A dual-switching spin-crossover framework with redox regulation and guest response

Abstract A dual-switching spin crossover metal-organic framework (SCO-MOF) [Fe(TPB){$ Pt^{II} $(CN)4}]·3iPrOH·$ 4H_{2} $O (TPB = 1,2,4,5-tetra(pyridin-4-yl)benzene) is developed via the combination of redox-active framework and tunable guests. The reversible structural transformation between [$ Pt^{...
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Autor*in:	Wang, Long-Fei [verfasserIn] Wu, Si-Guo Ruan, Ze-Yu Jian, Ai-Qi Cui, Wen Ni, Zhao-Ping Tong, Ming-Liang

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	spin crossover iron(II) post-synthetic modification redox host-guest interaction

Anmerkung:	© Science China Press 2023

Übergeordnetes Werk:	Enthalten in: Science in China - Asheville, NC : Science in China Press, 1995, 66(2023), 6 vom: 08. Mai, Seite 1744-1749
Übergeordnetes Werk:	volume:66 ; year:2023 ; number:6 ; day:08 ; month:05 ; pages:1744-1749

Links:	Volltext

DOI / URN:	10.1007/s11426-023-1573-8

Katalog-ID:	SPR051826127

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520			\|a Abstract A dual-switching spin crossover metal-organic framework (SCO-MOF) [Fe(TPB){$ Pt^{II} $(CN)4}]·3iPrOH·$ 4H_{2} $O (TPB = 1,2,4,5-tetra(pyridin-4-yl)benzene) is developed via the combination of redox-active framework and tunable guests. The reversible structural transformation between [$ Pt^{II} $(CN)4]2− and [$ Pt^{IV} %$ Br_{2} $(CN)4]2− moieties can be manipulated by redox post-synthetic modification (PSM), which results in the change of SCO behaviors from step-wise to one-step. The influences of the oxidative addition of bromides on the ligand field splitting of Fe side are further explored by density functional theory calculations. Besides, the modulation of hysteretic four-/three-step, one-step and four-step SCO behaviors can be achieved by tuning the composition of guest molecules. Therefore, the combination of electronic bistability, redox reaction and guest recognition in a homogeneous lattice provides a utility platform for designing multi-responsive molecule-based materials.
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allfields	10.1007/s11426-023-1573-8 doi (DE-627)SPR051826127 (SPR)s11426-023-1573-8-e DE-627 ger DE-627 rakwb eng Wang, Long-Fei verfasserin aut A dual-switching spin-crossover framework with redox regulation and guest response 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Science China Press 2023 Abstract A dual-switching spin crossover metal-organic framework (SCO-MOF) [Fe(TPB){$ Pt^{II} $(CN)4}]·3iPrOH·$ 4H_{2} $O (TPB = 1,2,4,5-tetra(pyridin-4-yl)benzene) is developed via the combination of redox-active framework and tunable guests. The reversible structural transformation between [$ Pt^{II} $(CN)4]2− and [$ Pt^{IV} %$ Br_{2} $(CN)4]2− moieties can be manipulated by redox post-synthetic modification (PSM), which results in the change of SCO behaviors from step-wise to one-step. The influences of the oxidative addition of bromides on the ligand field splitting of Fe side are further explored by density functional theory calculations. Besides, the modulation of hysteretic four-/three-step, one-step and four-step SCO behaviors can be achieved by tuning the composition of guest molecules. Therefore, the combination of electronic bistability, redox reaction and guest recognition in a homogeneous lattice provides a utility platform for designing multi-responsive molecule-based materials. spin crossover (dpeaa)DE-He213 iron(II) (dpeaa)DE-He213 post-synthetic modification (dpeaa)DE-He213 redox (dpeaa)DE-He213 host-guest interaction (dpeaa)DE-He213 Wu, Si-Guo aut Ruan, Ze-Yu aut Jian, Ai-Qi aut Cui, Wen aut Ni, Zhao-Ping aut Tong, Ming-Liang aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 66(2023), 6 vom: 08. Mai, Seite 1744-1749 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:66 year:2023 number:6 day:08 month:05 pages:1744-1749 https://dx.doi.org/10.1007/s11426-023-1573-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 66 2023 6 08 05 1744-1749
