Transforming bulk alkenes and alkynes into fine chemicals enabled by single-atom site catalysis
Abstract The addition and substitution reactions across a variety of alkenes and alkynes have been playing an important role in organic synthesis. In particular, catalyses enabled by homogeneous complexes as well as heterogenous nanomaterials have been much received attentions over decades. Along wi...
Ausführliche Beschreibung
Autor*in: |
Guo, Ping [verfasserIn] |
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E-Artikel |
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Sprache: |
Englisch |
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2022 |
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Anmerkung: |
© Tsinghua University Press 2022 |
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Übergeordnetes Werk: |
Enthalten in: Nano research - [S.l.] : Tsinghua Press, 2008, 15(2022), 9 vom: 28. Juni, Seite 7840-7860 |
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Übergeordnetes Werk: |
volume:15 ; year:2022 ; number:9 ; day:28 ; month:06 ; pages:7840-7860 |
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DOI / URN: |
10.1007/s12274-022-4495-z |
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SPR05093094X |
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520 | |a Abstract The addition and substitution reactions across a variety of alkenes and alkynes have been playing an important role in organic synthesis. In particular, catalyses enabled by homogeneous complexes as well as heterogenous nanomaterials have been much received attentions over decades. Along with these blooming progresses in these fields, single-atom site catalysts (SACs) exhibit outstanding performances in terms of reactivity and selectivity, thus providing a new powerful strategy to upgrade these bulk chemicals. Herein, we summarize the reactions of alkenes and alkynes enabled by SACs, in which catalytic hydrogenation, hydrosilylation, hydroboration, hydroformylation, and cross coupling have been included. Moreover, preparations and fine structures of the corresponding SACs have been described, therefore providing a better understanding and overview to address the origin of catalytic activity in the reported examples. | ||
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700 | 1 | |a Zhao, Jie |4 aut | |
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10.1007/s12274-022-4495-z doi (DE-627)SPR05093094X (SPR)s12274-022-4495-z-e DE-627 ger DE-627 rakwb eng Guo, Ping verfasserin aut Transforming bulk alkenes and alkynes into fine chemicals enabled by single-atom site catalysis 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press 2022 Abstract The addition and substitution reactions across a variety of alkenes and alkynes have been playing an important role in organic synthesis. In particular, catalyses enabled by homogeneous complexes as well as heterogenous nanomaterials have been much received attentions over decades. Along with these blooming progresses in these fields, single-atom site catalysts (SACs) exhibit outstanding performances in terms of reactivity and selectivity, thus providing a new powerful strategy to upgrade these bulk chemicals. Herein, we summarize the reactions of alkenes and alkynes enabled by SACs, in which catalytic hydrogenation, hydrosilylation, hydroboration, hydroformylation, and cross coupling have been included. Moreover, preparations and fine structures of the corresponding SACs have been described, therefore providing a better understanding and overview to address the origin of catalytic activity in the reported examples. single-atom site catalysts (SACs) (dpeaa)DE-He213 alkenes (dpeaa)DE-He213 alkynes (dpeaa)DE-He213 Liu, Hongyuan aut Zhao, Jie aut Enthalten in Nano research [S.l.] : Tsinghua Press, 2008 15(2022), 9 vom: 28. Juni, Seite 7840-7860 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:15 year:2022 number:9 day:28 month:06 pages:7840-7860 https://dx.doi.org/10.1007/s12274-022-4495-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 15 2022 9 28 06 7840-7860 |
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10.1007/s12274-022-4495-z doi (DE-627)SPR05093094X (SPR)s12274-022-4495-z-e DE-627 ger DE-627 rakwb eng Guo, Ping verfasserin aut Transforming bulk alkenes and alkynes into fine chemicals enabled by single-atom site catalysis 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press 2022 Abstract The addition and substitution reactions across a variety of alkenes and alkynes have been playing an important role in organic synthesis. In particular, catalyses enabled by homogeneous complexes as well as heterogenous nanomaterials have been much received attentions over decades. Along with these blooming progresses in these fields, single-atom site catalysts (SACs) exhibit outstanding performances in terms of reactivity and selectivity, thus providing a new powerful strategy to upgrade these bulk chemicals. Herein, we summarize the reactions of alkenes and alkynes enabled by SACs, in which catalytic hydrogenation, hydrosilylation, hydroboration, hydroformylation, and cross coupling have been included. Moreover, preparations and fine structures of the corresponding SACs have been described, therefore providing a better understanding and overview to address the origin of catalytic activity in the reported examples. single-atom site catalysts (SACs) (dpeaa)DE-He213 alkenes (dpeaa)DE-He213 alkynes (dpeaa)DE-He213 Liu, Hongyuan aut Zhao, Jie aut Enthalten in Nano research [S.l.] : Tsinghua Press, 2008 15(2022), 9 vom: 28. Juni, Seite 7840-7860 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:15 year:2022 number:9 day:28 month:06 pages:7840-7860 https://dx.doi.org/10.1007/s12274-022-4495-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 15 2022 9 28 06 7840-7860 |
