Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance

Abstract A 100 nm synthetic diamond particle with a large (>4 ppm) amount of nitrogen vacancy (NV) centers has been studied. The latter exhibit lines associated with forbidden Δms= 2 and allowed Δms= 1 transitions in the electron paramagnetic resonance (EPR) spectra of the ground state of the $ N...
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Autor*in:	Osipov, V. Yu. [verfasserIn] Bogdanov, K. V. Treussart, F. Rampersaud, A. Baranov, A. V.

Format:	E-Artikel
Sprache:	Englisch

Erschienen:	2023

Anmerkung:	© Pleiades Publishing, Ltd. 2023. ISSN 0030-400X, Optics and Spectroscopy, 2023, Vol. 131, No. 1, pp. 38–47. © Pleiades Publishing, Ltd., 2023. Russian Text © The Author(s), 2022, published in Optika i Spektroskopiya, 2022, Vol. 130, No. 2, pp. 332–341. English Text © Ioffe Institute, 2023.

Übergeordnetes Werk:	Enthalten in: Optics and spectroscopy - Pleiades Publishing, 1996, 131(2023), 1 vom: Jan., Seite 38-47
Übergeordnetes Werk:	volume:131 ; year:2023 ; number:1 ; month:01 ; pages:38-47

Links:	Volltext

DOI / URN:	10.1134/S0030400X2303013X

Katalog-ID:	SPR055145841

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520			\|a Abstract A 100 nm synthetic diamond particle with a large (>4 ppm) amount of nitrogen vacancy (NV) centers has been studied. The latter exhibit lines associated with forbidden Δms= 2 and allowed Δms= 1 transitions in the electron paramagnetic resonance (EPR) spectra of the ground state of the $ NV^{(–)} $ center. The luminescence intensity of particles in the range 550–800 nm increases with an increase in the irradiation dose of 5 MeV electrons and correlates with the integrated intensity of the peak EPR line with a g-factor g = 4.27. This value is used to estimate the concentration of $ NV^{(–)} $ centers and to select diamond powders with the highest fluorescence intensity. The dependence of the EPR signal intensity of the Δms= 2 transition of the $ NV^{(–)} $ center on the microwave power that increases before decaying rather well characterizes the crystal quality of the local environment of the centers under study in these particles. The intensity of the x, yΔms= 1 transition (at ~281.2 mT, 9.444 GHz) turns out to be sensitive to changes in particle size in the submicron range and the appearance of near-surface defects obtained during mechanical processing.
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allfields	10.1134/S0030400X2303013X doi (DE-627)SPR055145841 (SPR)S0030400X2303013X-e DE-627 ger DE-627 rakwb eng 530 VZ 11 ssgn 33.07 bkl 33.38 bkl Osipov, V. Yu. verfasserin aut Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2023. ISSN 0030-400X, Optics and Spectroscopy, 2023, Vol. 131, No. 1, pp. 38–47. © Pleiades Publishing, Ltd., 2023. Russian Text © The Author(s), 2022, published in Optika i Spektroskopiya, 2022, Vol. 130, No. 2, pp. 332–341. English Text © Ioffe Institute, 2023. Abstract A 100 nm synthetic diamond particle with a large (>4 ppm) amount of nitrogen vacancy (NV) centers has been studied. The latter exhibit lines associated with forbidden Δms= 2 and allowed Δms= 1 transitions in the electron paramagnetic resonance (EPR) spectra of the ground state of the $ NV^{(–)} $ center. The luminescence intensity of particles in the range 550–800 nm increases with an increase in the irradiation dose of 5 MeV electrons and correlates with the integrated intensity of the peak EPR line with a g-factor g = 4.27. This value is used to estimate the concentration of $ NV^{(–)} $ centers and to select diamond powders with the highest fluorescence intensity. The dependence of the EPR signal intensity of the Δms= 2 transition of the $ NV^{(–)} $ center on the microwave power that increases before decaying rather well characterizes the crystal quality of the local environment of the centers under study in these particles. The intensity of the x, yΔms= 1 transition (at ~281.2 mT, 9.444 GHz) turns out to be sensitive to changes in particle size in the submicron range and the appearance of near-surface defects obtained during mechanical processing. Bogdanov, K. V. aut Treussart, F. aut Rampersaud, A. aut Baranov, A. V. aut Enthalten in Optics and spectroscopy Pleiades Publishing, 1996 131(2023), 1 vom: Jan., Seite 38-47 (DE-627)32453244X (DE-600)2028261-8 1562-6911 nnns volume:131 year:2023 number:1 month:01 pages:38-47 https://dx.doi.org/10.1134/S0030400X2303013X lizenzpflichtig Volltext SYSFLAG_0 GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.07 VZ 33.38 VZ AR 131 2023 1 01 38-47
