From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis

Catalysis is a highly complex phenomenon involving fundamental processes on multiple length scales. The full-scale complexity of catalysis is only poorly understood, and how atomic-scale processes influence long-range order in the materials is not well documented experimentally. The result is that w...
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Gespeichert in:

Autor*in:	Hansen, Thomas Willum [verfasserIn] Willinger, Marc

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Schlagwörter:	Transmission electron microscopy (TEM) Scanning electron microscopy (SEM) Catalysis Kinetics

Anmerkung:	© The Author(s) 2023

Übergeordnetes Werk:	Enthalten in: MRS bulletin - Berlin : Springer, 1982, 48(2023), 8 vom: Aug., Seite 842-851
Übergeordnetes Werk:	volume:48 ; year:2023 ; number:8 ; month:08 ; pages:842-851

Links:	Volltext

DOI / URN:	10.1557/s43577-023-00596-3

Katalog-ID:	SPR053242149

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520			\|a Catalysis is a highly complex phenomenon involving fundamental processes on multiple length scales. The full-scale complexity of catalysis is only poorly understood, and how atomic-scale processes influence long-range order in the materials is not well documented experimentally. The result is that we still, to a large degree, develop new catalysts on the basis of iterative trial-and-error approaches. Elucidating the link between atomic-scale structural dynamics, feedback mechanisms, and collective behavior could be the key to a deeper understanding and further optimization of catalysts and processes. From imaging of quasi-static low-energy configurations through gas-phase-induced state switching to observation of complex nonequilibrium dynamics and oscillatory behavior, electron microscopy has provided novel insights over several length and time scales and has meanwhile matured from a service tool for catalyst researchers to a driving force in catalysis research. Here, we discuss new insights provided by novel instrumentation and the extension from in situ to operando investigations, enabling the study of mechanisms and kinetics of catalytic processes. Graphical abstract
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912			\|a GBV_ILN_2021
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912			\|a GBV_ILN_2026
912			\|a GBV_ILN_2027
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912			\|a GBV_ILN_2037
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912			\|a GBV_ILN_2049
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allfields	10.1557/s43577-023-00596-3 doi (DE-627)SPR053242149 (SPR)s43577-023-00596-3-e DE-627 ger DE-627 rakwb eng Hansen, Thomas Willum verfasserin aut From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2023 Catalysis is a highly complex phenomenon involving fundamental processes on multiple length scales. The full-scale complexity of catalysis is only poorly understood, and how atomic-scale processes influence long-range order in the materials is not well documented experimentally. The result is that we still, to a large degree, develop new catalysts on the basis of iterative trial-and-error approaches. Elucidating the link between atomic-scale structural dynamics, feedback mechanisms, and collective behavior could be the key to a deeper understanding and further optimization of catalysts and processes. From imaging of quasi-static low-energy configurations through gas-phase-induced state switching to observation of complex nonequilibrium dynamics and oscillatory behavior, electron microscopy has provided novel insights over several length and time scales and has meanwhile matured from a service tool for catalyst researchers to a driving force in catalysis research. Here, we discuss new insights provided by novel instrumentation and the extension from in situ to operando investigations, enabling the study of mechanisms and kinetics of catalytic processes. Graphical abstract Transmission electron microscopy (TEM) (dpeaa)DE-He213 Scanning electron microscopy (SEM) (dpeaa)DE-He213 Catalysis (dpeaa)DE-He213 Kinetics (dpeaa)DE-He213 Willinger, Marc (orcid)0000-0002-9996-7953 aut Enthalten in MRS bulletin Berlin : Springer, 1982 48(2023), 8 vom: Aug., Seite 842-851 (DE-627)379081628 (DE-600)2136359-6 1938-1425 nnns volume:48 year:2023 number:8 month:08 pages:842-851 https://dx.doi.org/10.1557/s43577-023-00596-3 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 48 2023 8 08 842-851