spelling	10.1007/s11426-023-1573-8 doi (DE-627)SPR051826127 (SPR)s11426-023-1573-8-e DE-627 ger DE-627 rakwb eng Wang, Long-Fei verfasserin aut A dual-switching spin-crossover framework with redox regulation and guest response 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Science China Press 2023 Abstract A dual-switching spin crossover metal-organic framework (SCO-MOF) [Fe(TPB){$ Pt^{II} $(CN)4}]·3iPrOH·$ 4H_{2} $O (TPB = 1,2,4,5-tetra(pyridin-4-yl)benzene) is developed via the combination of redox-active framework and tunable guests. The reversible structural transformation between [$ Pt^{II} $(CN)4]2− and [$ Pt^{IV} %$ Br_{2} $(CN)4]2− moieties can be manipulated by redox post-synthetic modification (PSM), which results in the change of SCO behaviors from step-wise to one-step. The influences of the oxidative addition of bromides on the ligand field splitting of Fe side are further explored by density functional theory calculations. Besides, the modulation of hysteretic four-/three-step, one-step and four-step SCO behaviors can be achieved by tuning the composition of guest molecules. Therefore, the combination of electronic bistability, redox reaction and guest recognition in a homogeneous lattice provides a utility platform for designing multi-responsive molecule-based materials. spin crossover (dpeaa)DE-He213 iron(II) (dpeaa)DE-He213 post-synthetic modification (dpeaa)DE-He213 redox (dpeaa)DE-He213 host-guest interaction (dpeaa)DE-He213 Wu, Si-Guo aut Ruan, Ze-Yu aut Jian, Ai-Qi aut Cui, Wen aut Ni, Zhao-Ping aut Tong, Ming-Liang aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 66(2023), 6 vom: 08. Mai, Seite 1744-1749 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:66 year:2023 number:6 day:08 month:05 pages:1744-1749 https://dx.doi.org/10.1007/s11426-023-1573-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 66 2023 6 08 05 1744-1749
allfields_unstemmed	10.1007/s11426-023-1573-8 doi (DE-627)SPR051826127 (SPR)s11426-023-1573-8-e DE-627 ger DE-627 rakwb eng Wang, Long-Fei verfasserin aut A dual-switching spin-crossover framework with redox regulation and guest response 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Science China Press 2023 Abstract A dual-switching spin crossover metal-organic framework (SCO-MOF) [Fe(TPB){$ Pt^{II} $(CN)4}]·3iPrOH·$ 4H_{2} $O (TPB = 1,2,4,5-tetra(pyridin-4-yl)benzene) is developed via the combination of redox-active framework and tunable guests. The reversible structural transformation between [$ Pt^{II} $(CN)4]2− and [$ Pt^{IV} %$ Br_{2} $(CN)4]2− moieties can be manipulated by redox post-synthetic modification (PSM), which results in the change of SCO behaviors from step-wise to one-step. The influences of the oxidative addition of bromides on the ligand field splitting of Fe side are further explored by density functional theory calculations. Besides, the modulation of hysteretic four-/three-step, one-step and four-step SCO behaviors can be achieved by tuning the composition of guest molecules. Therefore, the combination of electronic bistability, redox reaction and guest recognition in a homogeneous lattice provides a utility platform for designing multi-responsive molecule-based materials. spin crossover (dpeaa)DE-He213 iron(II) (dpeaa)DE-He213 post-synthetic modification (dpeaa)DE-He213 redox (dpeaa)DE-He213 host-guest interaction (dpeaa)DE-He213 Wu, Si-Guo aut Ruan, Ze-Yu aut Jian, Ai-Qi aut Cui, Wen aut Ni, Zhao-Ping aut Tong, Ming-Liang aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 66(2023), 6 vom: 08. Mai, Seite 1744-1749 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:66 year:2023 number:6 day:08 month:05 pages:1744-1749 https://dx.doi.org/10.1007/s11426-023-1573-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 66 2023 6 08 05 1744-1749
allfieldsGer	10.1007/s11426-023-1573-8 doi (DE-627)SPR051826127 (SPR)s11426-023-1573-8-e DE-627 ger DE-627 rakwb eng Wang, Long-Fei verfasserin aut A dual-switching spin-crossover framework with redox regulation and guest response 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Science China Press 2023 Abstract A dual-switching spin crossover metal-organic framework (SCO-MOF) [Fe(TPB){$ Pt^{II} $(CN)4}]·3iPrOH·$ 4H_{2} $O (TPB = 1,2,4,5-tetra(pyridin-4-yl)benzene) is developed via the combination of redox-active framework and tunable guests. The reversible structural transformation between [$ Pt^{II} $(CN)4]2− and [$ Pt^{IV} %$ Br_{2} $(CN)4]2− moieties can be manipulated by redox post-synthetic modification (PSM), which results in the change of SCO behaviors from step-wise to one-step. The influences of the oxidative addition of bromides on the ligand field splitting of Fe side are further explored by density functional theory calculations. Besides, the modulation of hysteretic four-/three-step, one-step and four-step SCO behaviors can be achieved by tuning the composition of guest molecules. Therefore, the combination of electronic bistability, redox reaction and guest recognition in a homogeneous lattice provides a utility platform for designing multi-responsive molecule-based materials. spin crossover (dpeaa)DE-He213 iron(II) (dpeaa)DE-He213 post-synthetic modification (dpeaa)DE-He213 redox (dpeaa)DE-He213 host-guest interaction (dpeaa)DE-He213 Wu, Si-Guo aut Ruan, Ze-Yu aut Jian, Ai-Qi aut Cui, Wen aut Ni, Zhao-Ping aut Tong, Ming-Liang aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 66(2023), 6 vom: 08. Mai, Seite 1744-1749 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:66 year:2023 number:6 day:08 month:05 pages:1744-1749 https://dx.doi.org/10.1007/s11426-023-1573-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 66 2023 6 08 05 1744-1749
