A robust synthesis route of confined carbyne
Abstract The unique mechanical, optical, and electrical properties of carbyne, a one-dimensional allotrope of carbon, make it a highly promising material for various applications. It has been demonstrated that carbon nanotubes (CNTs) can serve as an ideal host for the formation of confined carbyne (...
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| Autor*in: |
Feng, Yanghao [verfasserIn] Zhang, Wendi [verfasserIn] Tang, Kunpeng [verfasserIn] Chen, Yingzhi [verfasserIn] Zhang, Jiou [verfasserIn] Cao, Kecheng [verfasserIn] Cui, Weili [verfasserIn] Shi, Lei [verfasserIn] |
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| Format: |
E-Artikel |
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| Sprache: |
Englisch |
| Erschienen: |
2024 |
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| Schlagwörter: |
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| Anmerkung: |
© Tsinghua University Press 2024 |
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| Übergeordnetes Werk: |
Enthalten in: Nano research - Tsinghua University Press, 2008, 17(2024), 7 vom: 11. Apr., Seite 6274-6280 |
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| Übergeordnetes Werk: |
volume:17 ; year:2024 ; number:7 ; day:11 ; month:04 ; pages:6274-6280 |
| Links: |
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| DOI / URN: |
10.1007/s12274-024-6571-z |
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| Katalog-ID: |
SPR056460171 |
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| 520 | |a Abstract The unique mechanical, optical, and electrical properties of carbyne, a one-dimensional allotrope of carbon, make it a highly promising material for various applications. It has been demonstrated that carbon nanotubes (CNTs) can serve as an ideal host for the formation of confined carbyne (CC), with the yield being influenced by the quality of the carbon nanotubes for confinement and the carbon source for carbyne growth. In this study, a robust synthesis route of CC within CNTs is proposed. $ C_{70} $ was utilized as a precursor to provide an additional carbon source, based on its ability to supply more carbon atoms than $ C_{60} $ at the same filling ratio. Multi-step transformation processes, including defect creation, were designed to enhance the yield of CC. As a result, the yield of CC was significantly increased for the $ C_{70} $ encapsulated single-walled CNTs by more than an order of magnitude than the empty counterparts, which also surpasses that of the double-walled CNTs, making it the most effective route for synthesizing CC. These findings highlight the importance of the additional carbon source and the optimal pathway for CC formation, offering valuable insights for the application of materials with high yield. | ||
| 650 | 4 | |a confined carbyne |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a yield enhancement |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a carbon nanotube |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a C |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a encapsulation |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a defect introduction |7 (dpeaa)DE-He213 | |
| 650 | 4 | |a Raman spectroscopy |7 (dpeaa)DE-He213 | |
| 700 | 1 | |a Zhang, Wendi |e verfasserin |4 aut | |
| 700 | 1 | |a Tang, Kunpeng |e verfasserin |4 aut | |
| 700 | 1 | |a Chen, Yingzhi |e verfasserin |4 aut | |
| 700 | 1 | |a Zhang, Jiou |e verfasserin |4 aut | |
| 700 | 1 | |a Cao, Kecheng |e verfasserin |4 aut | |
| 700 | 1 | |a Cui, Weili |e verfasserin |4 aut | |
| 700 | 1 | |a Shi, Lei |e verfasserin |4 aut | |