spelling	10.1134/S0030400X2303013X doi (DE-627)SPR055145841 (SPR)S0030400X2303013X-e DE-627 ger DE-627 rakwb eng 530 VZ 11 ssgn 33.07 bkl 33.38 bkl Osipov, V. Yu. verfasserin aut Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2023. ISSN 0030-400X, Optics and Spectroscopy, 2023, Vol. 131, No. 1, pp. 38–47. © Pleiades Publishing, Ltd., 2023. Russian Text © The Author(s), 2022, published in Optika i Spektroskopiya, 2022, Vol. 130, No. 2, pp. 332–341. English Text © Ioffe Institute, 2023. Abstract A 100 nm synthetic diamond particle with a large (>4 ppm) amount of nitrogen vacancy (NV) centers has been studied. The latter exhibit lines associated with forbidden Δms= 2 and allowed Δms= 1 transitions in the electron paramagnetic resonance (EPR) spectra of the ground state of the $ NV^{(–)} $ center. The luminescence intensity of particles in the range 550–800 nm increases with an increase in the irradiation dose of 5 MeV electrons and correlates with the integrated intensity of the peak EPR line with a g-factor g = 4.27. This value is used to estimate the concentration of $ NV^{(–)} $ centers and to select diamond powders with the highest fluorescence intensity. The dependence of the EPR signal intensity of the Δms= 2 transition of the $ NV^{(–)} $ center on the microwave power that increases before decaying rather well characterizes the crystal quality of the local environment of the centers under study in these particles. The intensity of the x, yΔms= 1 transition (at ~281.2 mT, 9.444 GHz) turns out to be sensitive to changes in particle size in the submicron range and the appearance of near-surface defects obtained during mechanical processing. Bogdanov, K. V. aut Treussart, F. aut Rampersaud, A. aut Baranov, A. V. aut Enthalten in Optics and spectroscopy Pleiades Publishing, 1996 131(2023), 1 vom: Jan., Seite 38-47 (DE-627)32453244X (DE-600)2028261-8 1562-6911 nnns volume:131 year:2023 number:1 month:01 pages:38-47 https://dx.doi.org/10.1134/S0030400X2303013X lizenzpflichtig Volltext SYSFLAG_0 GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.07 VZ 33.38 VZ AR 131 2023 1 01 38-47
allfields_unstemmed	10.1134/S0030400X2303013X doi (DE-627)SPR055145841 (SPR)S0030400X2303013X-e DE-627 ger DE-627 rakwb eng 530 VZ 11 ssgn 33.07 bkl 33.38 bkl Osipov, V. Yu. verfasserin aut Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2023. ISSN 0030-400X, Optics and Spectroscopy, 2023, Vol. 131, No. 1, pp. 38–47. © Pleiades Publishing, Ltd., 2023. Russian Text © The Author(s), 2022, published in Optika i Spektroskopiya, 2022, Vol. 130, No. 2, pp. 332–341. English Text © Ioffe Institute, 2023. Abstract A 100 nm synthetic diamond particle with a large (>4 ppm) amount of nitrogen vacancy (NV) centers has been studied. The latter exhibit lines associated with forbidden Δms= 2 and allowed Δms= 1 transitions in the electron paramagnetic resonance (EPR) spectra of the ground state of the $ NV^{(–)} $ center. The luminescence intensity of particles in the range 550–800 nm increases with an increase in the irradiation dose of 5 MeV electrons and correlates with the integrated intensity of the peak EPR line with a g-factor g = 4.27. This value is used to estimate the concentration of $ NV^{(–)} $ centers and to select diamond powders with the highest fluorescence intensity. The dependence of the EPR signal intensity of the Δms= 2 transition of the $ NV^{(–)} $ center on the microwave power that increases before decaying rather well characterizes the crystal quality of the local environment of the centers under study in these particles. The intensity of the x, yΔms= 1 transition (at ~281.2 mT, 9.444 GHz) turns out to be sensitive to changes in particle size in the submicron range and the appearance of near-surface defects obtained during mechanical processing. Bogdanov, K. V. aut Treussart, F. aut Rampersaud, A. aut Baranov, A. V. aut Enthalten in Optics and spectroscopy Pleiades Publishing, 1996 131(2023), 1 vom: Jan., Seite 38-47 (DE-627)32453244X (DE-600)2028261-8 1562-6911 nnns volume:131 year:2023 number:1 month:01 pages:38-47 https://dx.doi.org/10.1134/S0030400X2303013X lizenzpflichtig Volltext SYSFLAG_0 GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.07 VZ 33.38 VZ AR 131 2023 1 01 38-47
