Science China materials 65(2021), 2 vom: 26. Aug., Seite 364-372 volume:65 year:2021 number:2 day:26 month:08 pages:364-372 |
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Enthalten in Science China materials 65(2021), 2 vom: 26. Aug., Seite 364-372 volume:65 year:2021 number:2 day:26 month:08 pages:364-372 |
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Cheng, Jun @@aut@@ Hou, Guangmei @@aut@@ Sun, Qing @@aut@@ Chen, Qiong @@aut@@ Li, Deping @@aut@@ Li, Jianwei @@aut@@ Zeng, Zhen @@aut@@ Li, Kaikai @@aut@@ Yuan, Qunhui @@aut@@ Wang, Jiajun @@aut@@ Ci, Lijie @@aut@@ |
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However, safety issues and undesired lithium dendrite growth hinder its development. The application of solid-state electrolytes has attracted increasing attention as they can solve safety issues and show great potential to inhibit the growth of lithium dendrites. Polyethylene oxide (PEO)-based electrolytes are very promising due to their enhanced safety and excellent flexibility. However, they suffer from low ionic conductivity at room temperature and cannot effectively inhibit lithium dendrites at high temperatures due to the intrinsic semicrystalline properties and poor mechanical strength. In this work, a novel coral-like $ Li_{6.25} %$ Al_{0.25} %$ La_{3} %$ Zr_{2} $-$ O_{12} $ (C-LALZO) is synthesized to serve as an active ceramic filler in PEO. The PEO with LALZO coral (PLC) exhibits increased ionic conductivity and mechanical strength, which leads to uniform deposition/stripping of lithium metal. The Li symmetric cells with PLC do not cause a short circuit after cycling for 1500 h at 60°C. The assembled $ LiFePO_{4} $/PLC/Li batteries display excellent cycling stability at both 60 and 50°C. 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Cheng, Jun |
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Cheng, Jun misc coral-like garnet misc composite solid-state electrolyte misc all-solid-state battery A novel coral-like garnet for high-performance PEO-based all solid-state batteries |
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A novel coral-like garnet for high-performance PEO-based all solid-state batteries coral-like garnet (dpeaa)DE-He213 composite solid-state electrolyte (dpeaa)DE-He213 all-solid-state battery (dpeaa)DE-He213 |
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A novel coral-like garnet for high-performance PEO-based all solid-state batteries |
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Cheng, Jun Hou, Guangmei Sun, Qing Chen, Qiong Li, Deping Li, Jianwei Zeng, Zhen Li, Kaikai Yuan, Qunhui Wang, Jiajun Ci, Lijie |
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novel coral-like garnet for high-performance peo-based all solid-state batteries |
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A novel coral-like garnet for high-performance PEO-based all solid-state batteries |
| abstract |
Abstract As one of the most promising next-generation energy storage devices, the lithium-metal battery has been extensively investigated. However, safety issues and undesired lithium dendrite growth hinder its development. The application of solid-state electrolytes has attracted increasing attention as they can solve safety issues and show great potential to inhibit the growth of lithium dendrites. Polyethylene oxide (PEO)-based electrolytes are very promising due to their enhanced safety and excellent flexibility. However, they suffer from low ionic conductivity at room temperature and cannot effectively inhibit lithium dendrites at high temperatures due to the intrinsic semicrystalline properties and poor mechanical strength. In this work, a novel coral-like $ Li_{6.25} %$ Al_{0.25} %$ La_{3} %$ Zr_{2} $-$ O_{12} $ (C-LALZO) is synthesized to serve as an active ceramic filler in PEO. The PEO with LALZO coral (PLC) exhibits increased ionic conductivity and mechanical strength, which leads to uniform deposition/stripping of lithium metal. The Li symmetric cells with PLC do not cause a short circuit after cycling for 1500 h at 60°C. The assembled $ LiFePO_{4} $/PLC/Li batteries display excellent cycling stability at both 60 and 50°C. This work reveals that the electrochemical properties of the composite electrolyte can be effectively improved by tuning the microstructure of the filler, such as the C-LALZO architecture. © Science China Press and Springer-Verlag GmbH Germany, part of Springer Nature 2022 |
| abstractGer |
Abstract As one of the most promising next-generation energy storage devices, the lithium-metal battery has been extensively investigated. However, safety issues and undesired lithium dendrite growth hinder its development. The application of solid-state electrolytes has attracted increasing attention as they can solve safety issues and show great potential to inhibit the growth of lithium dendrites. Polyethylene oxide (PEO)-based electrolytes are very promising due to their enhanced safety and excellent flexibility. However, they suffer from low ionic conductivity at room temperature and cannot effectively inhibit lithium dendrites at high temperatures due to the intrinsic semicrystalline properties and poor mechanical strength. In this work, a novel coral-like $ Li_{6.25} %$ Al_{0.25} %$ La_{3} %$ Zr_{2} $-$ O_{12} $ (C-LALZO) is synthesized to serve as an active ceramic filler in PEO. The PEO with LALZO coral (PLC) exhibits increased ionic conductivity and mechanical strength, which leads to uniform deposition/stripping of lithium metal. The Li symmetric cells with PLC do not cause a short circuit after cycling for 1500 h at 60°C. The assembled $ LiFePO_{4} $/PLC/Li batteries display excellent cycling stability at both 60 and 50°C. This work reveals that the electrochemical properties of the composite electrolyte can be effectively improved by tuning the microstructure of the filler, such as the C-LALZO architecture. © Science China Press and Springer-Verlag GmbH Germany, part of Springer Nature 2022 |
| abstract_unstemmed |
Abstract As one of the most promising next-generation energy storage devices, the lithium-metal battery has been extensively investigated. However, safety issues and undesired lithium dendrite growth hinder its development. The application of solid-state electrolytes has attracted increasing attention as they can solve safety issues and show great potential to inhibit the growth of lithium dendrites. Polyethylene oxide (PEO)-based electrolytes are very promising due to their enhanced safety and excellent flexibility. However, they suffer from low ionic conductivity at room temperature and cannot effectively inhibit lithium dendrites at high temperatures due to the intrinsic semicrystalline properties and poor mechanical strength. In this work, a novel coral-like $ Li_{6.25} %$ Al_{0.25} %$ La_{3} %$ Zr_{2} $-$ O_{12} $ (C-LALZO) is synthesized to serve as an active ceramic filler in PEO. The PEO with LALZO coral (PLC) exhibits increased ionic conductivity and mechanical strength, which leads to uniform deposition/stripping of lithium metal. The Li symmetric cells with PLC do not cause a short circuit after cycling for 1500 h at 60°C. The assembled $ LiFePO_{4} $/PLC/Li batteries display excellent cycling stability at both 60 and 50°C. This work reveals that the electrochemical properties of the composite electrolyte can be effectively improved by tuning the microstructure of the filler, such as the C-LALZO architecture. © Science China Press and Springer-Verlag GmbH Germany, part of Springer Nature 2022 |
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A novel coral-like garnet for high-performance PEO-based all solid-state batteries |
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https://dx.doi.org/10.1007/s40843-021-1748-7 |
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Hou, Guangmei Sun, Qing Chen, Qiong Li, Deping Li, Jianwei Zeng, Zhen Li, Kaikai Yuan, Qunhui Wang, Jiajun Ci, Lijie |
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Hou, Guangmei Sun, Qing Chen, Qiong Li, Deping Li, Jianwei Zeng, Zhen Li, Kaikai Yuan, Qunhui Wang, Jiajun Ci, Lijie |
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10.1007/s40843-021-1748-7 |
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2024-07-03T15:39:16.994Z |
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| score |
7.4001503 |