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10.1007/s12274-024-6571-z doi (DE-627)SPR056460171 (SPR)s12274-024-6571-z-e DE-627 ger DE-627 rakwb eng 540 660 VZ Feng, Yanghao verfasserin aut A robust synthesis route of confined carbyne 2024 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press 2024 Abstract The unique mechanical, optical, and electrical properties of carbyne, a one-dimensional allotrope of carbon, make it a highly promising material for various applications. It has been demonstrated that carbon nanotubes (CNTs) can serve as an ideal host for the formation of confined carbyne (CC), with the yield being influenced by the quality of the carbon nanotubes for confinement and the carbon source for carbyne growth. In this study, a robust synthesis route of CC within CNTs is proposed. $ C_{70} $ was utilized as a precursor to provide an additional carbon source, based on its ability to supply more carbon atoms than $ C_{60} $ at the same filling ratio. Multi-step transformation processes, including defect creation, were designed to enhance the yield of CC. As a result, the yield of CC was significantly increased for the $ C_{70} $ encapsulated single-walled CNTs by more than an order of magnitude than the empty counterparts, which also surpasses that of the double-walled CNTs, making it the most effective route for synthesizing CC. These findings highlight the importance of the additional carbon source and the optimal pathway for CC formation, offering valuable insights for the application of materials with high yield. confined carbyne (dpeaa)DE-He213 yield enhancement (dpeaa)DE-He213 carbon nanotube (dpeaa)DE-He213 C (dpeaa)DE-He213 encapsulation (dpeaa)DE-He213 defect introduction (dpeaa)DE-He213 Raman spectroscopy (dpeaa)DE-He213 Zhang, Wendi verfasserin aut Tang, Kunpeng verfasserin aut Chen, Yingzhi verfasserin aut Zhang, Jiou verfasserin aut Cao, Kecheng verfasserin aut Cui, Weili verfasserin aut Shi, Lei verfasserin aut Enthalten in Nano research Tsinghua University Press, 2008 17(2024), 7 vom: 11. Apr., Seite 6274-6280 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:17 year:2024 number:7 day:11 month:04 pages:6274-6280 https://dx.doi.org/10.1007/s12274-024-6571-z X:SPRINGER Resolving-System lizenzpflichtig Volltext SYSFLAG_0 GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 17 2024 7 11 04 6274-6280 |
| spelling |
10.1007/s12274-024-6571-z doi (DE-627)SPR056460171 (SPR)s12274-024-6571-z-e DE-627 ger DE-627 rakwb eng 540 660 VZ Feng, Yanghao verfasserin aut A robust synthesis route of confined carbyne 2024 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press 2024 Abstract The unique mechanical, optical, and electrical properties of carbyne, a one-dimensional allotrope of carbon, make it a highly promising material for various applications. It has been demonstrated that carbon nanotubes (CNTs) can serve as an ideal host for the formation of confined carbyne (CC), with the yield being influenced by the quality of the carbon nanotubes for confinement and the carbon source for carbyne growth. In this study, a robust synthesis route of CC within CNTs is proposed. $ C_{70} $ was utilized as a precursor to provide an additional carbon source, based on its ability to supply more carbon atoms than $ C_{60} $ at the same filling ratio. Multi-step transformation processes, including defect creation, were designed to enhance the yield of CC. As a result, the yield of CC was significantly increased for the $ C_{70} $ encapsulated single-walled CNTs by more than an order of magnitude than the empty counterparts, which also surpasses that of the double-walled CNTs, making it the most effective route for synthesizing CC. These findings highlight the importance of the additional carbon source and the optimal pathway for CC formation, offering valuable insights for the application of materials with high yield. confined carbyne (dpeaa)DE-He213 yield enhancement (dpeaa)DE-He213 carbon nanotube (dpeaa)DE-He213 