allfieldsSound	10.1007/s11426-023-1573-8 doi (DE-627)SPR051826127 (SPR)s11426-023-1573-8-e DE-627 ger DE-627 rakwb eng Wang, Long-Fei verfasserin aut A dual-switching spin-crossover framework with redox regulation and guest response 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Science China Press 2023 Abstract A dual-switching spin crossover metal-organic framework (SCO-MOF) [Fe(TPB){$ Pt^{II} $(CN)4}]·3iPrOH·$ 4H_{2} $O (TPB = 1,2,4,5-tetra(pyridin-4-yl)benzene) is developed via the combination of redox-active framework and tunable guests. The reversible structural transformation between [$ Pt^{II} $(CN)4]2− and [$ Pt^{IV} %$ Br_{2} $(CN)4]2− moieties can be manipulated by redox post-synthetic modification (PSM), which results in the change of SCO behaviors from step-wise to one-step. The influences of the oxidative addition of bromides on the ligand field splitting of Fe side are further explored by density functional theory calculations. Besides, the modulation of hysteretic four-/three-step, one-step and four-step SCO behaviors can be achieved by tuning the composition of guest molecules. Therefore, the combination of electronic bistability, redox reaction and guest recognition in a homogeneous lattice provides a utility platform for designing multi-responsive molecule-based materials. spin crossover (dpeaa)DE-He213 iron(II) (dpeaa)DE-He213 post-synthetic modification (dpeaa)DE-He213 redox (dpeaa)DE-He213 host-guest interaction (dpeaa)DE-He213 Wu, Si-Guo aut Ruan, Ze-Yu aut Jian, Ai-Qi aut Cui, Wen aut Ni, Zhao-Ping aut Tong, Ming-Liang aut Enthalten in Science in China Asheville, NC : Science in China Press, 1995 66(2023), 6 vom: 08. Mai, Seite 1744-1749 (DE-627)327310405 (DE-600)2043454-6 1862-2771 nnns volume:66 year:2023 number:6 day:08 month:05 pages:1744-1749 https://dx.doi.org/10.1007/s11426-023-1573-8 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_152 GBV_ILN_161 GBV_ILN_171 GBV_ILN_187 GBV_ILN_224 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_702 AR 66 2023 6 08 05 1744-1749
language	English
source	Enthalten in Science in China 66(2023), 6 vom: 08. Mai, Seite 1744-1749 volume:66 year:2023 number:6 day:08 month:05 pages:1744-1749
sourceStr	Enthalten in Science in China 66(2023), 6 vom: 08. Mai, Seite 1744-1749 volume:66 year:2023 number:6 day:08 month:05 pages:1744-1749
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	spin crossover iron(II) post-synthetic modification redox host-guest interaction
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container_title	Science in China
authorswithroles_txt_mv	Wang, Long-Fei @@aut@@ Wu, Si-Guo @@aut@@ Ruan, Ze-Yu @@aut@@ Jian, Ai-Qi @@aut@@ Cui, Wen @@aut@@ Ni, Zhao-Ping @@aut@@ Tong, Ming-Liang @@aut@@
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author	Wang, Long-Fei
spellingShingle	Wang, Long-Fei misc spin crossover misc iron(II) misc post-synthetic modification misc redox misc host-guest interaction A dual-switching spin-crossover framework with redox regulation and guest response
authorStr	Wang, Long-Fei
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topic_title	A dual-switching spin-crossover framework with redox regulation and guest response spin crossover (dpeaa)DE-He213 iron(II) (dpeaa)DE-He213 post-synthetic modification (dpeaa)DE-He213 redox (dpeaa)DE-He213 host-guest interaction (dpeaa)DE-He213
topic	misc spin crossover misc iron(II) misc post-synthetic modification misc redox misc host-guest interaction
topic_unstemmed	misc spin crossover misc iron(II) misc post-synthetic modification misc redox misc host-guest interaction
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title	A dual-switching spin-crossover framework with redox regulation and guest response
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title_full	A dual-switching spin-crossover framework with redox regulation and guest response
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author_browse	Wang, Long-Fei Wu, Si-Guo Ruan, Ze-Yu Jian, Ai-Qi Cui, Wen Ni, Zhao-Ping Tong, Ming-Liang
