Development of low-cost nitrogen- and boron-doped carbon black cathode catalysts for the improvement of hydrogen-bromine flow battery cathode kinetics
Abstract In this study, carbon blacks, containing nitrogen and boron, are used as cathode catalysts first time in a hydrogen-bromine redox flow cell. Nitrogen and boron doping has been applied to carbon blacks to improve the limited properties of the Vulcan XC72 (VXC). Here, we have examined the eff...
Ausführliche Beschreibung
Gespeichert in:
| Autor*in: |
Duman, Büşranur [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2023 |
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| Anmerkung: |
© The Author(s), under exclusive licence to Springer Nature B.V. 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
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| Übergeordnetes Werk: |
Enthalten in: Journal of applied electrochemistry - Dordrecht [u.a.] : Springer Science + Business Media B.V, 1971, 53(2023), 7 vom: 15. Feb., Seite 1421-1431 |
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| Übergeordnetes Werk: |
volume:53 ; year:2023 ; number:7 ; day:15 ; month:02 ; pages:1421-1431 |
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| DOI / URN: |
10.1007/s10800-023-01864-5 |
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SPR051907240 |
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| 520 | |a Abstract In this study, carbon blacks, containing nitrogen and boron, are used as cathode catalysts first time in a hydrogen-bromine redox flow cell. Nitrogen and boron doping has been applied to carbon blacks to improve the limited properties of the Vulcan XC72 (VXC). Here, we have examined the effect of nitrogen-/boron-doped Vulcan XC72 carbon black on hydrogen-bromine flow cell performance. Nitrogen gas and boric acid are used as nitrogen and boron sources in the post-doping process, respectively. XRD, SEM, XPS, Raman spectroscopy, and $ N_{2} $ adsorption analyses are used to characterize the structures of cathode catalysts. The electrochemical characterization of the catalysts has been carried out with the cyclic voltammetry technique using the conventional three-electrode system connected to a potentiostat. We have addressed the effect of nitrogen and boron doping into the carbon black onto the flow battery performance by comparing their polarization and power curves. The maximum power densities with the VXC, N-VXC, and B-VXC cathode catalysts have been measured at 0.75 V as 360, 390, and 430 mW $ cm^{−2} $, respectively. Graphic Abstract | ||
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| 650 | 4 | |a Hydrogen-bromine flow battery |7 (dpeaa)DE-He213 | |
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10.1007/s10800-023-01864-5 doi (DE-627)SPR051907240 (SPR)s10800-023-01864-5-e DE-627 ger DE-627 rakwb eng Duman, Büşranur verfasserin (orcid)0000-0001-7761-1510 aut Development of low-cost nitrogen- and boron-doped carbon black cathode catalysts for the improvement of hydrogen-bromine flow battery cathode kinetics 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature B.V. 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Abstract In this study, carbon blacks, containing nitrogen and boron, are used as cathode catalysts first time in a hydrogen-bromine redox flow cell. Nitrogen and boron doping has been applied to carbon blacks to improve the limited properties of the Vulcan XC72 (VXC). Here, we have examined the effect of nitrogen-/boron-doped Vulcan XC72 carbon black on hydrogen-bromine flow cell performance. Nitrogen gas and boric acid are used as nitrogen and boron sources in the post-doping process, respectively. XRD, SEM, XPS, Raman spectroscopy, and $ N_{2} $ adsorption analyses are used to characterize the structures of cathode catalysts. The electrochemical characterization of the catalysts has been carried out with the cyclic voltammetry technique using the conventional three-electrode system connected to a potentiostat. We have addressed the effect of nitrogen and boron doping into the carbon black onto the flow battery performance by comparing their polarization and power