C (dpeaa)DE-He213 encapsulation (dpeaa)DE-He213 defect introduction (dpeaa)DE-He213 Raman spectroscopy (dpeaa)DE-He213 Zhang, Wendi verfasserin aut Tang, Kunpeng verfasserin aut Chen, Yingzhi verfasserin aut Zhang, Jiou verfasserin aut Cao, Kecheng verfasserin aut Cui, Weili verfasserin aut Shi, Lei verfasserin aut Enthalten in Nano research Tsinghua University Press, 2008 17(2024), 7 vom: 11. Apr., Seite 6274-6280 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:17 year:2024 number:7 day:11 month:04 pages:6274-6280 https://dx.doi.org/10.1007/s12274-024-6571-z X:SPRINGER Resolving-System lizenzpflichtig Volltext SYSFLAG_0 GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 17 2024 7 11 04 6274-6280 |
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10.1007/s12274-024-6571-z doi (DE-627)SPR056460171 (SPR)s12274-024-6571-z-e DE-627 ger DE-627 rakwb eng 540 660 VZ Feng, Yanghao verfasserin aut A robust synthesis route of confined carbyne 2024 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press 2024 Abstract The unique mechanical, optical, and electrical properties of carbyne, a one-dimensional allotrope of carbon, make it a highly promising material for various applications. It has been demonstrated that carbon nanotubes (CNTs) can serve as an ideal host for the formation of confined carbyne (CC), with the yield being influenced by the quality of the carbon nanotubes for confinement and the carbon source for carbyne growth. In this study, a robust synthesis route of CC within CNTs is proposed. $ C_{70} $ was utilized as a precursor to provide an additional carbon source, based on its ability to supply more carbon atoms than $ C_{60} $ at the same filling ratio. Multi-step transformation processes, including defect creation, were designed to enhance the yield of CC. As a result, the yield of CC was significantly increased for the $ C_{70} $ encapsulated single-walled CNTs by more than an order of magnitude than the empty counterparts, which also surpasses that of the double-walled CNTs, making it the most effective route for synthesizing CC. These findings highlight the importance of the additional carbon source and the optimal pathway for CC formation, offering valuable insights for the application of materials with high yield. confined carbyne (dpeaa)DE-He213 yield enhancement (dpeaa)DE-He213 carbon nanotube (dpeaa)DE-He213 C (dpeaa)DE-He213 encapsulation (dpeaa)DE-He213 defect introduction (dpeaa)DE-He213 Raman spectroscopy (dpeaa)DE-He213 Zhang, Wendi verfasserin aut Tang, Kunpeng verfasserin aut Chen, Yingzhi verfasserin aut Zhang, Jiou verfasserin aut Cao, Kecheng verfasserin aut Cui, Weili verfasserin aut Shi, Lei verfasserin aut Enthalten in Nano research Tsinghua University Press, 2008 17(2024), 7 vom: 11. Apr., Seite 6274-6280 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:17 year:2024 number:7 day:11 month:04 pages:6274-6280 https://dx.doi.org/10.1007/s12274-024-6571-z X:SPRINGER Resolving-System lizenzpflichtig Volltext SYSFLAG_0 GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 17 2024 7 11 04 6274-6280 |
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10.1007/s12274-024-6571-z doi (DE-627)SPR056460171 (SPR)s12274-024-6571-z-e DE-627 ger DE-627 rakwb eng 540 660 VZ Feng, Yanghao verfasserin aut A robust synthesis route of confined carbyne 2024 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press 2024 Abstract The unique mechanical, optical, and electrical properties of carbyne, a one-dimensional allotrope of carbon, make it a highly promising material for various applications. It has been demonstrated that carbon nanotubes (CNTs) can serve as an ideal host for the formation of confined carbyne (CC), with the yield being influenced by the quality of the carbon nanotubes for confinement and the carbon source for