allfieldsGer	10.1134/S0030400X2303013X doi (DE-627)SPR055145841 (SPR)S0030400X2303013X-e DE-627 ger DE-627 rakwb eng 530 VZ 11 ssgn 33.07 bkl 33.38 bkl Osipov, V. Yu. verfasserin aut Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2023. ISSN 0030-400X, Optics and Spectroscopy, 2023, Vol. 131, No. 1, pp. 38–47. © Pleiades Publishing, Ltd., 2023. Russian Text © The Author(s), 2022, published in Optika i Spektroskopiya, 2022, Vol. 130, No. 2, pp. 332–341. English Text © Ioffe Institute, 2023. Abstract A 100 nm synthetic diamond particle with a large (>4 ppm) amount of nitrogen vacancy (NV) centers has been studied. The latter exhibit lines associated with forbidden Δms= 2 and allowed Δms= 1 transitions in the electron paramagnetic resonance (EPR) spectra of the ground state of the $ NV^{(–)} $ center. The luminescence intensity of particles in the range 550–800 nm increases with an increase in the irradiation dose of 5 MeV electrons and correlates with the integrated intensity of the peak EPR line with a g-factor g = 4.27. This value is used to estimate the concentration of $ NV^{(–)} $ centers and to select diamond powders with the highest fluorescence intensity. The dependence of the EPR signal intensity of the Δms= 2 transition of the $ NV^{(–)} $ center on the microwave power that increases before decaying rather well characterizes the crystal quality of the local environment of the centers under study in these particles. The intensity of the x, yΔms= 1 transition (at ~281.2 mT, 9.444 GHz) turns out to be sensitive to changes in particle size in the submicron range and the appearance of near-surface defects obtained during mechanical processing. Bogdanov, K. V. aut Treussart, F. aut Rampersaud, A. aut Baranov, A. V. aut Enthalten in Optics and spectroscopy Pleiades Publishing, 1996 131(2023), 1 vom: Jan., Seite 38-47 (DE-627)32453244X (DE-600)2028261-8 1562-6911 nnns volume:131 year:2023 number:1 month:01 pages:38-47 https://dx.doi.org/10.1134/S0030400X2303013X lizenzpflichtig Volltext SYSFLAG_0 GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.07 VZ 33.38 VZ AR 131 2023 1 01 38-47
allfieldsSound	10.1134/S0030400X2303013X doi (DE-627)SPR055145841 (SPR)S0030400X2303013X-e DE-627 ger DE-627 rakwb eng 530 VZ 11 ssgn 33.07 bkl 33.38 bkl Osipov, V. Yu. verfasserin aut Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance 2023 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Pleiades Publishing, Ltd. 2023. ISSN 0030-400X, Optics and Spectroscopy, 2023, Vol. 131, No. 1, pp. 38–47. © Pleiades Publishing, Ltd., 2023. Russian Text © The Author(s), 2022, published in Optika i Spektroskopiya, 2022, Vol. 130, No. 2, pp. 332–341. English Text © Ioffe Institute, 2023. Abstract A 100 nm synthetic diamond particle with a large (>4 ppm) amount of nitrogen vacancy (NV) centers has been studied. The latter exhibit lines associated with forbidden Δms= 2 and allowed Δms= 1 transitions in the electron paramagnetic resonance (EPR) spectra of the ground state of the $ NV^{(–)} $ center. The luminescence intensity of particles in the range 550–800 nm increases with an increase in the irradiation dose of 5 MeV electrons and correlates with the integrated intensity of the peak EPR line with a g-factor g = 4.27. This value is used to estimate the concentration of $ NV^{(–)} $ centers and to select diamond powders with the highest fluorescence intensity. The dependence of the EPR signal intensity of the Δms= 2 transition of the $ NV^{(–)} $ center on the microwave power that increases before decaying rather well characterizes the crystal quality of the local