spelling	10.1557/s43577-023-00596-3 doi (DE-627)SPR053242149 (SPR)s43577-023-00596-3-e DE-627 ger DE-627 rakwb eng Hansen, Thomas Willum verfasserin aut From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2023 Catalysis is a highly complex phenomenon involving fundamental processes on multiple length scales. The full-scale complexity of catalysis is only poorly understood, and how atomic-scale processes influence long-range order in the materials is not well documented experimentally. The result is that we still, to a large degree, develop new catalysts on the basis of iterative trial-and-error approaches. Elucidating the link between atomic-scale structural dynamics, feedback mechanisms, and collective behavior could be the key to a deeper understanding and further optimization of catalysts and processes. From imaging of quasi-static low-energy configurations through gas-phase-induced state switching to observation of complex nonequilibrium dynamics and oscillatory behavior, electron microscopy has provided novel insights over several length and time scales and has meanwhile matured from a service tool for catalyst researchers to a driving force in catalysis research. Here, we discuss new insights provided by novel instrumentation and the extension from in situ to operando investigations, enabling the study of mechanisms and kinetics of catalytic processes. Graphical abstract Transmission electron microscopy (TEM) (dpeaa)DE-He213 Scanning electron microscopy (SEM) (dpeaa)DE-He213 Catalysis (dpeaa)DE-He213 Kinetics (dpeaa)DE-He213 Willinger, Marc (orcid)0000-0002-9996-7953 aut Enthalten in MRS bulletin Berlin : Springer, 1982 48(2023), 8 vom: Aug., Seite 842-851 (DE-627)379081628 (DE-600)2136359-6 1938-1425 nnns volume:48 year:2023 number:8 month:08 pages:842-851 https://dx.doi.org/10.1557/s43577-023-00596-3 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 48 2023 8 08 842-851
allfields_unstemmed	10.1557/s43577-023-00596-3 doi (DE-627)SPR053242149 (SPR)s43577-023-00596-3-e DE-627 ger DE-627 rakwb eng Hansen, Thomas Willum verfasserin aut From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2023 Catalysis is a highly complex phenomenon involving fundamental processes on multiple length scales. The full-scale complexity of catalysis is only poorly understood, and how atomic-scale processes influence long-range order in the materials is not well documented experimentally. The result is that we still, to a large degree, develop new catalysts on the basis of iterative trial-and-error approaches. Elucidating the link between atomic-scale structural dynamics, feedback mechanisms, and collective behavior could be the key to a deeper understanding and further optimization of catalysts and processes. From imaging of quasi-static low-energy configurations through gas-phase-induced state switching to observation of complex nonequilibrium dynamics and oscillatory behavior, electron microscopy has provided novel insights over several length and time scales and has meanwhile matured from a service tool for catalyst researchers to a driving force in catalysis research. Here, we discuss new insights provided by novel instrumentation and the extension from in situ to operando investigations, enabling the study of mechanisms and kinetics of catalytic processes. Graphical abstract Transmission electron microscopy (TEM) (dpeaa)DE-He213 Scanning electron microscopy (SEM) (dpeaa)DE-He213 Catalysis (dpeaa)DE-He213 Kinetics (dpeaa)DE-He213 Willinger, Marc (orcid)0000-0002-9996-7953 aut Enthalten in MRS bulletin Berlin : Springer, 1982 48(2023), 8 vom: Aug., Seite 842-851 (DE-627)379081628 (DE-600)2136359-6 1938-1425 nnns volume:48 year:2023 number:8 month:08 pages:842-851 https://dx.doi.org/10.1557/s43577-023-00596-3 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 48 2023 8 08 842-851
allfieldsGer	10.1557/s43577-023-00596-3 doi (DE-627)SPR053242149 (SPR)s43577-023-00596-3-e DE-627 ger DE-627 rakwb eng Hansen, Thomas Willum verfasserin aut From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2023 Catalysis is a highly complex phenomenon involving fundamental processes on multiple length scales. The full-scale complexity of catalysis is only poorly understood, and how atomic-scale processes influence long-range order in the materials is not well documented experimentally. The result is that we still, to a large degree, develop new catalysts on the basis of iterative trial-and-error approaches. Elucidating the link between atomic-scale structural dynamics, feedback mechanisms, and collective behavior could be the key to a deeper understanding and further optimization of catalysts and processes. From imaging of quasi-static low-energy configurations through gas-phase-induced state switching to observation of complex nonequilibrium dynamics and oscillatory behavior, electron microscopy has provided novel insights over several length and time scales and has meanwhile matured from a service tool for catalyst researchers to a driving force in catalysis research. Here, we discuss new insights provided by novel instrumentation and the extension from in situ to operando investigations, enabling the study of mechanisms and kinetics of catalytic processes. Graphical abstract Transmission electron microscopy (TEM) (dpeaa)DE-He213 Scanning electron microscopy (SEM) (dpeaa)DE-He213 Catalysis (dpeaa)DE-He213 Kinetics (dpeaa)DE-He213 Willinger, Marc (orcid)0000-0002-9996-7953 aut Enthalten in MRS bulletin Berlin : Springer, 1982 48(2023), 8 vom: Aug., Seite 842-851 (DE-627)379081628 (DE-600)2136359-6 1938-1425 nnns volume:48 year:2023 number:8 month:08 pages:842-851 https://dx.doi.org/10.1557/s43577-023-00596-3 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 48 2023 8 08 842-851