carbyne growth. In this study, a robust synthesis route of CC within CNTs is proposed. $ C_{70} $ was utilized as a precursor to provide an additional carbon source, based on its ability to supply more carbon atoms than $ C_{60} $ at the same filling ratio. Multi-step transformation processes, including defect creation, were designed to enhance the yield of CC. As a result, the yield of CC was significantly increased for the $ C_{70} $ encapsulated single-walled CNTs by more than an order of magnitude than the empty counterparts, which also surpasses that of the double-walled CNTs, making it the most effective route for synthesizing CC. These findings highlight the importance of the additional carbon source and the optimal pathway for CC formation, offering valuable insights for the application of materials with high yield. confined carbyne (dpeaa)DE-He213 yield enhancement (dpeaa)DE-He213 carbon nanotube (dpeaa)DE-He213 C (dpeaa)DE-He213 encapsulation (dpeaa)DE-He213 defect introduction (dpeaa)DE-He213 Raman spectroscopy (dpeaa)DE-He213 Zhang, Wendi verfasserin aut Tang, Kunpeng verfasserin aut Chen, Yingzhi verfasserin aut Zhang, Jiou verfasserin aut Cao, Kecheng verfasserin aut Cui, Weili verfasserin aut Shi, Lei verfasserin aut Enthalten in Nano research Tsinghua University Press, 2008 17(2024), 7 vom: 11. Apr., Seite 6274-6280 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:17 year:2024 number:7 day:11 month:04 pages:6274-6280 https://dx.doi.org/10.1007/s12274-024-6571-z X:SPRINGER Resolving-System lizenzpflichtig Volltext SYSFLAG_0 GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 17 2024 7 11 04 6274-6280 |
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10.1007/s12274-024-6571-z doi (DE-627)SPR056460171 (SPR)s12274-024-6571-z-e DE-627 ger DE-627 rakwb eng 540 660 VZ Feng, Yanghao verfasserin aut A robust synthesis route of confined carbyne 2024 Text txt rdacontent Computermedien c rdamedia Online-Ressource cr rdacarrier © Tsinghua University Press 2024 Abstract The unique mechanical, optical, and electrical properties of carbyne, a one-dimensional allotrope of carbon, make it a highly promising material for various applications. It has been demonstrated that carbon nanotubes (CNTs) can serve as an ideal host for the formation of confined carbyne (CC), with the yield being influenced by the quality of the carbon nanotubes for confinement and the carbon source for carbyne growth. In this study, a robust synthesis route of CC within CNTs is proposed. $ C_{70} $ was utilized as a precursor to provide an additional carbon source, based on its ability to supply more carbon atoms than $ C_{60} $ at the same filling ratio. Multi-step transformation processes, including defect creation, were designed to enhance the yield of CC. As a result, the yield of CC was significantly increased for the $ C_{70} $ encapsulated single-walled CNTs by more than an order of magnitude than the empty counterparts, which also surpasses that of the double-walled CNTs, making it the most effective route for synthesizing CC. These findings highlight the importance of the additional carbon source and the optimal pathway for CC formation, offering valuable insights for the application of materials with high yield. confined carbyne (dpeaa)DE-He213 yield enhancement (dpeaa)DE-He213 carbon nanotube (dpeaa)DE-He213 C (dpeaa)DE-He213 encapsulation (dpeaa)DE-He213 defect introduction (dpeaa)DE-He213 Raman spectroscopy (dpeaa)DE-He213 Zhang, Wendi verfasserin aut Tang, Kunpeng verfasserin aut Chen, Yingzhi verfasserin aut Zhang, Jiou verfasserin aut Cao, Kecheng verfasserin aut Cui, Weili verfasserin aut Shi, Lei verfasserin aut Enthalten in Nano research Tsinghua University Press, 2008 17(2024), 7 vom: 11. Apr., Seite 6274-6280 (DE-627)57375361X (DE-600)2442216-2 1998-0000 nnns volume:17 