environment of the centers under study in these particles. The intensity of the x, yΔms= 1 transition (at ~281.2 mT, 9.444 GHz) turns out to be sensitive to changes in particle size in the submicron range and the appearance of near-surface defects obtained during mechanical processing. Bogdanov, K. V. aut Treussart, F. aut Rampersaud, A. aut Baranov, A. V. aut Enthalten in Optics and spectroscopy Pleiades Publishing, 1996 131(2023), 1 vom: Jan., Seite 38-47 (DE-627)32453244X (DE-600)2028261-8 1562-6911 nnns volume:131 year:2023 number:1 month:01 pages:38-47 https://dx.doi.org/10.1134/S0030400X2303013X lizenzpflichtig Volltext SYSFLAG_0 GBV_SPRINGER GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_206 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2008 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2119 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 33.07 VZ 33.38 VZ AR 131 2023 1 01 38-47
language	English
source	Enthalten in Optics and spectroscopy 131(2023), 1 vom: Jan., Seite 38-47 volume:131 year:2023 number:1 month:01 pages:38-47
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authorswithroles_txt_mv	Osipov, V. Yu. @@aut@@ Bogdanov, K. V. @@aut@@ Treussart, F. @@aut@@ Rampersaud, A. @@aut@@ Baranov, A. V. @@aut@@
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author	Osipov, V. Yu.
spellingShingle	Osipov, V. Yu. ddc 530 ssgn 11 bkl 33.07 bkl 33.38 Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance
authorStr	Osipov, V. Yu.
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topic_title	530 VZ 11 ssgn 33.07 bkl 33.38 bkl Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance
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title	Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance
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title_full	Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance
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author_browse	Osipov, V. Yu. Bogdanov, K. V. Treussart, F. Rampersaud, A. Baranov, A. V.
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title_sort	identification of nv centers in synthetic fluorescent nanodiamonds and control of defectiveness of crystallites using electron paramagnetic resonance
title_auth	Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance
abstract	Abstract A 100 nm synthetic diamond particle with a large (>4 ppm) amount of nitrogen vacancy (NV) centers has been studied. The latter exhibit lines associated with forbidden Δms= 2 and allowed Δms= 1 transitions in the electron paramagnetic resonance (EPR) spectra of the ground state of the $ NV^{(–)} $ center. The luminescence intensity of particles in the range 550–800 nm increases with an increase in the irradiation dose of 5 MeV electrons and correlates with the integrated intensity of the peak EPR line with a g-factor g = 4.27. This value is used to estimate the concentration of $ NV^{(–)} $ centers and to select diamond powders with the highest fluorescence intensity. The dependence of the EPR signal intensity of the Δms= 2 transition of the $ NV^{(–)} $ center on the microwave power that increases before decaying rather well characterizes the crystal quality of the local environment of the centers under study in these particles. The intensity of the x, yΔms= 1 transition (at ~281.2 mT, 9.444 GHz) turns out to be sensitive to changes in particle size in the submicron range and the appearance of near-surface defects obtained during mechanical processing. © Pleiades Publishing, Ltd. 2023. ISSN 0030-400X, Optics and Spectroscopy, 2023, Vol. 131, No. 1, pp. 38–47. © Pleiades Publishing, Ltd., 2023. Russian Text © The Author(s), 2022, published in Optika i Spektroskopiya, 2022, Vol. 130, No. 2, pp. 332–341. English Text © Ioffe Institute, 2023.
