The cooperation effect of Ni and Pt in the hydrogenation of acetic acid
Abstract The catalytic hydrogenation of carboxylic acid to alcohols is one of the important strategies for the conversion of biomass. Herein, a series of Ni-doped PtSn catalysts were prepared, characterized and studied in the hydrogenation of acetic acid. The Ni dopant has a strong interaction with...
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Gespeichert in:
| Autor*in: |
Pan, Deng [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2021 |
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| Anmerkung: |
© Higher Education Press 2021 |
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| Übergeordnetes Werk: |
Enthalten in: Frontiers of chemical engineering in China - Beijing : Higher Education Press, 2007, 16(2021), 3 vom: 31. Aug., Seite 397-407 |
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| Übergeordnetes Werk: |
volume:16 ; year:2021 ; number:3 ; day:31 ; month:08 ; pages:397-407 |
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| DOI / URN: |
10.1007/s11705-021-2076-4 |
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| 520 | |a Abstract The catalytic hydrogenation of carboxylic acid to alcohols is one of the important strategies for the conversion of biomass. Herein, a series of Ni-doped PtSn catalysts were prepared, characterized and studied in the hydrogenation of acetic acid. The Ni dopant has a strong interaction with Pt, which promotes the hydrogen adsorption, providing an activated hydrogen-rich environment for the hydrogenation. Meanwhile, the presence of Ni also improves the Pt dispersion, giving more accessible active sites for hydrogen activation. The cooperation of Pt and Ni significantly promotes the catalytic activity of the hydrogenation of acetic acid to ethanol. As a result, the catalyst with 0.1% Ni exhibits the best reaction activity, and its space time yield is twice as that of the PtSn/$ SiO_{2} $ catalyst. It provides a meaningful instruction on the catalyst design for the carboxylic acid hydrogenation. | ||
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10.1007/s11705-021-2076-4 doi (DE-627)SPR050556118 (SPR)s11705-021-2076-4-e DE-627 ger DE-627 rakwb eng Pan, Deng verfasserin aut The cooperation effect of Ni and Pt in the hydrogenation of acetic acid 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Higher Education Press 2021 Abstract The catalytic hydrogenation of carboxylic acid to alcohols is one of the important strategies for the conversion of biomass. Herein, a series of Ni-doped PtSn catalysts were prepared, characterized and studied in the hydrogenation of acetic acid. The Ni dopant has a strong interaction with Pt, which promotes the hydrogen adsorption, providing an activated hydrogen-rich environment for the hydrogenation. Meanwhile, the presence of Ni also improves the Pt dispersion, giving more accessible active sites for hydrogen activation. The cooperation of Pt and Ni significantly promotes the catalytic activity of the hydrogenation of acetic acid to ethanol. As a result, the catalyst with 0.1% Ni exhibits the best reaction activity, and its space time yield is twice as that of the PtSn/$ SiO_{2} $ catalyst. It provides a meaningful instruction on the catalyst design for the carboxylic acid hydrogenation. acetic acid (dpeaa)DE-He213 ethanol (dpeaa)DE-He213 hydrogenation (dpeaa)DE-He213 Pt (dpeaa)DE-He213 Ni (dpeaa)DE-He213 cooperation effect (dpeaa)DE-He213 Zhou, Jiahua aut Peng, Bo aut Wang, Shengping aut Zhao, Yujun aut Ma, Xinbin aut Enthalten in Frontiers of chemical engineering in China Beijing : Higher Education Press, 2007 16(2021), 3 vom: 31. Aug., Seite 397-407 (DE-627)545787602 (DE-600)2388862-3 1673-7474 nnns volume:16 year:2021 number:3 day:31 month:08 pages:397-407 https://dx.doi.org/10.1007/s11705-021-2076-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 16 2021 3 31 08 397-407 |
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10.1007/s11705-021-2076-4 doi (DE-627)SPR050556118 (SPR)s11705-021-2076-4-e DE-627 ger DE-627 rakwb eng Pan, Deng verfasserin aut The cooperation effect of Ni and Pt in the hydrogenation of acetic acid 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Higher Education Press 2021 Abstract The catalytic hydrogenation of carboxylic acid to alcohols is one of the important strategies for the conversion of biomass. Herein, a series of Ni-doped PtSn catalysts were prepared, characterized and studied in the hydrogenation of acetic acid. The Ni dopant has a strong interaction with Pt, which promotes the hydrogen adsorption, providing an activated hydrogen-rich environment for the hydrogenation. Meanwhile, the presence of Ni also improves the Pt dispersion, giving more accessible active sites for hydrogen activation. The cooperation of Pt and Ni significantly promotes the catalytic activity of the hydrogenation of acetic acid to ethanol. As a result, the catalyst with 0.1% Ni