allfieldsSound	10.1557/s43577-023-00596-3 doi (DE-627)SPR053242149 (SPR)s43577-023-00596-3-e DE-627 ger DE-627 rakwb eng Hansen, Thomas Willum verfasserin aut From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © The Author(s) 2023 Catalysis is a highly complex phenomenon involving fundamental processes on multiple length scales. The full-scale complexity of catalysis is only poorly understood, and how atomic-scale processes influence long-range order in the materials is not well documented experimentally. The result is that we still, to a large degree, develop new catalysts on the basis of iterative trial-and-error approaches. Elucidating the link between atomic-scale structural dynamics, feedback mechanisms, and collective behavior could be the key to a deeper understanding and further optimization of catalysts and processes. From imaging of quasi-static low-energy configurations through gas-phase-induced state switching to observation of complex nonequilibrium dynamics and oscillatory behavior, electron microscopy has provided novel insights over several length and time scales and has meanwhile matured from a service tool for catalyst researchers to a driving force in catalysis research. Here, we discuss new insights provided by novel instrumentation and the extension from in situ to operando investigations, enabling the study of mechanisms and kinetics of catalytic processes. Graphical abstract Transmission electron microscopy (TEM) (dpeaa)DE-He213 Scanning electron microscopy (SEM) (dpeaa)DE-He213 Catalysis (dpeaa)DE-He213 Kinetics (dpeaa)DE-He213 Willinger, Marc (orcid)0000-0002-9996-7953 aut Enthalten in MRS bulletin Berlin : Springer, 1982 48(2023), 8 vom: Aug., Seite 842-851 (DE-627)379081628 (DE-600)2136359-6 1938-1425 nnns volume:48 year:2023 number:8 month:08 pages:842-851 https://dx.doi.org/10.1557/s43577-023-00596-3 kostenfrei Volltext GBV_USEFLAG_A SYSFLAG_A GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_121 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_165 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_374 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 48 2023 8 08 842-851
language	English
source	Enthalten in MRS bulletin 48(2023), 8 vom: Aug., Seite 842-851 volume:48 year:2023 number:8 month:08 pages:842-851
sourceStr	Enthalten in MRS bulletin 48(2023), 8 vom: Aug., Seite 842-851 volume:48 year:2023 number:8 month:08 pages:842-851
format_phy_str_mv	Article
institution	findex.gbv.de
topic_facet	Transmission electron microscopy (TEM) Scanning electron microscopy (SEM) Catalysis Kinetics
isfreeaccess_bool	true
container_title	MRS bulletin
authorswithroles_txt_mv	Hansen, Thomas Willum @@aut@@ Willinger, Marc @@aut@@
publishDateDaySort_date	2023-08-01T00:00:00Z
hierarchy_top_id	379081628
id	SPR053242149
language_de	englisch
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author	Hansen, Thomas Willum
spellingShingle	Hansen, Thomas Willum misc Transmission electron microscopy (TEM) misc Scanning electron microscopy (SEM) misc Catalysis misc Kinetics From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis
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topic_title	From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis Transmission electron microscopy (TEM) (dpeaa)DE-He213 Scanning electron microscopy (SEM) (dpeaa)DE-He213 Catalysis (dpeaa)DE-He213 Kinetics (dpeaa)DE-He213
topic	misc Transmission electron microscopy (TEM) misc Scanning electron microscopy (SEM) misc Catalysis misc Kinetics
topic_unstemmed	misc Transmission electron microscopy (TEM) misc Scanning electron microscopy (SEM) misc Catalysis misc Kinetics
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title	From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis
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title_full	From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis
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title_sort	from atomistic to collective dynamics: bridging gaps in gas-phase electron microscopy for catalysis
title_auth	From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis
abstract	Catalysis is a highly complex phenomenon involving fundamental processes on multiple length scales. The full-scale complexity of catalysis is only poorly understood, and how atomic-scale processes influence long-range order in the materials is not well documented experimentally. The result is that we still, to a large degree, develop new catalysts on the basis of iterative trial-and-error approaches. Elucidating the link between atomic-scale structural dynamics, feedback mechanisms, and collective behavior could be the key to a deeper understanding and further optimization of catalysts and processes. From imaging of quasi-static low-energy configurations through gas-phase-induced state switching to observation of complex nonequilibrium dynamics and oscillatory behavior, electron microscopy has provided novel insights over several length and time scales and has meanwhile matured from a service tool for catalyst researchers to a driving force in catalysis research. Here, we discuss new insights provided by novel instrumentation and the extension from in situ to operando investigations, enabling the study of mechanisms and kinetics of catalytic processes. Graphical abstract © The Author(s) 2023