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doi_str_mv	10.1007/s11426-023-1573-8
title_sort	dual-switching spin-crossover framework with redox regulation and guest response
title_auth	A dual-switching spin-crossover framework with redox regulation and guest response
abstract	Abstract A dual-switching spin crossover metal-organic framework (SCO-MOF) [Fe(TPB){$ Pt^{II} $(CN)4}]·3iPrOH·$ 4H_{2} $O (TPB = 1,2,4,5-tetra(pyridin-4-yl)benzene) is developed via the combination of redox-active framework and tunable guests. The reversible structural transformation between [$ Pt^{II} $(CN)4]2− and [$ Pt^{IV} %$ Br_{2} $(CN)4]2− moieties can be manipulated by redox post-synthetic modification (PSM), which results in the change of SCO behaviors from step-wise to one-step. The influences of the oxidative addition of bromides on the ligand field splitting of Fe side are further explored by density functional theory calculations. Besides, the modulation of hysteretic four-/three-step, one-step and four-step SCO behaviors can be achieved by tuning the composition of guest molecules. Therefore, the combination of electronic bistability, redox reaction and guest recognition in a homogeneous lattice provides a utility platform for designing multi-responsive molecule-based materials. © Science China Press 2023
abstractGer	Abstract A dual-switching spin crossover metal-organic framework (SCO-MOF) [Fe(TPB){$ Pt^{II} $(CN)4}]·3iPrOH·$ 4H_{2} $O (TPB = 1,2,4,5-tetra(pyridin-4-yl)benzene) is developed via the combination of redox-active framework and tunable guests. The reversible structural transformation between [$ Pt^{II} $(CN)4]2− and [$ Pt^{IV} %$ Br_{2} $(CN)4]2− moieties can be manipulated by redox post-synthetic modification (PSM), which results in the change of SCO behaviors from step-wise to one-step. The influences of the oxidative addition of bromides on the ligand field splitting of Fe side are further explored by density functional theory calculations. Besides, the modulation of hysteretic four-/three-step, one-step and four-step SCO behaviors can be achieved by tuning the composition of guest molecules. Therefore, the combination of electronic bistability, redox reaction and guest recognition in a homogeneous lattice provides a utility platform for designing multi-responsive molecule-based materials. © Science China Press 2023
abstract_unstemmed	Abstract A dual-switching spin crossover metal-organic framework (SCO-MOF) [Fe(TPB){$ Pt^{II} $(CN)4}]·3iPrOH·$ 4H_{2} $O (TPB = 1,2,4,5-tetra(pyridin-4-yl)benzene) is developed via the combination of redox-active framework and tunable guests. The reversible structural transformation between [$ Pt^{II} $(CN)4]2− and [$ Pt^{IV} %$ Br_{2} $(CN)4]2− moieties can be manipulated by redox post-synthetic modification (PSM), which results in the change of SCO behaviors from step-wise to one-step. The influences of the oxidative addition of bromides on the ligand field splitting of Fe side are further explored by density functional theory calculations. Besides, the modulation of hysteretic four-/three-step, one-step and four-step SCO behaviors can be achieved by tuning the composition of guest molecules. Therefore, the combination of electronic bistability, redox reaction and guest recognition in a homogeneous lattice provides a utility platform for designing multi-responsive molecule-based materials. © Science China Press 2023
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title_short	A dual-switching spin-crossover framework with redox regulation and guest response
url	https://dx.doi.org/10.1007/s11426-023-1573-8
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author2	Wu, Si-Guo Ruan, Ze-Yu Jian, Ai-Qi Cui, Wen Ni, Zhao-Ping Tong, Ming-Liang
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The reversible structural transformation between [$ Pt^{II} $(CN)4]2− and [$ Pt^{IV} %$ Br_{2} $(CN)4]2− moieties can be manipulated by redox post-synthetic modification (PSM), which results in the change of SCO behaviors from step-wise to one-step. The influences of the oxidative addition of bromides on the ligand field splitting of Fe side are further explored by density functional theory calculations. Besides, the modulation of hysteretic four-/three-step, one-step and four-step SCO behaviors can be achieved by tuning the composition of guest molecules. 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A dual-switching spin-crossover framework with redox regulation and guest response

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