abstractGer	Abstract A 100 nm synthetic diamond particle with a large (>4 ppm) amount of nitrogen vacancy (NV) centers has been studied. The latter exhibit lines associated with forbidden Δms= 2 and allowed Δms= 1 transitions in the electron paramagnetic resonance (EPR) spectra of the ground state of the $ NV^{(–)} $ center. The luminescence intensity of particles in the range 550–800 nm increases with an increase in the irradiation dose of 5 MeV electrons and correlates with the integrated intensity of the peak EPR line with a g-factor g = 4.27. This value is used to estimate the concentration of $ NV^{(–)} $ centers and to select diamond powders with the highest fluorescence intensity. The dependence of the EPR signal intensity of the Δms= 2 transition of the $ NV^{(–)} $ center on the microwave power that increases before decaying rather well characterizes the crystal quality of the local environment of the centers under study in these particles. The intensity of the x, yΔms= 1 transition (at ~281.2 mT, 9.444 GHz) turns out to be sensitive to changes in particle size in the submicron range and the appearance of near-surface defects obtained during mechanical processing. © Pleiades Publishing, Ltd. 2023. ISSN 0030-400X, Optics and Spectroscopy, 2023, Vol. 131, No. 1, pp. 38–47. © Pleiades Publishing, Ltd., 2023. Russian Text © The Author(s), 2022, published in Optika i Spektroskopiya, 2022, Vol. 130, No. 2, pp. 332–341. English Text © Ioffe Institute, 2023.
abstract_unstemmed	Abstract A 100 nm synthetic diamond particle with a large (>4 ppm) amount of nitrogen vacancy (NV) centers has been studied. The latter exhibit lines associated with forbidden Δms= 2 and allowed Δms= 1 transitions in the electron paramagnetic resonance (EPR) spectra of the ground state of the $ NV^{(–)} $ center. The luminescence intensity of particles in the range 550–800 nm increases with an increase in the irradiation dose of 5 MeV electrons and correlates with the integrated intensity of the peak EPR line with a g-factor g = 4.27. This value is used to estimate the concentration of $ NV^{(–)} $ centers and to select diamond powders with the highest fluorescence intensity. The dependence of the EPR signal intensity of the Δms= 2 transition of the $ NV^{(–)} $ center on the microwave power that increases before decaying rather well characterizes the crystal quality of the local environment of the centers under study in these particles. The intensity of the x, yΔms= 1 transition (at ~281.2 mT, 9.444 GHz) turns out to be sensitive to changes in particle size in the submicron range and the appearance of near-surface defects obtained during mechanical processing. © Pleiades Publishing, Ltd. 2023. ISSN 0030-400X, Optics and Spectroscopy, 2023, Vol. 131, No. 1, pp. 38–47. © Pleiades Publishing, Ltd., 2023. Russian Text © The Author(s), 2022, published in Optika i Spektroskopiya, 2022, Vol. 130, No. 2, pp. 332–341. English Text © Ioffe Institute, 2023.
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title_short	Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance
url	https://dx.doi.org/10.1134/S0030400X2303013X
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Yu.</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2023</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="500" ind1=" " ind2=" "><subfield code="a">© Pleiades Publishing, Ltd. 2023. ISSN 0030-400X, Optics and Spectroscopy, 2023, Vol. 131, No. 1, pp. 38–47. © Pleiades Publishing, Ltd., 2023. Russian Text © The Author(s), 2022, published in Optika i Spektroskopiya, 2022, Vol. 130, No. 2, pp. 332–341. English Text © Ioffe Institute, 2023.</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Abstract A 100 nm synthetic diamond particle with a large (>4 ppm) amount of nitrogen vacancy (NV) centers has been studied. The latter exhibit lines associated with forbidden Δms= 2 and allowed Δms= 1 transitions in the electron paramagnetic resonance (EPR) spectra of the ground state of the $ NV^{(–)} $ center. The luminescence intensity of particles in the range 550–800 nm increases with an increase in the irradiation dose of 5 MeV electrons and correlates with the integrated intensity of the peak EPR line with a g-factor g = 4.27. 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Identification of NV Centers in Synthetic Fluorescent Nanodiamonds and Control of Defectiveness of Crystallites Using Electron Paramagnetic Resonance

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