year:2024 number:7 day:11 month:04 pages:6274-6280 https://dx.doi.org/10.1007/s12274-024-6571-z X:SPRINGER Resolving-System lizenzpflichtig Volltext SYSFLAG_0 GBV_SPRINGER SSG-OLC-PHA GBV_ILN_11 GBV_ILN_20 GBV_ILN_22 GBV_ILN_23 GBV_ILN_24 GBV_ILN_31 GBV_ILN_32 GBV_ILN_39 GBV_ILN_40 GBV_ILN_60 GBV_ILN_62 GBV_ILN_63 GBV_ILN_65 GBV_ILN_69 GBV_ILN_70 GBV_ILN_73 GBV_ILN_74 GBV_ILN_90 GBV_ILN_95 GBV_ILN_100 GBV_ILN_101 GBV_ILN_105 GBV_ILN_110 GBV_ILN_120 GBV_ILN_138 GBV_ILN_150 GBV_ILN_151 GBV_ILN_152 GBV_ILN_161 GBV_ILN_170 GBV_ILN_171 GBV_ILN_187 GBV_ILN_213 GBV_ILN_224 GBV_ILN_230 GBV_ILN_250 GBV_ILN_281 GBV_ILN_285 GBV_ILN_293 GBV_ILN_370 GBV_ILN_602 GBV_ILN_636 GBV_ILN_702 GBV_ILN_2001 GBV_ILN_2003 GBV_ILN_2004 GBV_ILN_2005 GBV_ILN_2006 GBV_ILN_2007 GBV_ILN_2009 GBV_ILN_2010 GBV_ILN_2011 GBV_ILN_2014 GBV_ILN_2015 GBV_ILN_2020 GBV_ILN_2021 GBV_ILN_2025 GBV_ILN_2026 GBV_ILN_2027 GBV_ILN_2031 GBV_ILN_2034 GBV_ILN_2037 GBV_ILN_2038 GBV_ILN_2039 GBV_ILN_2044 GBV_ILN_2048 GBV_ILN_2049 GBV_ILN_2050 GBV_ILN_2055 GBV_ILN_2056 GBV_ILN_2057 GBV_ILN_2059 GBV_ILN_2061 GBV_ILN_2064 GBV_ILN_2065 GBV_ILN_2068 GBV_ILN_2088 GBV_ILN_2093 GBV_ILN_2106 GBV_ILN_2107 GBV_ILN_2108 GBV_ILN_2110 GBV_ILN_2111 GBV_ILN_2112 GBV_ILN_2113 GBV_ILN_2118 GBV_ILN_2122 GBV_ILN_2129 GBV_ILN_2143 GBV_ILN_2144 GBV_ILN_2147 GBV_ILN_2148 GBV_ILN_2152 GBV_ILN_2153 GBV_ILN_2188 GBV_ILN_2190 GBV_ILN_2232 GBV_ILN_2336 GBV_ILN_2446 GBV_ILN_2470 GBV_ILN_2472 GBV_ILN_2507 GBV_ILN_2522 GBV_ILN_2548 GBV_ILN_4035 GBV_ILN_4037 GBV_ILN_4046 GBV_ILN_4112 GBV_ILN_4125 GBV_ILN_4126 GBV_ILN_4242 GBV_ILN_4246 GBV_ILN_4249 GBV_ILN_4251 GBV_ILN_4305 GBV_ILN_4306 GBV_ILN_4307 GBV_ILN_4313 GBV_ILN_4322 GBV_ILN_4323 GBV_ILN_4324 GBV_ILN_4325 GBV_ILN_4326 GBV_ILN_4328 GBV_ILN_4333 GBV_ILN_4334 GBV_ILN_4335 GBV_ILN_4336 GBV_ILN_4338 GBV_ILN_4393 GBV_ILN_4700 AR 17 2024 7 11 04 6274-6280 |
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Feng, Yanghao @@aut@@ Zhang, Wendi @@aut@@ Tang, Kunpeng @@aut@@ Chen, Yingzhi @@aut@@ Zhang, Jiou @@aut@@ Cao, Kecheng @@aut@@ Cui, Weili @@aut@@ Shi, Lei @@aut@@ |
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<?xml version="1.0" encoding="UTF-8"?><collection xmlns="http://www.loc.gov/MARC21/slim"><record><leader>01000naa a22002652 4500</leader><controlfield tag="001">SPR056460171</controlfield><controlfield tag="003">DE-627</controlfield><controlfield tag="005">20240704064720.0</controlfield><controlfield tag="007">cr uuu---uuuuu</controlfield><controlfield tag="008">240704s2024 xx |||||o 00| ||eng c</controlfield><datafield tag="024" ind1="7" ind2=" "><subfield code="a">10.1007/s12274-024-6571-z</subfield><subfield code="2">doi</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(DE-627)SPR056460171</subfield></datafield><datafield tag="035" ind1=" " ind2=" "><subfield code="a">(SPR)s12274-024-6571-z-e</subfield></datafield><datafield tag="040" ind1=" " ind2=" "><subfield code="a">DE-627</subfield><subfield code="b">ger</subfield><subfield code="c">DE-627</subfield><subfield code="e">rakwb</subfield></datafield><datafield tag="041" ind1=" " ind2=" "><subfield code="a">eng</subfield></datafield><datafield tag="082" ind1="0" ind2="4"><subfield code="a">540</subfield><subfield code="a">660</subfield><subfield code="q">VZ</subfield></datafield><datafield tag="100" ind1="1" ind2=" "><subfield code="a">Feng, Yanghao</subfield><subfield code="e">verfasserin</subfield><subfield code="4">aut</subfield></datafield><datafield tag="245" ind1="1" ind2="0"><subfield code="a">A robust synthesis route of confined carbyne</subfield></datafield><datafield tag="264" ind1=" " ind2="1"><subfield code="c">2024</subfield></datafield><datafield tag="336" ind1=" " ind2=" "><subfield code="a">Text</subfield><subfield code="b">txt</subfield><subfield code="2">rdacontent</subfield></datafield><datafield