curves. The maximum power densities with the VXC, N-VXC, and B-VXC cathode catalysts have been measured at 0.75 V as 360, 390, and 430 mW $ cm^{−2} $, respectively. Graphic Abstract N-doping (dpeaa)DE-He213 B-doping (dpeaa)DE-He213 Hydrogen-bromine flow battery (dpeaa)DE-He213 Cathode catalyst (dpeaa)DE-He213 Fıçıcılar, Berker (orcid)0000-0003-3882-1691 aut Enthalten in Journal of applied electrochemistry Dordrecht [u.a.] : Springer Science + Business Media B.V, 1971 53(2023), 7 vom: 15. Feb., Seite 1421-1431 (DE-627)302466037 (DE-600)1491094-9 1572-8838 nnns volume:53 year:2023 number:7 day:15 month:02 pages:1421-1431 https://dx.doi.org/10.1007/s10800-023-01864-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 53 2023 7 15 02 1421-1431 |
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10.1007/s10800-023-01864-5 doi (DE-627)SPR051907240 (SPR)s10800-023-01864-5-e DE-627 ger DE-627 rakwb eng Duman, Büşranur verfasserin (orcid)0000-0001-7761-1510 aut Development of low-cost nitrogen- and boron-doped carbon black cathode catalysts for the improvement of hydrogen-bromine flow battery cathode kinetics 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature B.V. 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Abstract In this study, carbon blacks, containing nitrogen and boron, are used as cathode catalysts first time in a hydrogen-bromine redox flow cell. Nitrogen and boron doping has been applied to carbon blacks to improve the limited properties of the Vulcan XC72 (VXC). Here, we have examined the effect of nitrogen-/boron-doped Vulcan XC72 carbon black on hydrogen-bromine flow cell performance. Nitrogen gas and boric acid are used as nitrogen and boron sources in the post-doping process, respectively. XRD, SEM, XPS, Raman spectroscopy, and $ N_{2} $ adsorption analyses are used to characterize the structures of cathode catalysts. The electrochemical characterization of the catalysts has been carried out with the cyclic voltammetry technique using the conventional three-electrode system connected to a potentiostat. We have addressed the effect of nitrogen and boron doping into the carbon black onto the flow battery performance by comparing their polarization and power curves. The maximum power densities with the VXC, N-VXC, and B-VXC cathode catalysts have been measured at 0.75 V as 360, 390, and 430 mW $ cm^{−2} $, respectively. Graphic Abstract N-doping (dpeaa)DE-He213 B-doping (dpeaa)DE-He213 Hydrogen-bromine flow battery (dpeaa)DE-He213 Cathode catalyst (dpeaa)DE-He213 Fıçıcılar, Berker (orcid)0000-0003-3882-1691 aut Enthalten in Journal of applied electrochemistry Dordrecht [u.a.] : Springer Science + Business Media B.V, 1971 53(2023), 7 vom: 15. Feb., Seite 1421-1431 (DE-627)302466037 (DE-600)1491094-9 1572-8838 nnns volume:53 year:2023 number:7 day:15 month:02 pages:1421-1431 https://dx.doi.org/10.1007/s10800-023-01864-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 53 2023 7 15 02 1421-1431 |
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10.1007/s10800-023-01864-5 doi (DE-627)SPR051907240 (SPR)s10800-023-01864-5-e DE-627 ger DE-627 rakwb eng Duman, Büşranur verfasserin (orcid)0000-0001-7761-1510 aut Development of low-cost nitrogen- and boron-doped carbon black cathode catalysts for the improvement of hydrogen-bromine flow battery cathode kinetics 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature B.V. 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Abstract In this study, carbon blacks, containing nitrogen and boron, are used as cathode catalysts first time in a hydrogen-bromine redox flow cell. Nitrogen and boron doping has been applied to carbon blacks to improve the limited properties of the Vulcan XC72 (VXC). Here, we have examined the effect of nitrogen-/boron-doped Vulcan XC72 carbon black on hydrogen-bromine flow cell performance. Nitrogen gas and boric acid are used as nitrogen and boron sources in the post-doping process, respectively. XRD, SEM, XPS, Raman spectroscopy, and $ N_{2} $ adsorption analyses are used to characterize the structures of cathode catalysts. The electrochemical characterization of the catalysts has