exhibits the best reaction activity, and its space time yield is twice as that of the PtSn/$ SiO_{2} $ catalyst. It provides a meaningful instruction on the catalyst design for the carboxylic acid hydrogenation. acetic acid (dpeaa)DE-He213 ethanol (dpeaa)DE-He213 hydrogenation (dpeaa)DE-He213 Pt (dpeaa)DE-He213 Ni (dpeaa)DE-He213 cooperation effect (dpeaa)DE-He213 Zhou, Jiahua aut Peng, Bo aut Wang, Shengping aut Zhao, Yujun aut Ma, Xinbin aut Enthalten in Frontiers of chemical engineering in China Beijing : Higher Education Press, 2007 16(2021), 3 vom: 31. Aug., Seite 397-407 (DE-627)545787602 (DE-600)2388862-3 1673-7474 nnns volume:16 year:2021 number:3 day:31 month:08 pages:397-407 https://dx.doi.org/10.1007/s11705-021-2076-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 16 2021 3 31 08 397-407 |
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10.1007/s11705-021-2076-4 doi (DE-627)SPR050556118 (SPR)s11705-021-2076-4-e DE-627 ger DE-627 rakwb eng Pan, Deng verfasserin aut The cooperation effect of Ni and Pt in the hydrogenation of acetic acid 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Higher Education Press 2021 Abstract The catalytic hydrogenation of carboxylic acid to alcohols is one of the important strategies for the conversion of biomass. Herein, a series of Ni-doped PtSn catalysts were prepared, characterized and studied in the hydrogenation of acetic acid. The Ni dopant has a strong interaction with Pt, which promotes the hydrogen adsorption, providing an activated hydrogen-rich environment for the hydrogenation. Meanwhile, the presence of Ni also improves the Pt dispersion, giving more accessible active sites for hydrogen activation. The cooperation of Pt and Ni significantly promotes the catalytic activity of the hydrogenation of acetic acid to ethanol. As a result, the catalyst with 0.1% Ni exhibits the best reaction activity, and its space time yield is twice as that of the PtSn/$ SiO_{2} $ catalyst. It provides a meaningful instruction on the catalyst design for the carboxylic acid hydrogenation. acetic acid (dpeaa)DE-He213 ethanol (dpeaa)DE-He213 hydrogenation (dpeaa)DE-He213 Pt (dpeaa)DE-He213 Ni (dpeaa)DE-He213 cooperation effect (dpeaa)DE-He213 Zhou, Jiahua aut Peng, Bo aut Wang, Shengping aut Zhao, Yujun aut Ma, Xinbin aut Enthalten in Frontiers of chemical engineering in China Beijing : Higher Education Press, 2007 16(2021), 3 vom: 31. Aug., Seite 397-407 (DE-627)545787602 (DE-600)2388862-3 1673-7474 nnns volume:16 year:2021 number:3 day:31 month:08 pages:397-407 https://dx.doi.org/10.1007/s11705-021-2076-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 16 2021 3 31 08 397-407 |
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10.1007/s11705-021-2076-4 doi (DE-627)SPR050556118 (SPR)s11705-021-2076-4-e DE-627 ger DE-627 rakwb eng Pan, Deng verfasserin aut The cooperation effect of Ni and Pt in the hydrogenation of acetic acid 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Higher Education Press 2021 Abstract The catalytic hydrogenation of carboxylic acid to alcohols is one of the important strategies for the conversion of biomass. Herein, a series of Ni-doped PtSn catalysts were prepared, characterized and studied in the hydrogenation of acetic acid. The Ni dopant has a strong interaction with Pt, which promotes the hydrogen adsorption, providing an activated hydrogen-rich environment for the hydrogenation. Meanwhile, the presence of Ni also improves the Pt dispersion, giving more accessible active sites for hydrogen activation. The cooperation of Pt and Ni significantly promotes the catalytic activity of the hydrogenation of acetic acid to ethanol. As a result, the catalyst with 0.1% Ni exhibits the best reaction activity, and its space time yield is twice as that of the PtSn/$ SiO_{2} $ catalyst. It provides a meaningful instruction on the catalyst design for the carboxylic acid hydrogenation. acetic acid (dpeaa)DE-He213 ethanol (dpeaa)DE-He213 hydrogenation (dpeaa)DE-He213 Pt (dpeaa)DE-He213 Ni (dpeaa)DE-He213 cooperation effect (dpeaa)DE-He213 Zhou, Jiahua aut Peng, Bo aut Wang, Shengping aut Zhao, Yujun aut Ma, Xinbin aut Enthalten in Frontiers of chemical engineering in China Beijing : Higher Education Press, 2007 16(2021), 3 vom: 31. Aug., Seite 397-407 (DE-627)545787602 (DE-600)2388862-3 1673-7474 nnns volume:16 year:2021 number:3 day:31 month:08 pages:397-407 https://dx.doi.org/10.1007/s11705-021-2076-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 16 2021 3 31 08 397-407 |