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10.1007/s12274-022-4495-z doi (DE-627)SPR05093094X (SPR)s12274-022-4495-z-e DE-627 ger DE-627 rakwb eng Guo, Ping verfasserin aut Transforming bulk alkenes and alkynes into fine chemicals enabled by single-atom site catalysis 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press 2022 Abstract The addition and substitution reactions across a variety of alkenes and alkynes have been playing an important role in organic synthesis. In particular, catalyses enabled by homogeneous complexes as well as heterogenous nanomaterials have been much received attentions over decades. Along with these blooming progresses in these fields, single-atom site catalysts (SACs) exhibit outstanding performances in terms of reactivity and selectivity, thus providing a new powerful strategy to upgrade these bulk chemicals. Herein, we summarize the reactions of alkenes and alkynes enabled by SACs, in which catalytic hydrogenation, hydrosilylation, hydroboration, hydroformylation, and cross coupling have been included. Moreover, preparations and fine structures of the corresponding SACs have been described, therefore providing a better understanding and overview to address the origin of catalytic activity in the reported examples. single-atom site catalysts (SACs) (dpeaa)DE-He213 alkenes (dpeaa)DE-He213 alkynes (dpeaa)DE-He213 Liu, Hongyuan aut Zhao, Jie aut Enthalten in Nano research [S.l.] : Tsinghua Press, 2008 15(2022), 9 vom: 28. Juni, Seite 7840-7860 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:15 year:2022 number:9 day:28 month:06 pages:7840-7860 https://dx.doi.org/10.1007/s12274-022-4495-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 15 2022 9 28 06 7840-7860 |
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10.1007/s12274-022-4495-z doi (DE-627)SPR05093094X (SPR)s12274-022-4495-z-e DE-627 ger DE-627 rakwb eng Guo, Ping verfasserin aut Transforming bulk alkenes and alkynes into fine chemicals enabled by single-atom site catalysis 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press 2022 Abstract The addition and substitution reactions across a variety of alkenes and alkynes have been playing an important role in organic synthesis. In particular, catalyses enabled by homogeneous complexes as well as heterogenous nanomaterials have been much received attentions over decades. Along with these blooming progresses in these fields, single-atom site catalysts (SACs) exhibit outstanding performances in terms of reactivity and selectivity, thus providing a new powerful strategy to upgrade these bulk chemicals. Herein, we summarize the reactions of alkenes and alkynes enabled by SACs, in which catalytic hydrogenation, hydrosilylation, hydroboration, hydroformylation, and cross coupling have been included. Moreover, preparations and fine structures of the corresponding SACs have been described, therefore providing a better understanding and overview to address the origin of catalytic activity in the reported examples. single-atom site catalysts (SACs) (dpeaa)DE-He213 alkenes (dpeaa)DE-He213 alkynes (dpeaa)DE-He213 Liu, Hongyuan aut Zhao, Jie aut Enthalten in Nano research [S.l.] : Tsinghua Press, 2008 15(2022), 9 vom: 28. Juni, Seite 7840-7860 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:15 year:2022 number:9 day:28 month:06 pages:7840-7860 https://dx.doi.org/10.1007/s12274-022-4495-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 15 2022 9 28 06 7840-7860 |
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10.1007/s12274-022-4495-z doi (DE-627)SPR05093094X (SPR)s12274-022-4495-z-e DE-627 ger DE-627 rakwb eng Guo, Ping verfasserin aut Transforming bulk alkenes and alkynes into fine chemicals enabled by single-atom site catalysis 2022 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press 2022 Abstract The addition and substitution reactions across a variety of alkenes and alkynes have been playing an important role in organic synthesis. In particular, catalyses enabled by homogeneous complexes as well as heterogenous nanomaterials have been much received attentions over decades. Along with these blooming progresses in these fields, single-atom site catalysts (SACs) exhibit outstanding performances in terms of reactivity and selectivity, thus providing a new powerful strategy to upgrade these bulk chemicals. Herein, we summarize the reactions of alkenes and alkynes enabled by SACs, in which catalytic hydrogenation, hydrosilylation, hydroboration, hydroformylation, and cross coupling have been included. Moreover, preparations and fine structures of the corresponding SACs have been described, therefore providing a better understanding and overview to address the origin of catalytic activity in the reported examples. single-atom site catalysts (SACs) (dpeaa)DE-He213 alkenes (dpeaa)DE-He213 alkynes (dpeaa)DE-He213 Liu, Hongyuan aut Zhao, Jie aut Enthalten in Nano research [S.l.] : Tsinghua Press, 2008 15(2022), 9 vom: 28. Juni, Seite 7840-7860 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:15 year:2022 number:9 day:28 month:06 pages:7840-7860 https://dx.doi.org/10.1007/s12274-022-4495-z lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 15 2022 9 28 06 7840-7860 |