tag="337" ind1=" " ind2=" "><subfield code="a">Computermedien</subfield><subfield code="b">c</subfield><subfield code="2">rdamedia</subfield></datafield><datafield tag="338" ind1=" " ind2=" "><subfield code="a">Online-Ressource</subfield><subfield code="b">cr</subfield><subfield code="2">rdacarrier</subfield></datafield><datafield tag="500" ind1=" " ind2=" "><subfield code="a">© Tsinghua University Press 2024</subfield></datafield><datafield tag="520" ind1=" " ind2=" "><subfield code="a">Abstract The unique mechanical, optical, and electrical properties of carbyne, a one-dimensional allotrope of carbon, make it a highly promising material for various applications. It has been demonstrated that carbon nanotubes (CNTs) can serve as an ideal host for the formation of confined carbyne (CC), with the yield being influenced by the quality of the carbon nanotubes for confinement and the carbon source for carbyne growth. In this study, a robust synthesis route of CC within CNTs is proposed. $ C_{70} $ was utilized as a precursor to provide an additional carbon source, based on its ability to supply more carbon atoms than $ C_{60} $ at the same filling ratio. Multi-step transformation processes, including defect creation, were designed to enhance the yield of CC. As a result, the yield of CC was significantly increased for the $ C_{70} $ encapsulated single-walled CNTs by more than an order of magnitude than the empty counterparts, which also surpasses that of the double-walled CNTs, making it the most effective route for synthesizing CC. 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| author |
Feng, Yanghao |
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Feng, Yanghao ddc 540 misc confined carbyne misc yield enhancement misc carbon nanotube misc C misc encapsulation misc defect introduction misc Raman spectroscopy A robust synthesis route of confined carbyne |
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540 660 VZ A robust synthesis route of confined carbyne confined carbyne (dpeaa)DE-He213 yield enhancement (dpeaa)DE-He213 carbon nanotube (dpeaa)DE-He213 C (dpeaa)DE-He213 encapsulation (dpeaa)DE-He213 defect introduction (dpeaa)DE-He213 Raman spectroscopy (dpeaa)DE-He213 |
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ddc 540 misc confined carbyne misc yield enhancement misc carbon nanotube misc C misc encapsulation misc defect introduction misc Raman spectroscopy |
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ddc 540 misc confined carbyne misc yield enhancement misc carbon nanotube misc C misc encapsulation misc defect introduction misc Raman spectroscopy |
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A robust synthesis route of confined carbyne |
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Feng, Yanghao Zhang, Wendi Tang, Kunpeng Chen, Yingzhi Zhang, Jiou Cao, Kecheng Cui, Weili Shi, Lei |
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a robust synthesis route of confined carbyne |
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A robust synthesis route of confined carbyne |
| abstract |
Abstract The unique mechanical, optical, and electrical properties of carbyne, a one-dimensional allotrope of carbon, make it a highly promising material for various applications. It has been demonstrated that carbon nanotubes (CNTs) can serve as an ideal host for the formation of confined carbyne (CC), with the yield being influenced by the quality of the carbon nanotubes for confinement and the carbon source for carbyne growth. In this study, a robust synthesis route of CC within CNTs is proposed. $ C_{70} $ was utilized as a precursor to provide an additional carbon source, based on its ability to supply more carbon atoms than $ C_{60} $ at the same filling ratio. Multi-step transformation processes, including defect creation, were designed to enhance the yield of CC. As a result, the yield of CC was significantly increased for the $ C_{70} $ encapsulated single-walled CNTs by more than an order of magnitude than the empty counterparts, which also surpasses that of the double-walled CNTs, making it the most effective route for synthesizing CC. These findings highlight the importance of the additional carbon source and the optimal pathway for CC formation, offering valuable insights for the application of materials with high yield. © Tsinghua University Press 2024 |