been carried out with the cyclic voltammetry technique using the conventional three-electrode system connected to a potentiostat. We have addressed the effect of nitrogen and boron doping into the carbon black onto the flow battery performance by comparing their polarization and power curves. The maximum power densities with the VXC, N-VXC, and B-VXC cathode catalysts have been measured at 0.75 V as 360, 390, and 430 mW $ cm^{−2} $, respectively. Graphic Abstract N-doping (dpeaa)DE-He213 B-doping (dpeaa)DE-He213 Hydrogen-bromine flow battery (dpeaa)DE-He213 Cathode catalyst (dpeaa)DE-He213 Fıçıcılar, Berker (orcid)0000-0003-3882-1691 aut Enthalten in Journal of applied electrochemistry Dordrecht [u.a.] : Springer Science + Business Media B.V, 1971 53(2023), 7 vom: 15. Feb., Seite 1421-1431 (DE-627)302466037 (DE-600)1491094-9 1572-8838 nnns volume:53 year:2023 number:7 day:15 month:02 pages:1421-1431 https://dx.doi.org/10.1007/s10800-023-01864-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 53 2023 7 15 02 1421-1431 |
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10.1007/s10800-023-01864-5 doi (DE-627)SPR051907240 (SPR)s10800-023-01864-5-e DE-627 ger DE-627 rakwb eng Duman, Büşranur verfasserin (orcid)0000-0001-7761-1510 aut Development of low-cost nitrogen- and boron-doped carbon black cathode catalysts for the improvement of hydrogen-bromine flow battery cathode kinetics 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature B.V. 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Abstract In this study, carbon blacks, containing nitrogen and boron, are used as cathode catalysts first time in a hydrogen-bromine redox flow cell. Nitrogen and boron doping has been applied to carbon blacks to improve the limited properties of the Vulcan XC72 (VXC). Here, we have examined the effect of nitrogen-/boron-doped Vulcan XC72 carbon black on hydrogen-bromine flow cell performance. Nitrogen gas and boric acid are used as nitrogen and boron sources in the post-doping process, respectively. XRD, SEM, XPS, Raman spectroscopy, and $ N_{2} $ adsorption analyses are used to characterize the structures of cathode catalysts. The electrochemical characterization of the catalysts has been carried out with the cyclic voltammetry technique using the conventional three-electrode system connected to a potentiostat. We have addressed the effect of nitrogen and boron doping into the carbon black onto the flow battery performance by comparing their polarization and power curves. The maximum power densities with the VXC, N-VXC, and B-VXC cathode catalysts have been measured at 0.75 V as 360, 390, and 430 mW $ cm^{−2} $, respectively. Graphic Abstract N-doping (dpeaa)DE-He213 B-doping (dpeaa)DE-He213 Hydrogen-bromine flow battery (dpeaa)DE-He213 Cathode catalyst (dpeaa)DE-He213 Fıçıcılar, Berker (orcid)0000-0003-3882-1691 aut Enthalten in Journal of applied electrochemistry Dordrecht [u.a.] : Springer Science + Business Media B.V, 1971 53(2023), 7 vom: 15. Feb., Seite 1421-1431 (DE-627)302466037 (DE-600)1491094-9 1572-8838 nnns volume:53 year:2023 number:7 day:15 month:02 pages:1421-1431 https://dx.doi.org/10.1007/s10800-023-01864-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 53 2023 7 15 02 1421-1431 |
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10.1007/s10800-023-01864-5 doi (DE-627)SPR051907240 (SPR)s10800-023-01864-5-e DE-627 ger DE-627 rakwb eng Duman, Büşranur verfasserin (orcid)0000-0001-7761-1510 aut Development of low-cost nitrogen- and boron-doped carbon black cathode catalysts for the improvement of hydrogen-bromine flow battery cathode kinetics 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s), under exclusive licence to Springer Nature B.V. 