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Enthalten in Nano research 15(2022), 9 vom: 28. Juni, Seite 7840-7860 volume:15 year:2022 number:9 day:28 month:06 pages:7840-7860 |
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Enthalten in Nano research 15(2022), 9 vom: 28. Juni, Seite 7840-7860 volume:15 year:2022 number:9 day:28 month:06 pages:7840-7860 |
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Guo, Ping @@aut@@ Liu, Hongyuan @@aut@@ Zhao, Jie @@aut@@ |
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Guo, Ping misc single-atom site catalysts (SACs) misc alkenes misc alkynes Transforming bulk alkenes and alkynes into fine chemicals enabled by single-atom site catalysis |
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Transforming bulk alkenes and alkynes into fine chemicals enabled by single-atom site catalysis single-atom site catalysts (SACs) (dpeaa)DE-He213 alkenes (dpeaa)DE-He213 alkynes (dpeaa)DE-He213 |
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transforming bulk alkenes and alkynes into fine chemicals enabled by single-atom site catalysis |
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Transforming bulk alkenes and alkynes into fine chemicals enabled by single-atom site catalysis |
abstract |
Abstract The addition and substitution reactions across a variety of alkenes and alkynes have been playing an important role in organic synthesis. In particular, catalyses enabled by homogeneous complexes as well as heterogenous nanomaterials have been much received attentions over decades. Along with these blooming progresses in these fields, single-atom site catalysts (SACs) exhibit outstanding performances in terms of reactivity and selectivity, thus providing a new powerful strategy to upgrade these bulk chemicals. Herein, we summarize the reactions of alkenes and alkynes enabled by SACs, in which catalytic hydrogenation, hydrosilylation, hydroboration, hydroformylation, and cross coupling have been included. Moreover, preparations and fine structures of the corresponding SACs have been described, therefore providing a better understanding and overview to address the origin of catalytic activity in the reported examples. © Tsinghua University Press 2022 |
abstractGer |
Abstract The addition and substitution reactions across a variety of alkenes and alkynes have been playing an important role in organic synthesis. In particular, catalyses enabled by homogeneous complexes as well as heterogenous nanomaterials have been much received attentions over decades. Along with these blooming progresses in these fields, single-atom site catalysts (SACs) exhibit outstanding performances in terms of reactivity and selectivity, thus providing a new powerful strategy to upgrade these bulk chemicals. Herein, we summarize the reactions of alkenes and alkynes enabled by SACs, in which catalytic hydrogenation, hydrosilylation, hydroboration, hydroformylation, and cross coupling have been included. Moreover, preparations and fine structures of the corresponding SACs have been described, therefore providing a better understanding and overview to address the origin of catalytic activity in the reported examples. © Tsinghua University Press 2022 |
abstract_unstemmed |
Abstract The addition and substitution reactions across a variety of alkenes and alkynes have been playing an important role in organic synthesis. In particular, catalyses enabled by homogeneous complexes as well as heterogenous nanomaterials have been much received attentions over decades. Along with these blooming progresses in these fields, single-atom site catalysts (SACs) exhibit outstanding performances in terms of reactivity and selectivity, thus providing a new powerful strategy to upgrade these bulk chemicals. Herein, we summarize the reactions of alkenes and alkynes enabled by SACs, in which catalytic hydrogenation, hydrosilylation, hydroboration, hydroformylation, and cross coupling have been included. Moreover, preparations and fine structures of the corresponding SACs have been described, therefore providing a better understanding and overview to address the origin of catalytic activity in the reported examples. © Tsinghua University Press 2022 |
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Transforming bulk alkenes and alkynes into fine chemicals enabled by single-atom site catalysis |
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In particular, catalyses enabled by homogeneous complexes as well as heterogenous nanomaterials have been much received attentions over decades. Along with these blooming progresses in these fields, single-atom site catalysts (SACs) exhibit outstanding performances in terms of reactivity and selectivity, thus providing a new powerful strategy to upgrade these bulk chemicals. Herein, we summarize the reactions of alkenes and alkynes enabled by SACs, in which catalytic hydrogenation, hydrosilylation, hydroboration, hydroformylation, and cross coupling have been included. 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