| abstractGer |
Abstract The unique mechanical, optical, and electrical properties of carbyne, a one-dimensional allotrope of carbon, make it a highly promising material for various applications. It has been demonstrated that carbon nanotubes (CNTs) can serve as an ideal host for the formation of confined carbyne (CC), with the yield being influenced by the quality of the carbon nanotubes for confinement and the carbon source for carbyne growth. In this study, a robust synthesis route of CC within CNTs is proposed. $ C_{70} $ was utilized as a precursor to provide an additional carbon source, based on its ability to supply more carbon atoms than $ C_{60} $ at the same filling ratio. Multi-step transformation processes, including defect creation, were designed to enhance the yield of CC. As a result, the yield of CC was significantly increased for the $ C_{70} $ encapsulated single-walled CNTs by more than an order of magnitude than the empty counterparts, which also surpasses that of the double-walled CNTs, making it the most effective route for synthesizing CC. These findings highlight the importance of the additional carbon source and the optimal pathway for CC formation, offering valuable insights for the application of materials with high yield. © Tsinghua University Press 2024 |
| abstract_unstemmed |
Abstract The unique mechanical, optical, and electrical properties of carbyne, a one-dimensional allotrope of carbon, make it a highly promising material for various applications. It has been demonstrated that carbon nanotubes (CNTs) can serve as an ideal host for the formation of confined carbyne (CC), with the yield being influenced by the quality of the carbon nanotubes for confinement and the carbon source for carbyne growth. In this study, a robust synthesis route of CC within CNTs is proposed. $ C_{70} $ was utilized as a precursor to provide an additional carbon source, based on its ability to supply more carbon atoms than $ C_{60} $ at the same filling ratio. Multi-step transformation processes, including defect creation, were designed to enhance the yield of CC. As a result, the yield of CC was significantly increased for the $ C_{70} $ encapsulated single-walled CNTs by more than an order of magnitude than the empty counterparts, which also surpasses that of the double-walled CNTs, making it the most effective route for synthesizing CC. These findings highlight the importance of the additional carbon source and the optimal pathway for CC formation, offering valuable insights for the application of materials with high yield. © Tsinghua University Press 2024 |
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| title_short |
A robust synthesis route of confined carbyne |
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https://dx.doi.org/10.1007/s12274-024-6571-z |
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| author2 |
Zhang, Wendi Tang, Kunpeng Chen, Yingzhi Zhang, Jiou Cao, Kecheng Cui, Weili Shi, Lei |
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Zhang, Wendi Tang, Kunpeng Chen, Yingzhi Zhang, Jiou Cao, Kecheng Cui, Weili Shi, Lei |
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10.1007/s12274-024-6571-z |
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| score |
7.399952 |