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10.1007/s11705-021-2076-4 doi (DE-627)SPR050556118 (SPR)s11705-021-2076-4-e DE-627 ger DE-627 rakwb eng Pan, Deng verfasserin aut The cooperation effect of Ni and Pt in the hydrogenation of acetic acid 2021 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Higher Education Press 2021 Abstract The catalytic hydrogenation of carboxylic acid to alcohols is one of the important strategies for the conversion of biomass. Herein, a series of Ni-doped PtSn catalysts were prepared, characterized and studied in the hydrogenation of acetic acid. The Ni dopant has a strong interaction with Pt, which promotes the hydrogen adsorption, providing an activated hydrogen-rich environment for the hydrogenation. Meanwhile, the presence of Ni also improves the Pt dispersion, giving more accessible active sites for hydrogen activation. The cooperation of Pt and Ni significantly promotes the catalytic activity of the hydrogenation of acetic acid to ethanol. As a result, the catalyst with 0.1% Ni exhibits the best reaction activity, and its space time yield is twice as that of the PtSn/$ SiO_{2} $ catalyst. It provides a meaningful instruction on the catalyst design for the carboxylic acid hydrogenation. acetic acid (dpeaa)DE-He213 ethanol (dpeaa)DE-He213 hydrogenation (dpeaa)DE-He213 Pt (dpeaa)DE-He213 Ni (dpeaa)DE-He213 cooperation effect (dpeaa)DE-He213 Zhou, Jiahua aut Peng, Bo aut Wang, Shengping aut Zhao, Yujun aut Ma, Xinbin aut Enthalten in Frontiers of chemical engineering in China Beijing : Higher Education Press, 2007 16(2021), 3 vom: 31. Aug., Seite 397-407 (DE-627)545787602 (DE-600)2388862-3 1673-7474 nnns volume:16 year:2021 number:3 day:31 month:08 pages:397-407 https://dx.doi.org/10.1007/s11705-021-2076-4 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 16 2021 3 31 08 397-407 |
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The cooperation effect of Ni and Pt in the hydrogenation of acetic acid acetic acid (dpeaa)DE-He213 ethanol (dpeaa)DE-He213 hydrogenation (dpeaa)DE-He213 Pt (dpeaa)DE-He213 Ni (dpeaa)DE-He213 cooperation effect (dpeaa)DE-He213 |
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cooperation effect of ni and pt in the hydrogenation of acetic acid |
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The cooperation effect of Ni and Pt in the hydrogenation of acetic acid |
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Abstract The catalytic hydrogenation of carboxylic acid to alcohols is one of the important strategies for the conversion of biomass. Herein, a series of Ni-doped PtSn catalysts were prepared, characterized and studied in the hydrogenation of acetic acid. The Ni dopant has a strong interaction with Pt, which promotes the hydrogen adsorption, providing an activated hydrogen-rich environment for the hydrogenation. Meanwhile, the presence of Ni also improves the Pt dispersion, giving more accessible active sites for hydrogen activation. The cooperation of Pt and Ni significantly promotes the catalytic activity of the hydrogenation of acetic acid to ethanol. As a result, the catalyst with 0.1% Ni exhibits the best reaction activity, and its space time yield is twice as that of the PtSn/$ SiO_{2} $ catalyst. It provides a meaningful instruction on the catalyst design for the carboxylic acid hydrogenation. © Higher Education Press 2021 |
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Abstract The catalytic hydrogenation of carboxylic acid to alcohols is one of the important strategies for the conversion of biomass. Herein, a series of Ni-doped PtSn catalysts were prepared, characterized and studied in the hydrogenation of acetic acid. The Ni dopant has a strong interaction with Pt, which promotes the hydrogen adsorption, providing an activated hydrogen-rich environment for the hydrogenation. Meanwhile, the presence of Ni also improves the Pt dispersion, giving more accessible active sites for hydrogen activation. The cooperation of Pt and Ni significantly promotes the catalytic activity of the hydrogenation of acetic acid to ethanol. As a result, the catalyst with 0.1% Ni exhibits the best reaction activity, and its space time yield is twice as that of the PtSn/$ SiO_{2} $ catalyst. It provides a meaningful instruction on the catalyst design for the carboxylic acid hydrogenation. © Higher Education Press 2021 |
| abstract_unstemmed |
Abstract The catalytic hydrogenation of carboxylic acid to alcohols is one of the important strategies for the conversion of biomass. Herein, a series of Ni-doped PtSn catalysts were prepared, characterized and studied in the hydrogenation of acetic acid. The Ni dopant has a strong interaction with Pt, which promotes the hydrogen adsorption, providing an activated hydrogen-rich environment for the hydrogenation. Meanwhile, the presence of Ni also improves the Pt dispersion, giving more accessible active sites for hydrogen activation. The cooperation of Pt and Ni significantly promotes the catalytic activity of the hydrogenation of acetic acid to ethanol. As a result, the catalyst with 0.1% Ni exhibits the best reaction activity, and its space time yield is twice as that of the PtSn/$ SiO_{2} $ catalyst. It provides a meaningful instruction on the catalyst design for the carboxylic acid hydrogenation. © Higher Education Press 2021 |
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