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. Abstract In this study, carbon blacks, containing nitrogen and boron, are used as cathode catalysts first time in a hydrogen-bromine redox flow cell. Nitrogen and boron doping has been applied to carbon blacks to improve the limited properties of the Vulcan XC72 (VXC). Here, we have examined the effect of nitrogen-/boron-doped Vulcan XC72 carbon black on hydrogen-bromine flow cell performance. Nitrogen gas and boric acid are used as nitrogen and boron sources in the post-doping process, respectively. XRD, SEM, XPS, Raman spectroscopy, and $ N_{2} $ adsorption analyses are used to characterize the structures of cathode catalysts. The electrochemical characterization of the catalysts has been carried out with the cyclic voltammetry technique using the conventional three-electrode system connected to a potentiostat. We have addressed the effect of nitrogen and boron doping into the carbon black onto the flow battery performance by comparing their polarization and power curves. The maximum power densities with the VXC, N-VXC, and B-VXC cathode catalysts have been measured at 0.75 V as 360, 390, and 430 mW $ cm^{−2} $, respectively. Graphic Abstract N-doping (dpeaa)DE-He213 B-doping (dpeaa)DE-He213 Hydrogen-bromine flow battery (dpeaa)DE-He213 Cathode catalyst (dpeaa)DE-He213 Fıçıcılar, Berker (orcid)0000-0003-3882-1691 aut Enthalten in Journal of applied electrochemistry Dordrecht [u.a.] : Springer Science + Business Media B.V, 1971 53(2023), 7 vom: 15. Feb., Seite 1421-1431 (DE-627)302466037 (DE-600)1491094-9 1572-8838 nnns volume:53 year:2023 number:7 day:15 month:02 pages:1421-1431 https://dx.doi.org/10.1007/s10800-023-01864-5 lizenzpflichtig Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 53 2023 7 15 02 1421-1431 |
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Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Abstract In this study, carbon blacks, containing nitrogen and boron, are used as cathode catalysts first time in a hydrogen-bromine redox flow cell. Nitrogen and boron doping has been applied to carbon blacks to improve the limited properties of the Vulcan XC72 (VXC). Here, we have examined the effect of nitrogen-/boron-doped Vulcan XC72 carbon black on hydrogen-bromine flow cell performance. Nitrogen gas and boric acid are used as nitrogen and boron sources in the post-doping process, respectively. XRD, SEM, XPS, Raman spectroscopy, and $ N_{2} $ adsorption analyses are used to characterize the structures of cathode catalysts. The electrochemical characterization of the catalysts has been carried out with the cyclic voltammetry technique using the conventional three-electrode system connected to a potentiostat. We have addressed the effect of nitrogen and boron doping into the carbon black onto the flow battery performance by comparing their polarization and power curves. The maximum power densities with the VXC, N-VXC, and B-VXC cathode catalysts have been measured at 0.75 V as 360, 390, and 430 mW $ cm^{−2} $, respectively. 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Duman, Büşranur |
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Duman, Büşranur misc N-doping misc B-doping misc Hydrogen-bromine flow battery misc Cathode catalyst Development of low-cost nitrogen- and boron-doped carbon black cathode catalysts for the improvement of hydrogen-bromine flow battery cathode kinetics |
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Development of low-cost nitrogen- and boron-doped carbon black cathode catalysts for the improvement of hydrogen-bromine flow battery cathode kinetics N-doping (dpeaa)DE-He213 B-doping (dpeaa)DE-He213 Hydrogen-bromine flow battery (dpeaa)DE-He213 Cathode catalyst (dpeaa)DE-He213 |
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development of low-cost nitrogen- and boron-doped carbon black cathode catalysts for the improvement of hydrogen-bromine flow battery cathode kinetics |
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Development of low-cost nitrogen- and boron-doped carbon black cathode catalysts for the improvement of hydrogen-bromine flow battery cathode kinetics |