abstractGer	Catalysis is a highly complex phenomenon involving fundamental processes on multiple length scales. The full-scale complexity of catalysis is only poorly understood, and how atomic-scale processes influence long-range order in the materials is not well documented experimentally. The result is that we still, to a large degree, develop new catalysts on the basis of iterative trial-and-error approaches. Elucidating the link between atomic-scale structural dynamics, feedback mechanisms, and collective behavior could be the key to a deeper understanding and further optimization of catalysts and processes. From imaging of quasi-static low-energy configurations through gas-phase-induced state switching to observation of complex nonequilibrium dynamics and oscillatory behavior, electron microscopy has provided novel insights over several length and time scales and has meanwhile matured from a service tool for catalyst researchers to a driving force in catalysis research. Here, we discuss new insights provided by novel instrumentation and the extension from in situ to operando investigations, enabling the study of mechanisms and kinetics of catalytic processes. Graphical abstract © The Author(s) 2023
abstract_unstemmed	Catalysis is a highly complex phenomenon involving fundamental processes on multiple length scales. The full-scale complexity of catalysis is only poorly understood, and how atomic-scale processes influence long-range order in the materials is not well documented experimentally. The result is that we still, to a large degree, develop new catalysts on the basis of iterative trial-and-error approaches. Elucidating the link between atomic-scale structural dynamics, feedback mechanisms, and collective behavior could be the key to a deeper understanding and further optimization of catalysts and processes. From imaging of quasi-static low-energy configurations through gas-phase-induced state switching to observation of complex nonequilibrium dynamics and oscillatory behavior, electron microscopy has provided novel insights over several length and time scales and has meanwhile matured from a service tool for catalyst researchers to a driving force in catalysis research. Here, we discuss new insights provided by novel instrumentation and the extension from in situ to operando investigations, enabling the study of mechanisms and kinetics of catalytic processes. Graphical abstract © The Author(s) 2023
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title_short	From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis
url	https://dx.doi.org/10.1557/s43577-023-00596-3
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up_date	2024-07-03T18:05:51.120Z
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fullrecord_marcxml	<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000naa a22002652 4500</leader><controlfield tag="001">SPR053242149</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20231002150229.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">231002s2023 xx \|\|\|\|\|o 00\| \|\|eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1557/s43577-023-00596-3</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)SPR053242149</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(SPR)s43577-023-00596-3-e</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Hansen, Thomas Willum</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2023</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="500" ind1=" " ind2=" "><subfield code="a">© The Author(s) 2023</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Catalysis is a highly complex phenomenon involving fundamental processes on multiple length scales. The full-scale complexity of catalysis is only poorly understood, and how atomic-scale processes influence long-range order in the materials is not well documented experimentally. The result is that we still, to a large degree, develop new catalysts on the basis of iterative trial-and-error approaches. Elucidating the link between atomic-scale structural dynamics, feedback mechanisms, and collective behavior could be the key to a deeper understanding and further optimization of catalysts and processes. From imaging of quasi-static low-energy configurations through gas-phase-induced state switching to observation of complex nonequilibrium dynamics and oscillatory behavior, electron microscopy has provided novel insights over several length and time scales and has meanwhile matured from a service tool for catalyst researchers to a driving force in catalysis research. Here, we discuss new insights provided by novel instrumentation and the extension from in situ to operando investigations, enabling the study of mechanisms and kinetics of catalytic processes. 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From atomistic to collective dynamics: Bridging gaps in gas-phase electron microscopy for catalysis

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