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Abstract In this study, carbon blacks, containing nitrogen and boron, are used as cathode catalysts first time in a hydrogen-bromine redox flow cell. Nitrogen and boron doping has been applied to carbon blacks to improve the limited properties of the Vulcan XC72 (VXC). Here, we have examined the effect of nitrogen-/boron-doped Vulcan XC72 carbon black on hydrogen-bromine flow cell performance. Nitrogen gas and boric acid are used as nitrogen and boron sources in the post-doping process, respectively. XRD, SEM, XPS, Raman spectroscopy, and $ N_{2} $ adsorption analyses are used to characterize the structures of cathode catalysts. The electrochemical characterization of the catalysts has been carried out with the cyclic voltammetry technique using the conventional three-electrode system connected to a potentiostat. We have addressed the effect of nitrogen and boron doping into the carbon black onto the flow battery performance by comparing their polarization and power curves. The maximum power densities with the VXC, N-VXC, and B-VXC cathode catalysts have been measured at 0.75 V as 360, 390, and 430 mW $ cm^{−2} $, respectively. Graphic Abstract © The Author(s), under exclusive licence to Springer Nature B.V. 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
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Abstract In this study, carbon blacks, containing nitrogen and boron, are used as cathode catalysts first time in a hydrogen-bromine redox flow cell. Nitrogen and boron doping has been applied to carbon blacks to improve the limited properties of the Vulcan XC72 (VXC). Here, we have examined the effect of nitrogen-/boron-doped Vulcan XC72 carbon black on hydrogen-bromine flow cell performance. Nitrogen gas and boric acid are used as nitrogen and boron sources in the post-doping process, respectively. XRD, SEM, XPS, Raman spectroscopy, and $ N_{2} $ adsorption analyses are used to characterize the structures of cathode catalysts. The electrochemical characterization of the catalysts has been carried out with the cyclic voltammetry technique using the conventional three-electrode system connected to a potentiostat. We have addressed the effect of nitrogen and boron doping into the carbon black onto the flow battery performance by comparing their polarization and power curves. The maximum power densities with the VXC, N-VXC, and B-VXC cathode catalysts have been measured at 0.75 V as 360, 390, and 430 mW $ cm^{−2} $, respectively. Graphic Abstract © The Author(s), under exclusive licence to Springer Nature B.V. 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
| abstract_unstemmed |
Abstract In this study, carbon blacks, containing nitrogen and boron, are used as cathode catalysts first time in a hydrogen-bromine redox flow cell. Nitrogen and boron doping has been applied to carbon blacks to improve the limited properties of the Vulcan XC72 (VXC). Here, we have examined the effect of nitrogen-/boron-doped Vulcan XC72 carbon black on hydrogen-bromine flow cell performance. Nitrogen gas and boric acid are used as nitrogen and boron sources in the post-doping process, respectively. XRD, SEM, XPS, Raman spectroscopy, and $ N_{2} $ adsorption analyses are used to characterize the structures of cathode catalysts. The electrochemical characterization of the catalysts has been carried out with the cyclic voltammetry technique using the conventional three-electrode system connected to a potentiostat. We have addressed the effect of nitrogen and boron doping into the carbon black onto the flow battery performance by comparing their polarization and power curves. The maximum power densities with the VXC, N-VXC, and B-VXC cathode catalysts have been measured at 0.75 V as 360, 390, and 430 mW $ cm^{−2} $, respectively. Graphic Abstract © The Author(s), under exclusive licence to Springer Nature B.V. 2023. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law. |
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7 |
| title_short |
Development of low-cost nitrogen- and boron-doped carbon black cathode catalysts for the improvement of hydrogen-bromine flow battery cathode kinetics |
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https://dx.doi.org/10.1007/s10800-023-01864-5 |
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Fıçıcılar, Berker |
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10.1007/s10800-023-01864-5 |
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| score |
7.3988714 |